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Effect of initial pH on anaerobic digestionof waste activated sludge under direct electrical stimulation |
CHEN Ying, YIN Chang-kai, ZHU Nan-wen, YUAN Hai-ping, LOU Zi-yang |
School of Environmental Science and Engineering, Shanghai Jiaotong University, Shanghai 200240, China |
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Abstract Batch tests were operated to investigate effects of initial pH (3,5,7,9,11) on anaerobic digestion of waste activated sludge under 0.6V direct electrical stimulation. Initial pH had a great influence on biogas production and VS removal efficiency. At the optimal initial pH of 9, maximum methane yield of 224mLCH4/g VS and VS removal efficiency of 38.1% were achieved after 32days digestion. Initial pH could accelerate hydrolysis and acidification process of waste activated sludge. Alkaline environment (pH 9, 11) enhanced SCOD and VFAs concentrations in suspensions, especially at pH 11. Acetic acid and butyric acid were dominant at pH 3and 11while acetic acid and propionic acid were main products at pH 5, 7 and 9. Initial pH facilitates release of ammonium from waste activated sludge and in acidic environment ammonium was released in excess.
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Received: 19 June 2015
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[1] |
Seggiani M, Vitolo S, Puccini M, et al. Cogasification of sewage sludge in an updraft gasifier[J]. Journal of Fuel, 2012,93: 486-491.
|
[2] |
Khalid Azeem, Arshad Muhammad, Anjum Muzammil, et al. The anaerobic digestion of solid organic waste[J]. Journal of Waste Management, 2011,31:1737-1744.
|
[3] |
刘 阳,彭永臻,韩玉伟,等.游离氨对热水解联合中温厌氧消化处理剩余污泥的影响[J]. 中国环境科学, 2015,35(9):2650-2657.
|
[4] |
Go¢mez X, Cuetos MJ, Cara J, et al. Anaerobic co-digestion of primary sludge and the fruit and vegetable fraction of the municipal solid wastes[J]. Journal of Renewable Energy, 2006, 31:2017-2024.
|
[5] |
Feng Yinghong, Zhang Yaobin, Chen Shuo, et al. Enhanced production of methane from waste activated sludge by the combination of high-solid anaerobic digestion and microbial electrolysis cell with iron-graphite electrode[J]. Journal of Chemical Engineering, 2015,259:787-794.
|
[6] |
Kotoyoshi Nakanishi, Hiroharu Tokuda, Takahiko Soga, et al. Effect of Electric Current on Growth and Alcohol Production by Yeast Cells[J]. Journal of Fermentation and bioenoineer, 1998,85(2):250-253.
|
[7] |
She Peng, Song Bo, Xing Xin-Hui, et al. Electrolytic stimulation of bacteriaEnterobacter dissolvens by a direct current[J]. Journal of Biochemical Engineering, 2011,31:1737-1744.
|
[8] |
佟 倜,张 羽,刘晓冬,等.静电场和芒刺静电场对野生型大肠杆菌生长的实验研究[J]. 中国医学物理学杂志, 2005,22(4): 580-582.
|
[9] |
Beschkov V, Velizarov S, Agathos S N, et al. Bacterial denitrification of waste water stimulated by constant electric field[J]. Journal of Biochemical Engineering, 2004,17(2):141-145.
|
[10] |
Y G Chen, S Jiang, H Y Yuan, et al. Hydrolysis and acidification of waste activated sludge at different pHs[J]. Journal of Water Research, 2007,41(3):683-689.
|
[11] |
国家环境保护总局《水和废水监测分析方法》编委会.水和废水监测分析方法[M]. 4版.北京:中国环境科学出版社, 2002.
|
[12] |
Cai M L, Wei Y S, Liu J X. Enhanced biohydrogen production from sewage sludge with alkaline pretreatment[J]. Journal of Environment Science and Technology, 2004,38:3195-3202.
|
[13] |
肖本益,刘俊新.污水处理系统剩余污泥碱处理融胞效果研究[J]. 环境科学, 2006,27(2):319-323.
|
[14] |
刘常青,赵由才,张江山,等.酸性预处理污泥厌氧发酵产氢[J]. 环境科学, 2008,28(10):2008-2011.
|
[15] |
FU W G, Mathews A P. Lactic acid production from lactose by Lactobacillus plantarum: kinetic model and effects of pH, substrate, andoxygen[J]. Journal of Biochemical Engineering, 1999,3(3):163-170.
|
[16] |
高树梅,赵明星,许之扬,等.餐厨垃圾固渣厌氧发酵产甲烷潜力及Logistic动力学研究[J]. 安全与环境学报, 2015,15(1): 263-267.
|
[17] |
Chen Yinguang, Jiang Su, Yuan Hongying, et al. Hydrolysis and acidification of waste activated sludge at different pHs[J]. Journal of Water Research, 2007,41:683-689.
|
[18] |
郭燕锋,孔晓英,刘婉玉,等.有机负荷对厨余垃圾常温厌氧发酵产甲烷的影响[J]. 农业工程学报, 2011,27:96-100.
|
[19] |
Rajinikanth Rajagopal, Daniel I Massé, A critical review on inhibition of anaerobic digestion process by excess ammonia[J]. Bioresource Technology[J]. 2013,143:632-641.
|
[20] |
Orhan Yenigün, Burak Demirel. Ammonia inhibition in anaerobic digestion: A review[J]. Journal of Process Biochemistry, 2013,48:901-911.
|
[21] |
刘 阳,彭永臻,韩玉伟,等.游离氨对热水解联合中温厌氧消化处理剩余污泥的影响[J]. 中国环境科学, 2015,35(9):2650-2657.
|
|
|
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