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| The sorption properties of tylosin by black carbon-humic acid complex |
| DONG Hao1, GUO Xue-tao1, WU Hui-jun1, YANG Chen2, PENG Dan3, GAO Liang-min1, HU You-biao1 |
1. School of Earth and Environment, Anhui University of Science and Technology, Huainan 232001, China;
2. College of Environment and Energy, South China University of Technology, Guangzhou 510006, China;
3. School of Traffic and Environment, Shenzhen Institute of Information Technology, Shenzhen 518172, China |
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Abstract Based on tylosin was wsed as one representative organic pollutant, the sorption characteristics and mechanism of tylosin on different sources of nano black carbon-humic acid complexes was invesitigated. Results showed that the sorption capacity of black carbon and humic acid complex was higher than that of black carbon and humic acid; the sorption equilibrium could be obttained within 24hours; the sorption kinetics of tylosin on both black carbon and black carbon-humic acid complex fitted the pseudo-second-order kinetics model; the sorption isotherms could fit well with the Henry model and Freundlich model; the sorption capacity of tylosin on black carbon and humic acid complex would be altered in different solution chemistries (i.e., pH and ionic strength of solutions). Ion-exchange, hydrogen-bond, and hydrophobic play a main role in the sorption of tylosin on black carbon and humic acid complex.
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Received: 05 May 2016
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孙瑞珠,马玉龙,张娟,等.泰乐菌素降解菌的筛选及其降解动力学研究[J]. 中国环境科学, 2013,33(4):722-727.
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Ji L L, Zhu D Q, Wan Y Q, et al. Adsorption of tetracycline and sulfamethoxazole on crop residue-derived ashes:Implication for the relative importance of black carbon to soil sorption[J]. Environmental Science & Technology, 2011,45(13):5580-5586.
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Lou L P, Luo L, Hu B L, et al. The sorption of pentachlorophenol by aged sediment supplemented with black carbon produced from rice straw and fly ash[J]. Bioresource Technology, 2012,112:61-66.
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Jia M, Wang F, Bian Y R, et al. Effects of pH and metal ions on oxytetracycline sorption to maize-straw-derived biochar[J]. Bioresource Technology, 2013,136:87-93.
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Guo X T, Yang C, Dang Z, et al. The influences of pH and ionic strength on the sorption of tylosin on goethite[J]. Environmental Science and Pollution Research, 2014,21(4):2572-2580.
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Zheng H, Wang Z Y, Zhao J, et al. Sorption of antibiotic sulfamethoxazole varies with biochars produced at different temperatures[J]. Environmental Pollution, 2013,181:60-67.
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Guo X T, Yang C, Zhang J, et al. Sorption and photodegradation of tylosin and sulfamethazine by humic acid-coated goethite[J]. RSC Advances, 2015,5(122):100464-100471.
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林建伟,詹艳慧,陆霞.锆改性沸石对水中磷酸盐和铵的吸附特性[J]. 中国环境科学, 2012,32(11):2023-2031.
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Ruan Z H, Wu J H, Xie J, et al. Facile preparation of rosin-based biochar coated bentonite for supporting α-Fe2O3 nanoparticles and its application for Cr(vi) adsorption[J]. Journal of Materials Chemistry A, 2015,3(8):4595-4603.
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Luo L, Lou L P, Cui X Y, et al. Sorption and desorption of pentachlorophenol to black carbon of three different origins[J]. Journal of Hazardous Materials, 2011,185(2/3):639-646.
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Lin K, Ding J, Wang H, et al. Goethite-mediated transformation of bisphenol A[J]. Chemosphere, 2012,89(7):789-795.
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| [16] |
张晶,郭学涛,葛建华,等.针铁矿-腐殖酸的复合物对泰乐菌素的吸附[J]. 环境工程学报, 2016,10(3):1145-1151.
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Lian F, Sun B B, Chen X, et al. Effect of humic acid (HA) on sulfonamide sorption by biochars[J]. Environmental Pollution, 2015,204:306-312.
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Zhang Q, Zhao L, Dong Y H, et al. Sorption of norfloxacin onto humic acid extracted from weathered coal[J]. Journal of Environmental Management, 2012,102:165-172.
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Guo X T, Dong H, Yang C, et al. Application of goethite modified biochar for tylosin removal from aqueous solution[J]. Colloids and Surfaces A:Physicochemical and Engineering Aspects, 2016,502:81-88.
