土壤-水稻系统重金属空间异质性研究——以浙江省嵊州市为例

Abstract
Figure/Table
References (0)
Related Citation (15)

Download: PDF (1191 KB) HTML (1 KB)
Export: BibTeX | EndNote (RIS)

Abstract

There was a total of 94 pairs of soil and rice samples were collected from Shengzhou, Zhejiang Province. The results indicated that the mean soil concentrations of five heavy metals including Cd, Cu, Ni, Pb and Zn were 0.20, 28.64, 27.03, 38.51 and 98.74mg/kg, respectively. Compared with the National Guidelines, the heavy metals were enriched in paddy soils of the study area. Part of paddy farmland was seriously contaminated by heavy metals in Shengzhou city. However, the heavy metals in rice still remained at a safe level. The Cd, Cu, Ni, Pb, Zn concentrations in paddy soil had a moderate variability coefficients of 45.00%, 46.65%, 81.54%, 18.07%, 32.47%, respectively. Kriging interpolation and the Local Moran's I were used to identify the contaminated hotspots of these five metals. It was found out that the soil Cd, Cu, Ni, Zn had a very similar spatial pattern-higher concentrations located in the middle part of the study area while relatively lower levels in the eastern and western regions, which could be attributed to industrialization and other anthropogenic activities. The accumulation and bioavailability of heavy metals in the soil-rice system may be influenced by both soil heavy metal concentrations and soil physico-chemical properties. It may pose a potential threat to local ecosystem and human health as a long-term effect.

Key words： soil-rice system heavy metals spatial variation Moran's I geostatistics

Received: 27 May 2015

PACS:	X53
	X171.5

	Service

	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	GAO Zhi-qun
	ZHANG Mei-jian
	ZHAO Ke-li
	FU Wei-jun
	GAO Wei

Cite this article:

GAO Zhi-qun,ZHANG Mei-jian,ZHAO Ke-li等. Heavy metal contamination in soil-rice system and its spatial variation in Shengzhou City[J]. CHINA ENVIRONMENTAL SCIENCECE, 2016, 36(1): 215-224.

URL:

http://manu36.magtech.com.cn/Jweb_zghjkx/EN/ OR http://manu36.magtech.com.cn/Jweb_zghjkx/EN/Y2016/V36/I1/215

