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Primary particulate matter (PM) emission inventory from agricultural activities in northeastern China |
LI Rui-min1,2, TONG Quan-song1, CHEN Wei-wei1, WANG Yi-yong1, ZHANG Shi-chun1, ZHANG Xue-lei1, ZHAO Hong-mei1, HE Yue-xin1,2 |
1. Key Labortory of Wetland Ecology and Environment, Northeast Institute of Geography and Agroecology, Changchun 130102, China;
2. University of Chinese Academy of Sciences, Beijing 100049, China |
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Abstract Agricultural PM10 and PM2.5 inventories on the county-level scale in northeastern China were developed in this study. Based on bottom-Up method, we firstly collect the agricultural activity data, including conventional farming operations (i.e., straw burning, land preparation, harvest, grain processing, fertilizer, agricultural machinery, and wind erosion), emission factors of these operations and crop area at each county. And then, county-level PM10and PM2.5 emission inventories from agricultural operations in 2010 were developed and spatio-temporal distributions were analyzed. The results showed that the magnitude of agricultural PM10 and PM2.5 emissions in northeastern China were 54.6×104 tons and 35.6×104 tons, respectively. The PM10 and PM2.5 emissions from straw burning were highest, which accounted for 60% and 87% of the total emissions, respectively. In addition, land preparing occupied 27% and 6% for PM10 and PM2.5, respectively. The spatial distribution of agricultural PM emissions, concentrated on three plains, i.e., the Sanjiang Plain (in the northeast of Heilongjiang), the Songnen Plain (in the middle of Heilongjiang and Jilin Provinces), the Liaohe Plain (in the middle of Liaoning Provinces). Based on temporal variations, agricultural PM10 emissions mainly occurred in May, September and October, which contributed 88% of total emissions. The PM2.5 was mainly released in September and October. The uncertainty of emission inventory was 184.3%. More information on local emission factors will be helpful to decrease the emission inventory uncertainty.
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Received: 10 November 2015
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[1] |
Baker J B, Southard R J, Mitchell J P. Agricultural dust production in standard and conservation tillage systems in the San Joaquin Valley [J]. Journal of Environmental Quality, 2005, 34(4):1260-1269.
|
[2] |
Hinz T, van der Hoek K. Particulate matter emissions from arable production-a guide for UNECE emission inventories [Z]. T. Hinz T. und K. Tamoschat-Depolt (Hrsg.): Particulate Matter in and from Agriculture. Landbauforschung Völkenrode, Sonderheft, 2007,308.
|
[3] |
Holmén B, Miller D, Hiscox A, et al. Near-source particulate emissions and plume dynamics from agricultural field operations [J]. Journal of Atmospheric Chemistry, 2008,59(2):117-134.
|
[4] |
Aneja V P, Schlesinger W H, Erisman J W. Effects of agriculture upon the air quality and climate: Research, policy, and regulations [J]. Environmental Science & Technology, 2009,43(12):4234-4240.
|
[5] |
Pattey E, Qiu G, Fiset S, et al. Primary particulate matter emissions and trends from Canadian agriculture [J]. Air Pollution XXIII, 2015,198:143.
|
[6] |
陈卫卫.农业土壤耕作大气颗粒物排放研究进展 [J]. 农业环境科学学报, 2015,34(7):1225-1232.
|
[7] |
赵 鹏,朱 彤,梁宝生,等.北京郊区农田夏季大气颗粒物质量和离子成分谱分布特征 [J]. 环境科学, 2006,27(2):193-199.
|
[8] |
EEA, Crop production and agricultural soils, in EMEP/EEA Emission Inventory Guidebook, 2009[EB/OL].2014-12-10.
|
[9] |
高卫东,魏文寿,刘明哲.塔里木盆地区域沙尘气溶胶特征分析 [J]. 干旱区地理, 2002,25(2):165-169.
|
[10] |
Cao J J, Chow J C, Watson J G, et al. Size-differentiated source profiles for fugitive dust in the Chinese Loess Plateau [J]. Atmospheric Environment, 2008,42(10):2261-2275.
|
[11] |
Xin H S, Schaefer D M, Liu Q P, et al. Effects of polyurethane coated urea supplement on in vitro ruminal fermentation, ammonia release dynamics and lactating performance of Holstein dairy cows fed a steam-flaked corn-based diet [J]. Asian-Aust. J. Anim. Sci., 2010,23:491-500.
|
[12] |
康富贵,李耀辉.近10a西北地区沙尘气溶胶研究综述 [J]. 干旱气象, 2011,29(2):144-150.
|
[13] |
Bogman P, Cornelis W, Rollé H, et al. Prediction of TSP and PM10 emissions from agricultural operations in Flanders, Belgium [C]//Proceedings of the 14th International Conference “Transport and Air Pollution”, Graz, Austria, June, 2005:1-3.
