Anthropogenic ammonia emission inventories of Zhejiang Province from 2013 to 2020

LU Sheng-kun; CHAO Na; CHEN Jin-yuan; WANG Qiong-zhen; WANG Hui

PDF(1459 KB)

China Environmental Science ›› 2022, Vol. 42 ›› Issue (10) : 4525-4536.

Air Pollution Control

Anthropogenic ammonia emission inventories of Zhejiang Province from 2013 to 2020

LU Sheng-kun¹, CHAO Na², CHEN Jin-yuan¹, WANG Qiong-zhen², WANG Hui³

Author information +

History +

Abstract

The anthropogenic ammonia emission inventories of Zhejiang Province from 2013~2020 were developed by using the emission factors method,, and the spatial distribution was carried out based on the ArcGIS software. The connection between ammonia emissions and NH₄⁺ concentration in PM_2.5 components of several cities in Zhejiang Province was also researched in this study. The results showed that anthropogenic ammonia emissions in Zhejiang Province from 2013~2020 decreased year by year. The ammonia emisson in 2020 was 13.5×10⁴t, decreased by 23.1% compared with 2013. Agricultural sources were a major source of anthropogenic NH₃ emissions, which accounted for 57.2%~69.6% of the total ammonia emssions from 2013~2020. The livestock and nitrogen fertilizer application shared high proportion of agricultural NH₃emissions, and the emissions of these two sources in 2020 decreased most significantly compared to the previous years, with 34.5% and 44.1% respectively. The spatial distribution results showed that regions with higher ammonia emissios mainly distributed in the north of Zhejiang Province and Jinqu Basin. The emisisons of Hangzhou and Jiaxing ranked the top two in Zhejiang Province. Cities with higher ammonia emissions also had higher NH₄⁺ concentration, and the downtrend of NH₄⁺ concentration in some cities was consistent with that of ammonia emissions

Key words

ammonia emission inventory / anthropogenic sources / interannual variation / NH₄⁺ / spatial distribution / Zhejiang Province

Cite this article

EndNote

Ris (Procite)

Bibtex

Download Citations

LU Sheng-kun, CHAO Na, CHEN Jin-yuan, WANG Qiong-zhen, WANG Hui. Anthropogenic ammonia emission inventories of Zhejiang Province from 2013 to 2020[J]. China Environmental Science. 2022, 42(10): 4525-4536

