热带气旋–热浪复合事件对珠三角暖季臭氧污染的影响

刘雨林, 黎梓欣, 吴燕星, 刘润

中国环境科学 ›› 2025, Vol. 45 ›› Issue (12) : 6552-6559.

PDF(3370 KB)
PDF(3370 KB)
中国环境科学 ›› 2025, Vol. 45 ›› Issue (12) : 6552-6559.
大气污染与控制

热带气旋–热浪复合事件对珠三角暖季臭氧污染的影响

  • 刘雨林1, 黎梓欣1, 吴燕星1, 刘润1,2
作者信息 +

Impact of tropical cyclone-heatwave compound events on ozone pollution in the Pearl River Delta during the warm season

  • LIU Yu-lin1, LI Zi-xin1, WU Yan-xing1, LIU Run1,2
Author information +
文章历史 +

摘要

基于2015~2023年暖季(6~9月)珠三角臭氧(O3)每小时浓度数据、热带气旋数据和气象再分析数据,对比分析其他事件、单独热浪事件(HW)、单独热带气旋事件(TC)和热带气旋-热浪复合事件(TC–HW)对珠三角O3的影响以及与O3污染事件的年际变化关系.结果表明,TC–HW复合事件发生时,珠三角O3浓度为(143.8±41.7) μg/m3,O3浓度的平均增长率为21.4%,O3超标率为36.8%.相比于其他事件、单独HW事件和单独TC事件,TC–HW复合事件使整个珠三角区域O3浓度提高了38.3 μg/m3.TC–HW复合事件与珠三角O3污染事件的年际变化呈现显著的正相关关系,其相关系数为0.68(P<0.05).TC–HW复合事件期间低云量、低湿度、低风速和强太阳辐射是导致珠三角O3污染事件发生的关键气象因素.

Abstract

Based on the hourly ozone (O3) concentration data, tropical cyclone (TC) data and meteorological reanalysis data in the Pearl River Delta (PRD) during the warm season (June-September) from 2015 to 2023, the impacts of various meteorological events, including isolated heat wave (HW) events, isolated TC events, and TC-HW compound events on O3 in PRD and their interannual variation relationship with O3 pollution events were compared and analyzed. The results showed that TC-HW compound events were associated with an average O3 concentration of (143.8±41.7) μg/m3, representing a mean growth rate of 21.4%, and a 36.8% likelihood of O3 pollution occurrence. Compared with other event categories, TC-HW compound events lead to an average regional O3 increase of 38.3μg/m3. A statistically significant positive correlation (r=0.68, P<0.05) was identified between the frequency of TC-HW compound events and the interannual variability of O3 pollution episodes. Meteorological conditions characterized by reduced cloud cover, low relative humidity, weakened wind speed, and enhanced solar radiation during the TC-HW compound events were identified as key drivers of increased O3 concentrations in the PRD.

关键词

热带气旋-热浪复合事件(TC–HW) / O3污染事件 / 年际变化 / 珠三角(PRD)

Key words

tropical cyclone-heatwave compound events (TC-HW) / O3 pollution events / interannual variation / Pearl River Delta (PRD)

引用本文

导出引用
刘雨林, 黎梓欣, 吴燕星, 刘润. 热带气旋–热浪复合事件对珠三角暖季臭氧污染的影响[J]. 中国环境科学. 2025, 45(12): 6552-6559
LIU Yu-lin, LI Zi-xin, WU Yan-xing, LIU Run. Impact of tropical cyclone-heatwave compound events on ozone pollution in the Pearl River Delta during the warm season[J]. China Environmental Science. 2025, 45(12): 6552-6559
中图分类号: X511   

