丹江口水库表层沉积物有机/无机磷形态特征

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Abstract

Forms and occurrence characteristics of organic phosphorus and inorganic phosphorus in surface sediments of Danjiangkou Reservoir were studied by sequential extraction method, and the bio-availability and release risk of phosphorus in various forms were also discussed combining with the spatial distribution characteristics of dissolved total phosphorus (DTP) in interstitial water. Contents of phosphorus with different forms were higher in rivers than that in reservoir area. TP of sampling sites ranged from 203.08 to 1625.61mg/kg, with the mean value of 642.51mg/kg. IP was the main phosphorus form, and IP took 52.9% of TP. Average value of Ca-Pi was 642.51mg/kg, taking 57.8% of IP. Ca-P_i was the main fraction for IP. NA-P_o dominated organic phosphorus (OP) in sediments, and the mean value was 180.83mg/kg, taking 59.7% of OP. WA-P_i、PA-P_i、Fe/Al-P_i、WA-P_o、PA-P_o had significant positive correlations with DTP in pore water, but not significant positive correlation between Ca-P_i, MA-P_o, NA-Po and DTP. Both contents of bio-available phosphorus and release flux of sediments from rivers were higher than that of reservoir area, and the release risk for phosphorus was higher.

Key words： sediments sequential extraction method organic phosphorus inorganic phosphorus fraction Danjiangkou Reservoir

Received: 02 September 2015

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X524

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	Articles by authors
	WANG Wen-wen
	WANG Shu-hang
	ZHAO Li
	JIANG Xia
	ZHANG Bo
	CHEN Jun-yi

Cite this article:

WANG Wen-wen,WANG Shu-hang,ZHAO Li等. Identification of inorganic and organic species of phosphorus and its bio-availability by aequential extraction method in surface sediments of Danjiangkou Reservoir[J]. CHINA ENVIRONMENTAL SCIENCECE, 2016, 36(3): 808-818.

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http://manu36.magtech.com.cn/Jweb_zghjkx/EN/ OR http://manu36.magtech.com.cn/Jweb_zghjkx/EN/Y2016/V36/I3/808