References

[1] 许中坚,刘广深,俞佳栋.氮循环的人为干扰与土壤酸化[J].地质地球化学, 2002,30(2):74-78.Xu Z J, Liu G S, Yu J D.Anthropogenic disturbance of nitrogen cycle and soil acidification[J].Geology and Geochemistry, 2002,30(2):74-78.
[2] Hamaoui-laguel L, Meleux F, Beekmann M, et al.Improving ammonia emissions in air quality modelling for france[J].Atmospheric Environment, 2014,92:584-595.
[3] 林岩,段雷,杨永森,等.模拟氮沉降对高硫沉降地区森林土壤酸化的贡献[J].环境科学, 2007,28(3):640-646.Lin Y, Duan L, Yang Y S, et al.Contribution of simulated nitrogen deposition to soil acidification in high sulfur sedimentation areas[J].Environmental Science, 2007,28(3):640-646.
[4] Kruse M, Apsimon H M, Bell J N B.Validity and uncertainty in the calculation of an emission inventory for ammonia arising from agriculture in Great Britain[J].Environmental Pollution, 1989,56(3):237-257.
[5] Sutton M A, Place C J, Eager M, et al.Assessment of the magnitude of ammonia emissions in the United Kingdom[J].Atmospheric Environment, 1995,29(12):1393-1411.
[6] Zhou Y, Cheng S, Lang J, et al.A comprehensive ammonia emission inventory with high-resolution and its evaluation in the Beijing-Tianjin-Hebei (BTH) region, China[J].Atmospheric Environment, 2015,106:305-317.
[7] 尹沙沙.珠江三角洲人为源氨排放清单及其对颗粒物形成贡献的研究[D].广州:华南理工大学, 2011.Yin S S.Anthropogenic Ammonia Emission Inventory in pearl river delta and its contribution to particulate matter formation[D].Guangzhou:South China University of Technology, 2011.
[8] 董艳强,陈长虹,黄成,等.长江三角洲地区人为源氨排放清单及分布特征[J].环境科学学报, 2009,29(8):1611-1617.Dong Y Q, Chen C H, Hung C, et al.Inventory and distribution characteristics of anthropogenic ammonia emissions from sources in the Yangtze River Delta region[J].Journal of Environmental Science, 2009,29(8):1611-1617.
[9] 冯小琼,陈军辉,姜涛,等.四川省2005~2014年农业源氨排放清单及分布特征[J].环境科学, 2017,38(7):2728-2737.Feng X Q, Chen J H, Jiang T, et al.Inventory and distribution characteristics of ammonia emissions from agricultural sources in Sichuan Province from 2005 to 2014[J].Environmental Science, 2017,38(7):2728-2737.
[10] 覃思,孔少飞,吴剑,等.1996~2016年湖北省氨排放时空差异及影响因素[J].中国环境科学, 2020,40(4):1403-1413.Qin S, Kong S F, Wu J, et al.Spatial-temporal differences and influencing factors of ammonia emissions in Hubei Province from 1996 to 2016[J].Chinese Environmental Science, 2020,40(4):1403-1413.
[11] Wu S P, Zhang Y J, Schwab J J, et al.High-resolution ammonia emissions inventories in Fujian, China, 2009~2015[J].Atmospheric Environment, 2017,162:100-114.
[12] 余飞翔,晁娜,吴建,等.浙江省2013年农业源氨排放清单研究[J].环境污染与防治, 2016,38(10):41-46.Yu F X, Chao N, Wu J, et al.Ammonia Emission Inventory from Agricultural Sources in Zhejiang Province in 2013[J].Environmental Pollution and Prevention, 2016,38(10):41-46.
[13] 赵睿东,于兴娜,侯新红,等.浙江省人为源氨排放清单建立及分布特征[J].环境科学, 2020,41(9):3976-3984.Zhao R D, Yu X N, Hou X H, et al.Establishment and distribution characteristics of anthropogenic ammonia emissions from anthropogenic sources in Zhejiang Province[J].Environmental Science, 2020,41(9):3976-3984.
[14] 浙江省人民政府.浙江省人民政府关于印发浙江省大气污染防治行动计划(2013~2017年)的通知[Z].浙江省人民政府公报, 2015,(Z3):27-40.People's Government of Zhejiang Province.Notice of the People's Government of Zhejiang Province on printing and distributing the action plan for the prevention and control of air pollution in Zhejiang Province (2013~2017)[Z].Bulletin of the People's Government of Zhejiang Province, 2015,(Z3):27-40.