[1]	陈岭啸,宋垠先,袁旭音,等.长江三角洲典型地区土壤-水稻系统中Cd的分布及其迁移制约因素[J]. 地球科学与环境学报, 2011,33(3):288-295.
[2]	金亮,李恋卿,潘根兴,等.苏北地区土壤-水稻系统重金属分布及其食物安全风险评价[J]. 生态与农村环境学报, 2007, 23(1):33-39.
[3]	严连香,黄标,邵学新,等.不同工业企业周围土壤-作物系统重金属Pb、Cd的空间变异及其迁移规律[J]. 土壤学报, 2009, 46(1):52-62.
[4]	陈圆圆,孙小静,王军,等.上海宝山区农业用地土壤重金属空间分异规律及分布特征研究[J]. 环境化学, 2010,29(2):215-219.
[5]	程旺大,姚海根,吴伟,等.土壤-水稻体系中的重金属污染及其控制[J]. 中国农业科技导报, 2005,7(4):51-54.
[6]	Tomohito Arao, Satoru Ishikawa, Masaharu Murakami, et al. Heavy metal contamination of agricultural soil and countermeasures in Japan[J]. Paddy and Water Environment, 2010,8(3):247-257.
[7]	王爽,李荣华,张增强,等.陕西潼关农田土壤及农作物重金属污染及潜在风险[J]. 中国环境科学, 2014,34(9):2313-2320.
[8]	谢建治,张书廷,赵新华,等.潮褐土镉锌复合污染对小白菜生长的影响[J]. 天津大学学报(自然科学与工程技术版), 2005, 38(5):426-431.
[9]	鲍士旦.土壤农化分析[M]. 北京:中国农业出版社, 2007:25-99.
[10]	黄中秋,傅伟军,周国模,等.浙江省森林土壤有机碳密度空间变异特征及其影响因[J]. 土壤学报, 2014,51(4):906-913.
[11]	Zhao K L, Fu W J, Liu X M, et al. Spatial variations of concentrations of copper and its speciation in the soil-rice system in Wenling of southeastern China[J]. Environmental Science and Pollution Rresearch International, 2014,21(11):7165-7176.
[12]	Li W R, Xu B B, Song Q J, et al. The identification of ‘hotspots’ of heavy metal pollution in soil-rice systems at a regional scale in eastern China[J]. Science of The Total Environment, 2014,472:407-420.
[13]	Wang Z Q. Geostatistics and its application in ecology[M]. Beijing:Science Press, 1999:26-29.
[14]	Chen T, Liu X M, Zhu M Z, et al. Identification of trace element sources and associated risk assessment in vegetable soils of the urban-rural transitional area of Hangzhou, China[J]. Environmental Pollution, 2008,151:67-78.
[15]	Chen T, Liu X M, Zhao K L, et al. Heavy metal sources identification and sampling uncertainty analysis in a field-scale vegetable soil of Hangzhou, China[J]. Environmental Pollution, 2009,157(3):1003-1010.
[16]	Zhao K L, Liu X M, Xu J M, et al. Heavy metal contaminations in a soil-rice system:identification of spatial dependence in relation to soil properties of paddy fields[J]. Journal of Hazardous Materials, 2010,181:778-87.
[17]	林啸,刘敏,侯立军,等.上海城市土壤和地表灰尘重金属污染现状及评价[J]. 中国环境科学, 2007,27(5):613-618.
[18]	Goovaerts P. Geostatistics in soil science:state-of-the-art and perspectives[J]. Geoderma, 1999,89:1-45.
[19]	Liu X, Xu J, Zhang M, Si B, Zhao K. Spatial variability of soil available Zn and Cu in paddy rice fields of China[J]. Environmental Geology, 2008,55:1569-76.
[20]	Miao Y, Mulla D J, Robert P C. Spatial variability of soil properties, corn quality and yield in two Illinois USA fields:implications for precision corn management[J]. Precision Agriculture, 2006,7(1):5-20.
[21]	Kravchenko A N, Thelen K D, Bullock D G, et al. Relationship among Crop Grain Yield, Topography, and Soil Electrical Conductivity Studied with Cross-Correlograms[J]. Agronomy Journal, 2003,95:1132-1139.
[22]	Liu X, Wu J, Xu J. Characterizing the risk assessment of heavy metals and sampling uncertainty analysis in paddy field by geostatistics and GIS[J]. Environmental Pollution (Barking, Essex:1987), 2006,141(2):257-264.
[23]	Zhao K L, Fu W J, Ye Z Q, et al. Contamination and Spatial Variation of Heavy Metals in the Soil-Rice System in Nanxun County, Southeastern China. Internationa[J]. Journal of Environmental Research and Public Health, 2015,12(2):1577-1594.
[24]	中国环境监测总站.中国土壤元素背景值[M]. 北京:中国环境科学出版社, 1990.
[25]	Zhang X Y, Sui Y Y, Zhang X D, et al. Spatial variability of nutrient properties in black soil of theast China[J]. Pedosphere, 2007,17:19-29.
[26]	GB2762-2005 食品中污染物限量[S].
[27]	GB15618-1995 土壤环境质量标准[S].
[28]	Reddy C N, Patrick W H J. Effect of redox potential and pH on the uptake of cadmium and lead by rice plants[J]. Journal of Environmental Quality, 1977,6:259-262.
[29]	Jung M C, Thornton I. Environmental contamination and seasonal variation of metals in soils, plants and waters in the paddy fields around a Pb-Zn mine in Korea[J]. Science of the Total Environment, 1997,198:105-121.
[30]	Basta N T, Ryan J A, Chaney R L. Trace element chemistry in residual-treated soil:key concepts and metal bioavailability[J]. Journal of Environmental Quality, 2005,34(1):49-63.
[31]	Kirkham M B. Cadmium in plants on polluted soils:Effects of soil factors, hyperaccumulation, and amendments[J]. Geoderma, 2006,137:19-32.
[32]	汤丽玲.作物吸收Cd的影响因素分析及籽实Cd含量的预测[J]. 农业环境科学学报, 2007,26(2):699-703.
[33]	魏志远,郭彬,漆智平.海南省文昌市水稻土重金属污染评价[J]. 安徽农业科学, 2009,37(35):17616-17619.
[34]	Zhang C S. Using multivariate analyses and GIS to identify pollutants and their spatial patterns in urban soils in Galway, Ireland[J]. Environmental Pollution (Barking, Essex:1987), 2006, 142(3):501-511.
[35]	Cambardella C A, Moorman A T, Novak J M, et al. Field-scale variability of soil properties in central Iowa soils[J]. Soil Science Society of America Journal, 1994,58:1501-1511.
[36]	孙锐,舒帆,孙卫玲,等.典型铅锌矿区水稻土重金属污染特征及其与土壤性质的关系[J]. 北京大学学报(自然科学版), 2012,48(1):139-146.