参考文献

[1] Wang Y, Gao W, Wang S, et al. Contrasting trends of PM2.5 and surface-ozone concentrations in China from 2013 to 2017 [J]. National Science Review, 2020,7(8):1331-1339.
[2] Ding A, Huang X, Nie W, et al. Significant reduction of PM2.5 in eastern China due to regional-scale emission control: evidence from SORPES in 2011~2018 [J]. Atmospheric Chemistry and Physics, 2019, 19(18):11791-11801.
[3] Ren J, Guo F, Xie S. Diagnosing ozone-NOx-VOC sensitivity and revealing causes of ozone increases in China based on 2013~2021 satellite retrievals [J]. Atmospheric Chemistry and Physics, 2022, 22(22):15035-15047.
[4] Sicard P, Agathokleous E, Anenberg S C, et al. Trends in urban air pollution over the last two decades: a global perspective [J]. Science of The Total Environment, 2023,858:160064.
[5] Du S, He C, Zhang L, et al. Policy implications for synergistic management of PM2.5 and O3 pollution from a pattern-process-sustainability perspective in China [J]. Science of the Total Environment, 2024,916:170210.
[6] Fu Y, Liao H, Yang Y. Interannual and decadal changes in tropospheric ozone in China and the associated chemistry-climate interactions: a review [J]. Advances in Atmospheric Sciences, 2019,36(9):975-993.
[7] Li K, Jacob D J, Shen L, et al. Increases in surface ozone pollution in China from 2013 to 2019: anthropogenic and meteorological influences [J]. Atmospheric Chemistry and Physics, 2020,20(19): 11423-11433.
[8] Liu H, Liu S, Xue B, et al. Ground-level ozone pollution and its health impacts in China [J]. Atmospheric Environment, 2018,173:223-230.
[9] Yue X, Unger N, Harper K, et al. Ozone and haze pollution weakens net primary productivity in China [J]. Atmospheric Chemistry and Physics, 2017,17(9):6073-6089.
[10] 沈 劲,杨土士,晏平仲,等.广东省臭氧污染特征及其成因分析 [J]. 环境科学与技术, 2020,43(12):90-95. Shen J, Yang T S, Yan P Z, et al. Characteristics and causes of ozone pollution in Guangdong Province [J]. Environmental Science & Technology, 2020,43(12):90-95.
[11] 王 芃,朱盛强,张梦媛,等.大气氧化性及其对二次污染物形成的贡献 [J]. 科学通报, 2022,67(18):2069-2078. Wang P, Zhu S Q, Zhang M Y, et al. Atmospheric oxidation capacity and its contribution to secondary pollutants formation [J]. Chinese Science Bulletin, 2022,67(18):2069-2078.
[12] Lu Y, Wang T. Decisive role of atmospheric circulation in the troposphere on ozone pollution in the Beijing-Tianjin-Hebei region [J]. Atmospheric Pollution Research, 2024,15(3):102024.
[13] Han H, Liu J, Shu L, et al. Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China [J]. Atmospheric Chemistry and Physics, 2020,20(1):203-222.
[14] Yan D, Zhang Z, Jin Z, et al. Ozone variability driven by the synoptic patterns over China during 2014~2022 and its implications for crop yield and economy [J]. Atmospheric Pollution Research, 2023,14(9): 101843.
[15] 胡安琪,谢晓栋,龚康佳,等.气候变化对中国夏季臭氧影响 [J]. 环境科学, 2023,44(4):1801-1810. Hu A Q, Xiao X D, Gong K J, et al. Impact of climate change on summer ozone in China [J]. Environmental Science, 2023,44(4): 1801-1810.
[16] Lu P, Liu R, Luo Z, et al. Impacts of compound extreme weather events on summer ozone in the Beijing-Tianjin-Hebei region [J]. Atmospheric Pollution Research, 2024,15(3):102030.
[17] Pu X, Wang T, Huang X, et al. Enhanced surface ozone during the heat wave of 2013 in Yangtze River Delta region, China [J]. Science of the Total Environment, 2017,603-604:807-816.
[18] Wang P, Yang Y, Li H, et al. North China Plain as a hot spot of ozone pollution exacerbated by extreme high temperatures [J]. Atmospheric Chemistry and Physics, 2022,22(7):4705-4719.
[19] Wang L, Yang X, Dong J, et al. Evolution of surface ozone pollution pattern in eastern China and its relationship with different intensity heatwaves [J]. Environmental Pollution, 2023,338:122725.
