南京市机动车排放VOCs的污染特征与健康风险评价

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Abstract In order to study volatile organic compounds (VOCs) from vehicle emissions impact on the environment and people health, a tunnel test was conducted the Fu Gui Mountain tunnel in Nanjing, China. The ambient level and composition characteristics, temporal variation characteristics, and chemical reactivity of VOCs were studied. The health risk of VOCs in the tunnel in the study area was assessed by using the international recognized health risk assessment method (US EPA). A total of 97VOC species were quantified in the samples collected at the entrance and exit of tunnel. The total concentrations of VOCs at the entrance and the exit were (87.28±7.08)μg/m³ and (225.63±59.19)μg/m³, respectively. The alkanes and aromatics concentration were the most abundant VOCs in the exit. The ozone formation potentials at the entrance and exit of tunnel were 101.48μg O₃/m³ and 402.01μg O₃/m³. Health Risk assessment showed that the hazard quotient (HQ) of 14major VOCs were between 8.07×10^-5 ~ 2.66×10^-1 in the entrance, but the HQ in the exit was in the range of 3.18×10^-4 ~ 2.92×10^-1. The non-carcinogenic hazard risk index (HI) at the tunnel entrance and exit were both less than 1, which were non-carcinogenic to human body. However, 5VOCs are carcinogenic to human body, such as 1,3-butadiene, chloroform, carbon tetrachloride, benzene and 1,1,2-trichloroethane which have a significant impact on human health.

Key words： tunnel test vehicle emissions volatile organic compounds (VOCs) health risks ozone formation potentials

Received: 06 March 2016

PACS:	X511
	X503.1

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	Articles by authors
	ZHANG Qi-jun
	WU Lin
	LIU Ming-yue
	FANG Xiao-zhen
	ZHANG Jing
	MAO Hong-jun
	SHAO Min
	LU Si-hua

Cite this article:

ZHANG Qi-jun,WU Lin,LIU Ming-yue等. Pollution characteristics and health risk assessment of VOCs from vehicle exhaust in Nanjing, China[J]. CHINA ENVIRONMENTAL SCIENCECE, 2016, 36(10): 3118-3125.

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http://manu36.magtech.com.cn/Jweb_zghjkx/EN/ OR http://manu36.magtech.com.cn/Jweb_zghjkx/EN/Y2016/V36/I10/3118

[1]	莫梓伟,陆思华,李悦,等.北京市典型溶剂使用企业VOCs排放成分特征 [J]. 中国环境科学, 2015,35(2):374-380.
[2]	韩博,吴建会,王凤炜,等.天津滨海新区工业源VOCs及恶臭物质排放特征 [J]. 中国环境科学, 2011,31(11):1776-1781.
[3]	Brown S G, Frankel A, Hafner H R. Source apportionment of VOCs in the Los Angeles area using positive matrix factorization [J]. Atmospheric Environment, 2007,41(2):227-237.
[4]	Shin H, Roh S, Kim J, et al. Temporal variation of volatile organic compounds and their major emission sources in Seoul, Korea [J]. Environmental Science and Pollution Research, 2013, 20(12):8717-8728.
[5]	Ling Z, Guo H, Cheng H, et al. Sources of ambient volatile organic compounds and their contributions to photochemical ozone formation at a site in the Pearl River Delta, southern China [J]. Environmental Pollution, 2011,159(10):2310-2319.
[6]	Waston J G, Chow J C, Fujita E M. Review of volatile organic compound source apportionment by chemical mass balance [J]. Atmospheric Environment, 2001,35(9):1567-1584.
[7]	于艳,王秀艳,杨文.天津市机动车二次有机气溶胶生成潜势的估算 [J]. 中国环境科学, 2015,35(2):381-386.
[8]	王玮,梁宝生,曾凡刚,等.谭裕沟隧道VOCs污染特征和排放因子研究 [J]. 环境科学研究, 2001,14(4):9-12.
[9]	Araizaga A, Mancilla Y, Mendoza A. Volatile organic compound emissions from light-duty vehicles in Monterrey, Mexico: a tunnel study [J]. International Journal of Environmental Research, 2013,7(2):277-292.
[10]	Lai C-H, Peng Y-P. Volatile hydrocarbon emissions from vehicles and vertical ventilations in the Hsuehshan traffic tunnel, Taiwan [J]. Environmental Monitoring and Assessment, 2012, 184(7):4015-4028.
[11]	Staehelin J, Schlpfer K, Brgin T, et al. Emission factors from road traffic from a tunnel study (Gubrist tunnel, Switzerland). Part I: concept and first results [J]. Science of the Total Environment, 1995,169(1):141-147.
[12]	Chiang H-L, Hwu C-S, Chen S-Y, et al. Emission factors and characteristics of criteria pollutants and volatile organic compounds (VOCs) in a freeway tunnel study [J]. Science of the Total Environment, 2007,381(1):200-211.
[13]	Ho K, Lee S, Ho W, et al. Vehicular emission of volatile organic compounds (VOCs) from a tunnel study in Hong Kong [J]. Atmospheric Chemistry and Physics, 2009,9(19):7491-7504.
[14]	王伯光,邵敏,张远航,等.机动车排放中挥发性有机污染物的组成及其特征研究 [J]. 环境科学研究, 2007,19(6):75-80.
[15]	林旭,朱彬,安俊琳,等.南京北郊VOCs对臭氧和二次有机气溶胶潜在贡献的研究 [J]. 中国环境科学, 2015,35(4):976- 986.
[16]	US EPA. Risk assessment guidance for superfund Volume I: Human health evaluation manual (Part F, Supplemental guidance for inhalation risk assessment) [R]. Washington D C: Office of Superfund Remedia-tion and Technology Innovation Environmental Protection Agency, 2009.
[17]	徐慧,邓君俊,邢振雨,等.厦门不同功能区VOCs的污染特征及健康风险评价 [J]. 环境科学学报, 2015,35(9):2701-2709.
[18]	南淑清,张霖琳,张丹,等.郑州市环境空气中VOCs的污染特征及健康风险评价 [J]. 生态环境学报, 2014,9:005.
[19]	Dutta C, Som D, Chatterjee A, et al. Mixing ratios of carbonyls and BTEX in ambient air of Kolkata, India and their associated health risk [J]. Environmental Monitoring and Assessment, 2009,148(1-4):97-107.
[20]	方晶晶,章骅,吕凡,等.生活垃圾收运过程中恶臭暴露的健康风险评估 [J]. 中国环境科学, 2015,35(3):906-916.
[21]	李雷,李红,王学中,等.广州市中心城区环境空气中挥发性有机物的污染特征与健康风险评价 [J]. 环境科学, 2013, 34(12):4558-4564.
[22]	夏芬美,李红,李金娟,等.北京市东北城区夏季环境空气中苯系物的污染特征与健康风险评价 [J]. 生态毒理学报, 2014, 9(6):1041-1052.