[15] 浙江省人民政府.浙江省人民政府关于印发浙江省打赢蓝天保卫战三年行动计划的通知[Z].浙江省人民政府公报, 2018,(24):3-28.People's Government of Zhejiang Province.Notice of the People's Government of Zhejiang Province on printing and distributing the three-year action plan for Zhejiang Province to win the blue sky defense war[Z].Communiqué of the People's Government of Zhejiang Province, 2018,(24):3-28.
[16] 生态环境部.大气氨源排放清单编制技术指南(试行)[R].北京:生态环境部, 2014.Ministry of Ecology and Environment.Technical guidelines for the preparation of atmospheric ammonia emission inventories (trial implementation)[R].Beijing:Ministry of Ecology and Environment 2014.
[17] 住房和城乡建设部.中国城市建设统计年鉴2013~2020[M].北京:中国统计出版社, 2020.Ministry of Housing and Urban-Rural Development.Statistical yearbook of China's urban construction 2013~2020[M].Beijing:China Statistics Press, 2020.
[18] 国家统计局能源统计司.中国能源统计年鉴2014~2020[M].北京:中国统计出版社, 2020.Department of Energy Statistics, National Bureau of Statistics.China energy statistics yearbook 2014~2020[M].Beijing:China Statistics Press, 2020.
[19] 浙江省统计局.浙江统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Zhejiang Provincial Bureau of Statistics.Zhejiang statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[20] 杭州市统计局.杭州统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Hangzhou Municipal Bureau of Statistics.Hangzhou statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[21] 湖州市统计局.湖州统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Huzhou Municipal Bureau of Statistics.Huzhou statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[22] 嘉兴市统计局.嘉兴统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Jiaxing Municipal Bureau of Statistics.Jiaxing statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[23] 金华市统计局.金华统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Jinhua Municipal Bureau of Statistics.Jinhua statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[24] 丽水市统计局.丽水统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Lishui Municipal Bureau of Statistics.Lishui statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[25] 宁波市统计局.宁波统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Ningbo Municipal Bureau of Statistics.Ningbo statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[26] 衢州市统计局.衢州统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Quzhou Municipal Bureau of Statistics.Quzhou statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[27] 绍兴市统计局.绍兴统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Shaoxing Municipal Bureau of Statistics.Shaoxing statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[28] 台州市统计局.台州统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Taizhou Municipal Bureau of Statistics.Taizhou statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[29] 温州市统计局.温州统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Wenzhou Municipal Bureau of Statistics.Wenzhou statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[30] 舟山市统计局.舟山统计年鉴2014~2021[M].北京:中国统计出版社, 2021.Zhoushan Municipal Bureau of Statistics.Zhoushan statistical yearbook 2014~2021[M].Beijing:China Statistics Press, 2021.
[31] 浙江省农业农村厅.浙江省畜牧业"十三五"规划(浙农计发[2016] 18号)[EB/OL].http://law.foodmate.net/show-194958.html, 2022.4.24.Department of Agriculture and Rural Affairs of Zhejiang Province.Zhejiang animal husbandry "13th Five-Year Plan" (Zhejiang Nongjifa[2016] No.18)[EB/OL].http://law.foodmate.net/show-194958.html.2022.4.24.