[20] 丁嘉豪,谢晓栋,龚康佳,等.2014~2020年夏季高温热浪期间臭氧变化特征--以长三角地区典型城市为例 [J]. 中国环境科学, 2024,44 (12):6549-6558. Ding J H, Xie X D, Gong K J, et al. Characteristics of ozone variations during summer heat waves in typical cities in the Yangtze River Delta Region from 2014 to 2020 [J]. China Environment Science, 2024,44 (12):6549-6558.
[21] Li M, Yang Y, Wang H, et al. Unique impacts of strong and westward-extended western Pacific subtropical high on ozone pollution over eastern China [J]. Environmental Pollution, 2024,358:124515.
[22] Lu S, Gong S, Chen J, et al. Composite effects of ENSO and EASM on summer ozone pollution in two regions of China [J]. Journal of Geophysical Research: Atmospheres, 2022,127(22):e2022JD036938.
[23] Zhou Y, Yang Y, Wang H, et al. Summer ozone pollution in China affected by the intensity of Asian monsoon systems [J]. Science of the Total Environment, 2022,849:157785.
[24] Ding H, Kong L, You Y, et al. Effects of tropical cyclones with different tracks on ozone pollution over the Pearl River Delta region [J]. Atmospheric Research, 2023,286:106680.
[25] Wang R, Bei N, Hu B, et al. The relationship between the intensified heat waves and deteriorated summertime ozone pollution in the Beijing-Tianjin-Hebei region, China, during 2013~2017 [J]. Environmental Pollution, 2022,314:120256.
[26] Xu J, Zhao Z, Wu Y, et al. Impacts of meteorological conditions on autumn surface ozone during 2014~2020 in the Pearl River Delta, China [J]. Earth and Space Science, 2023,10(2):e2022EA002742.
[27] Liu C, He C, Wang Y, et al. Characteristics and mechanism of a persistent ozone pollution event in Pearl River Delta induced by typhoon and subtropical high [J]. Atmospheric Environment, 2023, 310:119964.
[28] Deng T, Wang T, Wang S, et al. Impact of typhoon periphery on high ozone and high aerosol pollution in the Pearl River Delta region [J]. Science of the Total Environment, 2019,668:617-630.
[29] Lam Y, Cheung H, Ying C. Impact of tropical cyclone track change on regional air quality [J]. Science of The Total Environment, 2018,610-611:1347-1355.
[30] Lin X, Yuan Z, Yang L, et al. Impact of extreme meteorological events on ozone in the Pearl River Delta, China [J]. Aerosol and Air Quality Research, 2019,19(6):1307-1324.
[31] Xiao Y, Duan Z, Xiao Y, et al. Typhoon wind hazard analysis for southeast China coastal regions [J]. Structural Safety, 2011,33(4/5): 286-295.
[32] Wang P, Yang Y, Xue D, et al. Increasing compound hazards of tropical cyclones and heatwaves over southeastern coast of China under climate warming [J]. Journal of Climate, 2023,36(7):2243-2257.
[33] Zhang M, Yang Y, Zhan C, et al. Tropical cyclone-related heatwave episodes in the Greater Bay Area, China: synoptic patterns and urban-rural disparities [J]. Weather and Climate Extremes, 2024,44:100656.
[34] Hu T, Lin Y, Liu R, et al. What caused large ozone variabilities in three megacity clusters in eastern China during 2015~2020? [J]. Atmospheric Chemistry and Physics, 2024,24(3):1607-1626.
[35] Hu W, Liu R, Chen Z, et al. Processes conducive to high ozone formation in Pearl River Delta in the presence of pacific tropical cyclones [J]. Atmospheric Environment, 2023,307:119859.
[36] Matthews T, Wilby R, Murphy C. An emerging tropical cyclone-deadly heat compound hazard [J]. Nature Climate Change, 2019, 9(8):602-606.
[37] GB 3095-2012 环境空气质量标准 [S]. GB 3095-2012 Ambient air quality standard [S].
[38] Huang Z, Luo M, Gao M, et al. Different characteristics of independent and compound extreme heat and ozone pollution events in the Greater Bay Area of China [J]. International Journal of Applied Earth Observation and Geoinformation, 2023,124:103508.