[1]	袁和忠,沈吉,刘恩峰.太湖不同湖区沉积物磷形态变化分析[J]. 中国环境科学, 2010,30(11):1522-1528.
[2]	吴世凯,谢平,倪乐意,等.长江中下游地区湖泊中蓝藻及其与氮磷浓度的关系[J]. 水生态学杂志, 2014,35(3):19-25.
[3]	Pei Guofeng, Wang Qing, Liu Guoxiang. The role of periphyton in phosphorus retention in shallow lakes with different trophic status, China[J]. Aquatic Botany, 2015,125:17-22.
[4]	Baker D B, Confesor R, Ewing D E, et al. Phosphorus loading to Lake Erie from the Maumee, Sandusky and Cuyahoga rivers: The importance of bioavailability[J]. Journal of Great Lakes Research, 2014,40(3):502-517.
[5]	黎睿,王圣瑞,肖尚斌,等.长江中下游与云南高原湖泊沉积物磷形态及内源磷负荷[J]. 中国环境科学, 2015,35(6):1831-1839.
[6]	吴强亮,谢从新,赵峰,等.沉水植物苦草(Vallisneria natans)对沉积物中磷赋存形态的影响[J]. 湖泊科学, 2014,26(2):228-234.
[7]	张洪梅,刘鑫,邓建才,等.太湖沉积物再悬浮对水体中磷形态和浓度时空差异性影响[J]. 农业环境科学学报, 2013,32(11): 2251-2257.
[8]	Ni Zhaokui, Wang Shengrui. Historical accumulation and environmental risk of nitrogen and phosphorus in sediments of Erhai Lake, Southwest China[J]. Ecological Engineering, 2015, 79:42-53.
[9]	Tang Xianqiang, Wu Min, DAI Xichang, et al. Phosphorus storage dynamics and adsorption characteristics for sediment from a drinking water source reservoir and its relation with sediment compositions[J]. Ecological Engineering, 2014,64:276-284.
[10]	Wang Changhui, Liu Juanfeng, Pei Yuansheng. Effect of hydrogen sulfide on phosphorus lability in lake sediments amended with drinking water treatment residuals[J]. Chemosphere, 2013,91,(9):1344-1348.
[11]	Huang Lei, Fang Hongwei, Fazeli M, et al. Mobility of phosphorus induced by sediment resuspension in the Three Gorges Reservoir by flume experiment[J]. Chemosphere, 2015, 134:374-379.
[12]	Chen Shiyue, Chen Yingying, Liu Jiazhen, et al. Vertical variation of phosphorus forms in core sediments from Dongping Lake, China[J]. Procedia Environmental Sciences, 2011,10,Part B: 1797-1801.S
[13]	Jing Liandong, Liu Xingli, Bai Song, et al. Effects of sediment dredging on internal phosphorus: A comparative field study focused on iron and phosphorus forms in sediments[J]. Ecological Engineering, 2015,82:267-271.
[14]	Ivanoff D B, Reddy K R, Robinson S. Chemical fractionation of organic phosphorus in selected histosols[J]. Soil Science, 1998,163(1):36-45.
[15]	Bowman R A, Colf V. An exploratory method for fractionation of organic phosphorus from grassland soils[J]. Soil Science, 1978,125(2):95-101.
[16]	Golterman H L. Diferential extraetion of sediment phosphates with N T A solution[J]. Hydrobiology, 1982,91-92(1):683-687.
[17]	Ruban V, Brigault S, Demare E D, et al. An investigation of the origin and mobility of phosphorus in freshwater sediments from Bort-Les-Orgues Reservoir, France[J]. Journal of Environmental Monitoring, 1999,1(4):403-407.
[18]	Williams J D H, Shear H, Thomas R L. Availability to Scenedesmus,quadrcauda of different forms of phosphorus in sedimentary materials from the Great Lakes[J]. Limnology Oceanography, 1980,25:1-11.
[19]	Hiehjes A H, Lijklema L. Fractionation of inorganic phosphorus in calcareors sediments[J]. Journal of Environmental Quality, 1980,8:130-132.
[20]	Ruttenberg K C. Development of a sequential extraction method for different forms of phosphorus in marine sediments[J]. Limnology Oceanography, 1992,37:1460-1482.
[21]	Hedley M J, Stewart J W B, Chauhan B S. Changes in inorganic and organic soil phosphorus fractions induced by cultivation practices and by laboratory incubations[J]. Soil Science Society of America Journal, 1982,46(5):970-976.
[22]	李坤,李兆华,陈红兵,等.丹江口水库上游武当山剑河水质空间差异性分析[J]. 湖泊科学, 2013,25(5):649-654.
[23]	成庆利,张杰.丹江口水库水质现状分析与评价[J]. 环境与可持续发展, 2007,(1):12-14.
[24]	王书航,张博,姜霞,等.采用连续分级提取法研究沉积物中磷的化学形态[J]. 环境科学研究, 2015,28(9):47-53.
[25]	姜霞,王书航.沉积物质量评估手册[M]. 北京:科学出版社, 2012.
[26]	Wen Shengfang, Shan Baoqing, Zhang Hong. Metals in sediment/pore water in Chaohu Lake: Distribution, trends and flux[J]. Journal of Environmental Sciences, 2012,24(12):2041-2050.
[27]	Carling G T, Richards D C, Hoven H, et al. Relationships of surface water, pore water, and sediment chemistry in wetlands adjacent to Great Salt Lake, Utah, and potential impacts on plant community health[J]. Science of The Total Environment, 2013, 443(15):798-811.
[28]	Zhu Hongwei, Cheng Pengda, Wang Daozeng. Relative roles of resuspended particles and pore water in release of contaminants from sediment[J]. Water Science and Engineering, 2014,7(3): 344-350.
[29]	Cheng Dengmiao, Liu Xinhui, Wang Liang, et al. Seasonal variation and sediment-water exchange of antibiotics in a shallower large lake in North China[J]. Science of The Total Environment, 2014,476-477,266-275.
[30]	Xiang Sulin, Zhou Wenbin. Phosphorus forms and distribution in the sediments of Poyang Lake, China[J]. International Journal of Sediment Research, 2011,26(2):230-238.
[31]	宋媛媛,冯慕华,苏争光,等.抚仙湖不同来源沉积物磷形态垂向分布特征[J]. 环境科学学报, 2013,33(9):2579-2589.
[32]	陈春瑜,徐晓梅,邓伟明,等.滇池表层沉积物对磷的吸附特征[J]. 环境科学学报, 2014,34(12):3065-3075.
[33]	Mudroch A, Azcue D J M. Manual of aquatic sediment sampling[M]. Boca Raton: Lewis Publications, 1995.
[34]	He Z, Griffin T S, Honeycutt C W. Evaluation of soil phosphorus transformations by sequential fractionation and phosphatase hydrolysis[J]. Soil Science, 2004,169(7):515-527.
[35]	Zaaboub N, Ounis A, Helali M A, et al. Phosphorus speciation in sediments and assessment of nutrient exchange at the water-sediment interface in a Mediterranean lagoon: Implications for management and restoration[J]. Ecological Engineering, 2014,73(12):115-125.
[36]	Fabre A, Qotbi A, Dauta A, et al. Relation between algal available phosphate in the sediments of the River Garonne and chemically-determined phosphate fractions[J].Hydrobiologia, 1996,335(1): 43-48.
[37]	王忠威,王圣瑞,戴建军,等.洱海沉积物中磷的赋存形态[J]. 环境科学研究, 2012,25(6):652-658.
[38]	史静,俎晓静,张乃明,等.滇池草海沉积物磷形态空间分布特征及影响因素[J]. 中国环境科学, 2013,33(10):1808-1813.
[39]	Zhu Mengyuan, Zhu Guangwei, Li Wei, et al. Estimation of the algal-available phosphorus pool in sediments of a large, shallow eutrophic lake (Taihu, China) using profiled SMT fractional analysis[J]. Environmental Pollution, 2013,173:216-223.
[40]	Zhang Runyu, We Fengchang, Liu Congqiang, et al. Characteristics of organic phosphorus fractions in different trophic sediments of lakes from the middle and lower reaches of Yangtze River region and Southwestern Plateau, China[J]. Environmental Pollution, 2008,152:366-372.
[41]	范业宽,李世俊. Bowman-Cole石灰性土壤有机磷分组法的改进[J]. 土壤通报, 2004,35(6):743-749.
[42]	Liu Jinyong, Wang Hui, Yang Haijun, et al. Detection of phosphorus species in sediments of artificial landscape lakes in China by fractionation and phosphorus-31nuclear magnetic resonance spectroscopy[J]. Environmental Pollution, 2009,157: 49-56.
[43]	长江水利委员会长江勘测规划设计研究院.南水北调中线一期工程丹江口水利枢纽大坝加高工程初步设计阶段水库建设征地移民规划设计报告[R]. 武汉, 2005.
[44]	王剑,尹炜,赵晓琳,等.丹江口水库新增淹没区农田土壤潜在风险评估[J]. 中国环境科学, 2015,35(1):157-164.