[32] 王琛,尹沙沙,于世杰,等.河南省2013年大气氨排放清单建立及分布特征[J].环境科学, 2018,39(3):1023-1030.Wang C, Yin S S, Yu S J, et al.Establishment and distribution characteristics of atmospheric ammonia emission inventory in Henan Province in 2013[J].Environmental Science, 2018,39(3):1023-1030.
[33] 杨志鹏.基于物质流方法的中国畜牧业氨排放估算及区域比较研究[D].北京:北京大学, 2008.Yang Z P.Estimation and regional comparison of ammonia emissions from animal husbandry in China based on material flow method[D].Beijing:Peking University, 2008.
[34] 巨晓棠和谷保静.我国农田氮肥施用现状、问题及趋势[J].植物营养与肥料学报, 2014,20(4):783-795.Ju X T and Gu B J.Current situation, problems and trends of nitrogen fertilizer application in farmland in China[J].Journal of Plant Nutrition and Fertilizer, 2014,20(4):783-795.
[35] 毕于运.秸秆资源评价与利用研究[D].北京:中国农业科学院, 2010.Bi Y Y.Evaluation and utilization of straw resources[D].Beijing:Chinese Academy of Agricultural Sciences, 2010.
[36] 浙江省生态环境厅.关于发布《浙江省第二次全国污染源普查公报》的公告[R].杭州:浙江省生态环境厅, 2020.Department of Ecology and Environment of Zhejiang Province.Announcement on the publication of the communique of the second national pollution source census of Zhejiang Province[R].Hangzhou:Department of Ecology and Environment of Zhejiang Province, 2020.
[37] 董文煊,邢佳,王书肖.1994~2006年中国人为源大气氨排放时空分布[J].环境科学, 2010,31(7):1457-1463.Dong W X, Xing J, Wang S X.Spatio-temporal distribution of atmospheric ammonia emissions from Chinese sources from 1994 to 2006[J].Environmental Science, 2010,31(7):1457-1463.
[38] US EPA.AP-42:Compilation of Air Emissions Factors[R].Washington D.C.:US EPA, 1995.
[39] IIASA.Emission stage-specific NH₃ emission factors for livestock categories[R].Austria:International Institute for Applied Systems Analysis, 2010.
[40] Sutton M A, Dragosits U, Tang Y S, et al.Ammonia emissions from non-agricultural sources in the UK[J].Atmospheric Environment, 2000,34(6):855-869.
[41] 曹国良,张小曳,王丹,等.中国大陆生物质燃烧排放的污染物清单[J].中国环境科学, 2005,25(4):389-393.Cao G L, Zhang X Y, Wang D, et al.List of pollutants emitted by Chinese mainland biomass combustion[J].China Environmental Science, 2005,25(4):389-393.
[42] 王丽,李雪铭,许妍.中国大陆秸秆露天焚烧的经济损失研究[J].干旱区资源与环境, 2008,(2):170-175.Wang L, Li X M, Xu Y.A study on the economic loss of open burning of Chinese mainland straw[J].Resources and Environment in Arid Areas, 2008,(2):170-175.
[43] 李冰洁,陈金媛,刘铮铮,等.浙江省大气颗粒物PM_2.5中全氟化合物污染特征分析及健康风险评估[J].环境科学, 2022,43(2):639-648.Li B J, Chen J Y, Liu Z Z, et al.Analysis of perfluorinated compound pollution characteristics and health risk assessment in PM_2.5 atmospheric particulate matter in Zhejiang Province[J].Environmental Science, 2022,43(2):639-648.
[44] 赵佳佳.杭州市细颗粒物(PM_2.5)源解析研究[D].杭州:浙江工业大学, 2015.Zhao J J.Source analysis of fine particulate matter (PM_2.5) in Hangzhou[D].Hangzhou:Zhejiang University of Technology, 2015.
[45] 董孝华,王巨安,徐立江.慈溪大气PM₁₀及其水溶性离子污染特征研究[J].环境科学导刊, 2016,35(4):27-35.Dong X H, Wang J A, Xu L J.Characteristics of atmospheric PM₁₀ and its water-soluble ion pollution in Cixi[J].Environmental Science Guide, 2016,35(4):27-35.
[46] 赵志鹏.嘉兴市2016~2017年PM_2.5的源解析及细胞毒性初探[D].上海:上海交通大学, 2019.Zhao Z P.Source analysis and cytotoxicity of PM_2.5 in Jiaxing City, 2016~2017[D].Shanghai:Shanghai Jiaotong University, 2019.
[47] 葛琳琳,郑元铸,涂圣锋,等.温州市PM_2.5中水溶性离子污染特征及来源分析[J].浙江大学学报(理学版), 2017,44(1):112-120.Ge L L, Zheng Y Z, Tu S F, et al.Characteristics and source analysis of water-soluble ion pollution in PM_2.5 in Wenzhou[J].Journal of Zhejiang University (Science Edition), 2017,44(1):112-120.