[39] Qi C, Wang P, Yang Y, et al. Impacts of tropical cyclone-heat wave compound events on surface ozone in eastern China: comparison between the Yangtze River and Pearl River Deltas [J]. Atmospheric Chemistry and Physics, 2024,24(20):11775-11789.
[40] Wang T, Zhong Z, Sun Y, et al. Impacts of tropical cyclones on the meridional movement of the western Pacific subtropical high [J]. Atmospheric Science Letters, 2019,20(5):e893.
[41] Chang L, Xu J, Tie X, et al. The impact of climate change on the western Pacific subtropical high and the related ozone pollution in Shanghai, China [J]. Scientific Reports, 2019,9(1):16998.
[42] Shen L, Diao Y, Zhao T, et al. Meteorological influence on persistent O3pollution events in Wuxi in the Yangtze River Delta, China [J]. Science of the Total Environment, 2024,917:170484.
[43] 米艺华,杜惠云,李 杰,等.我国重点地区臭氧变化特征及与气象要素的关系 [J]. 中国环境科学, 2024,44(4):1894-1904. Mi Y H, Du H Y, Li J, et al. Ozone pollution characteristics and its relationship with meteorological factors of key regions in China [J]. China Environmental Science, 44(4):1894-1904.
[44] 邬双双,陈梓超,薛 鑫,等.基于KZ滤波分析气象对珠三角臭氧趋势的影响 [J]. 中国环境科学, 2024,44(4):1905-1911. Wu S S, Chen Z C, Xue X, et al. Analysis of meteorological effects on the trend of ozone in the Pearl River Delta using the KZ filtering method [J]. China Environmental Science, 2024,44(4):1905-1911.
[45] Yang X, Zeng G, Iyakaremye V, et al. Effects of different types of heat wave days on ozone pollution over Beijing-Tianjin-Hebei and its future projection [J]. Science of the Total Environment, 2022,837: 155762.
[46] 单文坡,殷永泉,杜世勇,等.夏季城市大气O3浓度影响因素及其相关关系 [J]. 环境科学, 2006,27(7):1276-1281. Shan W P, Yin Y Q, Du S Y, et al. Ozone pollution, influence factors and their correlation at urban area in summer [J]. Environmental Science, 2006,27(7):1276-1281.
[47] Kou W, Gao Y, Zhang S, et al. High downward surface solar radiation conducive to ozone pollution more frequent under global warming [J]. Science Bulletin, 2023,68(4):388-392.
[48] Dang R, Liao H, Fu Y. Quantifying the anthropogenic and meteorological influences on summertime surface ozone in China over 2012~2017 [J]. Science of The Total Environment, 2021,754:142394.
[49] Liao W, Wu L, Zhou S, et al. Impact of synoptic weather types on ground-level ozone concentrations in Guangzhou, China [J]. Asia-Pacific Journal of Atmospheric Sciences, 2021,57(2):169-180.
[50] Li K, Jacob D J, Liao H, et al. Anthropogenic drivers of 2013~2017 trends in summer surface ozone in China [J]. Proceedings of the National Academy of Sciences, 2019,116(2):422-427.
[51] 赵 伟,吕梦瑶,卢 清,等.热带气旋对珠三角秋季臭氧污染的影响 [J]. 环境科学, 2022,43(6):2957-2965. Zhao W, Lv M Y, Lu Q, et al. Effects of typical cyclones on ozone pollution in the Pearl River Delta in autumn [J]. Environmental Science, 2022,43(6):2957-2965.
[52] Ouyang S, Deng T, Liu R, et al. Impact of a subtropical high and a typhoon on a severe ozone pollution episode in the Pearl River Delta, China [J]. Atmospheric Chemistry and Physics, 2022,22(16):10751-10767.
[53] 董少柔,林爱兰,董彦彤.1961~2017年华南区域性持续高温过程年际变化成因分析 [J]. 大气科学, 2023,47(5):1325-1340. Dong S R, Lin A L, Dong Y T. Analysis of interannual variation of regionally persistent high-temperature events in South China during 1961~2017 [J]. Chinese Journal of Atmospheric Sciences, 2023,47(5): 1325-1340.
[54] 王 宁,马梁臣,霍 也.一次爆发性气旋引发东北地区暴雨成因分析 [J]. 气象与环境学报, 2022,38(3):19-28. Wang N, Mang L C, Huo Y. Analysis of rainstorm caused by an explosive cyclone in Northeast China [J]. Journal of Meteorology and Environment, 2022,38(3):19-28.

基金

国家重点研发计划项目(2023YFC3706204)

PDF(3370 KB)

Accesses

Citation

Detail

段落导航
相关文章

/

〈 〉