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Zhang J, He M C, Lin C Y, et al. Phenanthrene sorption to humic acids, humin, and black carbon in sediments from typical water systems in China[J]. Environmental Monitoring and Assessment, 2010,166(1-4):445-459.
|
| [1] |
Guo X T, Ge J H, Yang C, et al. Sorption behavior of tylosin and sulfamethazine on humic acid:kinetic and thermodynamic studies[J]. RSC Advances, 2015,5(72):58865-58872.
|
| [2] |
孙瑞珠,马玉龙,张娟,等.泰乐菌素降解菌的筛选及其降解动力学研究[J]. 中国环境科学, 2013,33(4):722-727.
|
| [3] |
郭学涛,杨琛,党志,等.环境因素对针铁矿光解泰乐菌素的影响[J]. 中国环境科学, 2014,34(2):364-370.
|
| [4] |
Rakshit S, Sarkaret D, Punamiya P, et al. Kinetics of oxytetracycline sorption on magnetite nanoparticles[J]. International Journal of Environmental Science and Technology, 2014,11(5):1207-1214.
|
| [5] |
Marc T, Joseph J P, Carles H, et al. Predicting contaminant adsorption in black carbon (biochar)-amended soil for the veterinary antimicrobial sulfamethazine[J]. Environmental Science & Technology, 2013,47(12):6197-6205.
|
| [6] |
Ji L L, Zhu D Q, Wan Y Q, et al. Adsorption of tetracycline and sulfamethoxazole on crop residue-derived ashes:Implication for the relative importance of black carbon to soil sorption[J]. Environmental Science & Technology, 2011,45(13):5580-5586.
|
| [7] |
Lou L P, Luo L, Hu B L, et al. The sorption of pentachlorophenol by aged sediment supplemented with black carbon produced from rice straw and fly ash[J]. Bioresource Technology, 2012,112:61-66.
|
| [8] |
Jia M, Wang F, Bian Y R, et al. Effects of pH and metal ions on oxytetracycline sorption to maize-straw-derived biochar[J]. Bioresource Technology, 2013,136:87-93.
|
| [9] |
Guo X T, Yang C, Dang Z, et al. The influences of pH and ionic strength on the sorption of tylosin on goethite[J]. Environmental Science and Pollution Research, 2014,21(4):2572-2580.
|
| [10] |
Zheng H, Wang Z Y, Zhao J, et al. Sorption of antibiotic sulfamethoxazole varies with biochars produced at different temperatures[J]. Environmental Pollution, 2013,181:60-67.
|
| [11] |
Guo X T, Yang C, Zhang J, et al. Sorption and photodegradation of tylosin and sulfamethazine by humic acid-coated goethite[J]. RSC Advances, 2015,5(122):100464-100471.
|
| [12] |
林建伟,詹艳慧,陆霞.锆改性沸石对水中磷酸盐和铵的吸附特性[J]. 中国环境科学, 2012,32(11):2023-2031.
|
| [13] |
Ruan Z H, Wu J H, Xie J, et al. Facile preparation of rosin-based biochar coated bentonite for supporting α-Fe2O3 nanoparticles and its application for Cr(vi) adsorption[J]. Journal of Materials Chemistry A, 2015,3(8):4595-4603.
|
| [14] |
Luo L, Lou L P, Cui X Y, et al. Sorption and desorption of pentachlorophenol to black carbon of three different origins[J]. Journal of Hazardous Materials, 2011,185(2/3):639-646.
|
| [15] |
Lin K, Ding J, Wang H, et al. Goethite-mediated transformation of bisphenol A[J]. Chemosphere, 2012,89(7):789-795.
|
| [16] |
张晶,郭学涛,葛建华,等.针铁矿-腐殖酸的复合物对泰乐菌素的吸附[J]. 环境工程学报, 2016,10(3):1145-1151.
|
| [17] |
Lian F, Sun B B, Chen X, et al. Effect of humic acid (HA) on sulfonamide sorption by biochars[J]. Environmental Pollution, 2015,204:306-312.
|
| [18] |
Zhang Q, Zhao L, Dong Y H, et al. Sorption of norfloxacin onto humic acid extracted from weathered coal[J]. Journal of Environmental Management, 2012,102:165-172.
|
| [19] |
Guo X T, Dong H, Yang C, et al. Application of goethite modified biochar for tylosin removal from aqueous solution[J]. Colloids and Surfaces A:Physicochemical and Engineering Aspects, 2016,502:81-88.
|
| [20] |
Zhang J, He M C, Lin C Y, et al. Phenanthrene sorption to humic acids, humin, and black carbon in sediments from typical water systems in China[J]. Environmental Monitoring and Assessment, 2010,166(1-4):445-459.
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