[48] 陶志华,谢松青,何微娜,等.台州市不同功能区环境空气PM_2.5的污染特征研究[J].浙江大学学报(理学版), 2017,44(4):464-471.Tao Z H, Xie S Q, He W N, et al.Pollution characteristics of ambient air PM_2.5 in different functional areas of Taizhou City[J].Journal of Zhejiang University (Science Edition), 2017,44(4):464-471.
[49] 赵博阳,项成龙,陈焕兵,等.金华市大气PM_2.5中WSON的质量浓度及来源[J].上海大学学报(自然科学版), 2018,24(3):437-445.Zhao B Y, Xiang C L, Chen H B, et al.Mass concentration and source of WSON in atmospheric PM_2.5 in Jinhua City[J].Journal of Shanghai University (Natural Science Edition), 2018,24(3):437-445.
[50] 徐新良.中国人口、土地利用类型及分级道路空间分布数据集[EB/OL].中国科学院资源环境科学数据中心数据注册与出版系统.http://www.resdc.cn/.2020.Xu X L.Datasets on spatial distribution of Chinese, land use types and hierarchical roads[EB/OL].Data Registration and Publication System of Data Center of Resources and Environmental Sciences, Chinese Academy of Sciences.http://www.resdc.cn/.2020.
[51] 卫新,王美青,徐萍.浙江省农业功能分区与区域农业发展研究[J].中国农业资源与区划, 2009,30(3):1-5.Wei X, Wang M Q, Xu P.Research on agricultural functional zoning and regional agricultural development in Zhejiang Province[J].Agricultural Resources and Regional Planning in China, 2009,30(3):1-5.
[52] 张会宇.基于因子分析的浙江省农业发展情况研究[J].农村经济与科技, 2019,30(18):149-151.Zhang H Y.A study on agricultural development in Zhejiang Province based on factor analysis[J].Rural Economy and Science and Technology, 2019,30(18):149-151.
[53] 沈兴玲,尹沙沙,郑君瑜,等.广东省人为源氨排放清单及减排潜力研究[J].环境科学学报, 2014,34(1):43-53.Shen X L, Yin S S, Zheng J Y, et al.Inventory of anthropogenic ammonia emissions from sources and its emission reduction potential in Guangdong Province[J].Journal of Environmental Science, 2014, 34(1):43-53.
[54] 赵国梁,常景云,成杰民,等.2008~2018年山东省人为源氨排放清单研究[J].环境污染与防治, 2021,43(2):259-265.Zhao G L, Chang J Y, Cheng J M, et al.Study on anthropogenic ammonia emission inventory from anthropogenic sources in Shandong Province from 2008 to 2018[J].Environmental Pollution and Prevention, 2021,43(2):259-265.
[55] Wang C, Yin S, Ling B, et al.High-resolution ammonia emission inventories with comprehensive analysis and evaluation in Henan, China, 2006~2016[J].Atmospheric Environment, 2018,193:11-23.
[56] 王康宏,沈丽,赵睿东.2006~2017年安徽省人为源氨排放清单及特征[J].大气科学学报, 2020,43(3):547-556.Wang K H, Shen L, Zhao R D.Inventories and characteristics of anthropogenic ammonia emissions from sources in Anhui Province, 2006~2017[J].Journal of Atmospheric Sciences, 2020,43(3):547-556.
[57] 侯新红,于兴娜,沈丽,等.2013~2017年江苏省人为源氨排放清单的建立及特征[J].环境科学, 2019,40(11):4862-4869.Hou X H, Yu X N, Shen L, et al.Establishment and characteristics of anthropogenic ammonia emission inventories from anthropogenic sources in Jiangsu Province from 2013 to 2017[J].Environmental Science, 2019,40(11):4862-4869.
[58] Huang X, Song Y, Li M M, et al.A high-resolution ammonia emission inventory in China[J].Global Biogeochemical Cycles, 2012,26(1):1-14.
[59] 清华大学.中国多尺度排放清单模型MEIC(Multi-resolution Emission Inventory for China)[EB/OL].http://www.meicmodel.org/, 2022-04-24.Tsinghua University.China Multi-resolution Emission Inventory for China[EB/OL].http://www.meicmodel.org/, 2022-04-24.
[60] 翟一然.长江三角洲地区大气污染人为源排放特征研究[D].南京:南京大学, 2012.Zhai Y R.Study on anthropogenic emission characteristics of air pollution in Yangtze River Delta[D].Nanjing:Nanjing University, 2012.