|
[14] |
臧 英,高焕文,周建忠.保护性耕作对农田土壤风蚀影响的试验研究 [J]. 农业工程学报, 2003,19(2):56-60.
|
[15] |
张楚莹,王书肖,赵 瑜,等.中国人为源颗粒物排放现状与趋势分析 [J]. 环境科学, 2009,30(7):1881-1887.
|
[16] |
李向阳,丁晓妹,高 宏,等.中国北方典型城市API特征分析 [J]. 干旱区资源与环境, 2011,25(3):96-101.
|
[17] |
叶 瑜,方修琦,任玉玉,等.东北地区过去300年耕地覆盖变化 [J]. 中国科学:D辑, 2009,39(3):340-350.
|
[18] |
马建堂.中国统计年鉴2012 [M]. 2012.
|
[19] |
廉 毅,高枞亭,任红玲.20世纪90年代中国东北地区荒漠化的发展与区域气候变化 [J]. 气象学报, 2001,59(6):730-736.
|
[20] |
CARB. Assessing Area Source Emissions [EB/OL]. [2014-12-21]. http://www. wrapair.org/forums/dejf/. . ./Ch10-Harvesting_ Rev06. Doc.
|
[21] |
Liousse C, Penner J E, Chuang C, et al. A global three‐dimensional model study of carbonaceous aerosols[J]. Journal of Geophysical Research: Atmospheres, 1996,101(D14):19411-19432.
|
[22] |
祝 斌,朱先磊,张元勋,等.农作物秸秆燃烧PM2.5排放因子的研究 [J]. 环境科学研究, 2005,18(2):29-33.
|
[23] |
王书肖,张楚莹.中国秸秆露天焚烧大气污染物排放时空分布 [J]. 中国科技论文在线, 2008,3(5):329-333.
|
[24] |
Metro Vancouver. 2005 Lower Fraser Valley air emissions. Inventory & Forecast and BackCast. Detailed listing of results and methodology [Z]. 2010.
|
[25] |
Pattey E, Qiu G. Trends in primary particulate matter emissions from Canadian agriculture [J]. Journal of the Air & Waste Management Association, 2012,62(7):737-747.
|
[26] |
扬尘源排放清单编制技术指南试行 [Z]. 2014.
|
[27] |
Hinz T, Tamoschat-Depolt K. Particulate Matter in and from Agriculture [M]. Germany: Landbauforschung Völkenrode, 2002: 1-7.
|
[28] |
曹国良,张小曳,龚山陵,等.中国区域主要颗粒物及污染气体的排放源清单 [J]. 科学通报, 2011,56(3):261-268.
|
[29] |
黑龙江统计局.黑龙江统计年鉴-2010 [M]. 北京:中国统计出版社, 2010.
|
[30] |
吉林统计局.吉林统计年鉴-2010 [M]. 北京:中国统计出版社, 2010
|
[31] |
辽宁统计局.辽宁统计年鉴-2010 [M]. 北京:中国统计出版社, 2010.
|
[32] |
内蒙古统计局.内蒙古统计年鉴-2010 [M]. 北京:中国统计出版社, 2010.
|
[33] |
毕于运,高春雨,王亚静,等.中国秸秆资源数量估算 [J]. 农业工程学报, 2009,(12):211-217.
|
[34] |
农业技术经济手册(修订本) [Z]. 1986.
|
[35] |
中国农业统计年鉴2012 [M]. 北京:中国农业出版社, 2012.
|
[36] |
中华人民共和国农业部种植管理司.http://www.zzys.moa. gov.cn/[EB/Z].
|
[37] |
U. S. Environmental Protection Agency. Compilation of Air Pollutant Emission Factors AP-42, Fifth Edition [EB/OL]. http://www. epa. gov/ttnchie1/ap42/2014-12-21.
|
[38] |
Jenkin, B. Atmospheric pollutant emission factors from open burning of agricultural and forest biomass by wind tunnel simulations, Tables 4.1.1to 4.1.8 [Z]. Davis:university of California, Davis, 1996.
|
[39] |
张 强.中国区域细颗粒物排放及模拟研究 [D]. 北京:清华大学, 2005.
|
[40] |
李瑞敏,张世春,王毅勇,等.三江平原作物收获期大气颗粒物浓度特征 [J]. 中国环境科学, 2015,35(3):676-682.
|
[41] |
王 卫,李秀彬.中国耕地有机质含量变化对土地生产力影响的定量研究 [J]. 地理科学, 2002,22(1):24-28.
|
[42] |
陆 炳,孔少飞,韩 斌,等.2007年中国大陆地区生物质燃烧排放污染物清单 [J]. 中国环境科学, 2011,31(2):186-194.
|
|
|
|