太湖西岸沉积物中两种致嗅物质的分布特征

Abstract
Figure/Table
References (37)
Related Citation (15)

Download: PDF (752 KB) HTML (1 KB)
Export: BibTeX | EndNote (RIS)

Abstract

In this study, two typical particulate taste and odor compounds of β-Cyclocitral and β-Ionone in the sediments of the west littoral zone of Lake Taihu were investigated, by applying the headspace solid phase micro extraction method and the preconcentration and temperament combined technology. The results displayed that the highest contents of the β-Cyclocitral and β-Ionone in the surface sediments around the Maodu River was detected to be 797.88ng/(g·dw) and 1669.37ng/(g·dw), respectively, which was far higher than that of olfactory threshold. In the spatial distribution, the content of the taste and odor compounds was higher in natural reed zone than that of the artificial reed ditch in the surface sediment (<4cm), and similarly, it was higher in the near shore than that of in the open area. When the high-density cyanobacteria gathered, died and deposited to the bottom of the lake, the sediment Eh was reduced, which promoted the produce of taste and odor compounds and the formation of black-bloom. Therefore, we propose to immediately remove the cyanobacteria and dredge the sediments in the littoral zone of Lake Taihu.

Key words： HS-SPME GC/MS sediment β-cyclocitral β-ionone

Received: 30 March 2016

PACS:

X131.2

	Service

	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	LIU Xian-sheng
	XU Xiao-guang
	HUANG He-yong
	ZHAO Yan-ping
	CHEN Chong
	ZHAO Yue
	WANG Guo-xiang

Cite this article:

LIU Xian-sheng,XU Xiao-guang,HUANG He-yong等. Analysis of two odorous compounds in sediment in west nearshore zone of Taihu[J]. CHINA ENVIRONMENTAL SCIENCECE, 2017, 37(1): 302-309.

URL:

http://manu36.magtech.com.cn/Jweb_zghjkx/EN/ OR http://manu36.magtech.com.cn/Jweb_zghjkx/EN/Y2017/V37/I1/302

[1]	卢信,冯紫艳,商景阁,等.不同有机基质诱发的水体黑臭及主要致臭物(VOSCs)产生机制研究[J]. 环境科学, 2012,33(9):3152-3159.
[2]	Shen Q, Liu C, Zhou Q, et al. Effects of physical and chemical characteristics of surface sediments in the formation of shallow lake algae-induced black bloom[J]. Journal of Environmental Sciences, 2013,25(12):2353-2360.
[3]	He W, Shang J, Lu X, et al. Effects of sludge dredging on the prevention and control of algae-caused black bloom in Taihu Lake, China[J]. Journal of Environmental Sciences, 2013,25(3):430-440.
[4]	Shen Q, Zhou Q, Shang J, et al. Beyond hypoxia:occurrence and characteristics of black blooms due to the decomposition of the submerged plant Potamogeton crispus in a shallow lake[J]. Journal of Environmental Sciences, 2014,26(2):281-288.
[5]	刘小华,叶英,袁宁,等.吹扫捕集法结合三重四极杆气质联用仪测定水中5种臭味物质含量[J]. 环境化学, 2014,33(6):1056-1058.
[6]	杨华,席劲瑛,胡洪营,等. HS-SPME-GC-MS法测定黑臭河流中二甲基三硫醚[J]. 环境科学与技术, 2011,(S1):223-226.
[7]	张锡辉,伍婧娉,王治军,等. HS-SPME-GC法测定水中典型嗅味物质[J]. 中国给水排水, 2007,23(2):78-82.
[8]	黎雯,吴文忠.东湖富营养水体中藻菌异味性次生代谢产物的研究[J]. 生态学报, 1999,19(2):212-216.
[9]	李林,宋立荣,甘南琴,等.顶空固相微萃取-气相色谱-质谱测定水中异味化合物[J]. 分析化学, 2005,33(8):1058-1062.
[10]	李林.淡水水体中藻源异味化合物的分布,动态变化与降解研究[D]. 武汉:中国科学院水生生物研究所, 2005.
[11]	李大鹏,李伟光.S市水源水致臭物质分析研究[J]. 苏州科技学院学报:工程技术版, 2006,19(2):52-53.
[12]	Chen J, Xie P, Ma Z, et al. A systematic study on spatial and seasonal patterns of eight taste and odor compounds with relation to various biotic and abiotic parameters in Gonghu Bay of Lake Taihu, China[J]. Science of the Total Environment, 2010,409(2):314-325.
[13]	于建伟,李宗来,曹楠,等.无锡市饮用水嗅味突发事件致嗅原因及潜在问题分析[J]. 环境科学学报, 2007,(11):1771-1777.
[14]	Ashitani K, Hishida Y, Fujiwara K. Behavior of musty odorous compounds during the process of water treatment[J]. Water Science and Technology, 1988,20(8/9):261-267.
[15]	Li L, Wan N, Gan N Q, et al. Annual dynamics and origins of the odorous compounds in the pilot experimental area of Lake Dianchi, China[J]. Water Science & Technology, 2007,55(5).
[16]	邵晨,黎雷,于水利,等.产嗅藻类对东太湖某地原水中嗅味物质2-MIB的贡献[J]. 中国环境科学, 2014,34(9):2328-2333.
[17]	李巧霞,潘纲,王丹,等.太湖十八湾嗅味物质变化规律及除嗅方法[J]. 环境工程学报, 2012,6(9):3191-3195.
[18]	成银,高乃云,张可佳.硫醚类嗅味物质的检测和去除技术研究进展[J]. 四川环境, 2011,30(2):119-124.
[19]	Yu S, Xiao Q, Zhong X, et al. Simultaneous determination of six earthy-musty smelling compounds in water by headspace solid- phase microextraction coupled with gas chromatography-mass spectrometry[J]. Analytical Methods, 2014,6(22):9152-9159.
[20]	Martínez C, Ramírez N, Gómez V, et al. Simultaneous determination of 76micropollutants in water samples by headspace solid phase microextraction and gas chromatography- mass spectrometry[J]. Talanta, 2013,116:937-945.
[21]	马康,张金娜,何雅娟,等.顶空固相微萃取-气质联用测定环境水样中7种痕量土霉味物质[J]. 分析化学, 2011,29(12):1823- 1829.
[22]	Gostelow P, Parsons S A, Stuetz R M. Odour measurements for sewage treatment works[J]. Water Research, 2001,35(3):579- 597.
[23]	刘树娟.硝酸钙对深圳河底泥中嗅味物质原位控制方法研究[D]. 北京:清华大学, 2012.
[24]	Zuo Y, Li L, Zhang T, et al. Contribution of Streptomyces in sediment to earthy odor in the overlying water in Xionghe Reservoir, China[J]. Water Research, 2010,44(20):6085-6094.
[25]	Kamermans P, Malta E, Verschuure J M, et al. Role of cold resistance and burial for winter survival and spring initiation of an Ulva spp. (Chlorophyta) bloom in a eutrophic lagoon (Veerse Meer lagoon, The Netherlands)[J]. Marine Biology, 1998, 131(1):45-51.
[26]	郑西来,张俊杰,陈蕾.再悬浮条件下沉积物内源磷迁移-转化机制研究进展[J]. 水科学进展, 2013,24(2):287-295.
[27]	应太林,张国莹.苏州河水体黑臭机理及底质再悬浮对水体的影响[J]. 上海环境科学, 1997,16(1):23-26.
[28]	Zimba P V, Grimm C C. A synoptic survey of musty/muddy odor metabolites and microcystin toxin occurrence and concentration in southeastern USA channel catfish (Ictalurus punctatus Ralfinesque) production ponds[J]. Aquaculture, 2003,218(1):81-87.
[29]	Ozaki K, Ohta A, Iwata C, et al. Lysis of cyanobacteria with volatile organic compounds[J]. Chemosphere, 2008,71(8):1531- 1538.
[30]	徐琛宇,李翠梅,袁祥,等.太湖上山水源地嗅味物质的研究与分析[J]. 生态与农村环境学报, 2015,31(5):736-742.
[31]	傅若农.固相微萃取(SPME)近几年的发展[J]. 分析试验室, 2015,(5):602-620.
[32]	Deng X, Xie P, Qi M, et al. Microwave-assisted purge-and-trap extraction device coupled with gas chromatography and mass spectrometry for the determination of five predominant odors in sediment, fish tissues, and algal cells[J]. Journal of Chromatography A, 2012,1219:75-82.
[33]	金星.藻类代谢产物中典型异味物质及其变化规律研究[D]. 南京:南京理工大学, 2009.
[34]	齐敏,孙小雪,邓绪伟,等.太湖不同形态异味物质含量,相互关系及其与环境因子关系的探讨[J]. 湖泊科学, 2013,25(1):31- 38.
[35]	崔连艳.固相微萃取-超临界萃取-气质联用方法在测定有机锡污染中的应用[D]. 南宁:广西大学, 2008.
[36]	王国芳,李先宁,方洋,等.底泥对藻源型局部黑臭水体形成的影响[J]. 湖南大学学报(自然科学版), 2014,12:102-108.
[37]	叶春,李春华,陈小刚,等.太湖湖滨带类型划分及生态修复模式研究[J]. 湖泊科学, 2012,24(6):822-828.