|
|
Single particle characteristics of fine particulate matter in dust |
YU Nan-jiao1,2, HUANG Bo3, LI Mei1,2, CHENG Peng1,2, LI Lei1,2, HUANG Zheng-xu1,2, GAO Wei1,2, ZHOU Zhen1,2 |
1. Institute of Mass Spectrometer and Atmospheric Environmental, Jinan University, Guangzhou 510632, China;
2. Guangdong Engineering Research Center for atmospheric pollution online source apportionment system, Jinan University, Guangzhou 510632, China;
3. Guangzhou Hexin Instrument Company Limited, Guangzhou 510530, China |
|
|
Abstract Soil dust, road dust, construction dust and coal stock dust in Guangzhou were sampled, The size distributions and chemical composition of fine particles from sampled fugitive dusts were analyzed using a single particle aerosol mass spectrometer (SPAMS). Construction dust and other three types of fugitive dust showed bimodal and unimodal size distribution, respectively. The chemical composition of different dusts had a great diversity. The particles from soil dust were dominated by AlRich particles,accounting for 37.97% of the total number of ionized particles; The particles from road dust were dominated by CaRich particles which accounted for 24.92% of the total number of ionized particles; particles from construction dust were dominated by SiRich particles, accounting for 33.33% of the total number of ionized particles; particles from coal stock dust were dominated by CaRich particles, accounting for 64.92% of the total number of ionized particles. It is noted that road dust showed distinct characteristics of soil dust and motor vehicle exhaust. These unique characteristics of fugitive dust enable further source apportionment of dust particles. In addition, the percentage of secondary components was highest in road dust.
|
Received: 31 August 2016
|
|
|
|
|
[1] |
Bi X, Feng Y, Wu J, et al. Source apportionment of PM10 in six cities of northern China[J]. Atmospheric Environment, 2007, 41(5):903-912.
|
[2] |
吴国平,胡 伟,滕恩江,等.我国四城市空气中PM2.5和PM10的污染水平[J]. 中国环境科学, 1999,19(2):133-137.
|
[3] |
徐 虹,林丰妹,毕晓辉,等.杭州市大气降尘与PM10化学组成特征的研究[J]. 中国环境科学, 2011,31(1):1-7.
|
[4] |
南开大学,中国环境科学研究院,中国科学院大气物理研究所,等.大气颗粒物来源解析技术指南(试行)[EB/OL].http://www.mep.gov.cn/gkml/hbb/bwj/201308/t20130820_257699.htm,2013-08-14.
|
[5] |
张 晶,胡春玲,任 庆,等.城市扬尘污染现状及防治对策[J]. 环境保护科学, 2008,34(2):4-6.
|
[6] |
黄辉军,刘红年,蒋维楣,等.南京市PM2.5物理化学特性及来源解析[J]. 气候与环境研究, 2006,11(6):713-722.
|
[7] |
宋 娜,徐 虹,毕晓辉,等.海口市PM2.5和PM10来源解析[J]. 环境科学研究, 2015,28(10):1501-1509.
|
[8] |
肖致美,毕晓辉,冯银厂,等.宁波市环境空气中PM10和PM2.5来源解析[J]. 环境科学研究, 2012,25(5):549-555.
|
[9] |
吴 虹,张彩艳,王 静,等.青岛环境空气 PM10和PM2.5污染特征与来源比较[J]. 环境科学研究, 2013,26(6):583-589.
|
[10] |
Kong S, Han B, Bai Z, et al. Receptor modeling of PM2.5, PM10 and TSP in different seasons and long-range transport analysis at a coastal site of Tianjin, China[J]. Science of the Total Environment, 2010,408(20):4681-4694.
|
[11] |
杜 娟.广州PM2.5一半是"二手"[N]. 广州日报, 2015-4-20(04).
|
[12] |
Cao J J, Chow J C, Watson J G, et al. Size-differentiated source profiles for fugitive dust in the Chinese Loess Plateau[J]. Atmospheric Environment, 2008,42(10):2261-2275.
|
[13] |
Kong S, Ji Y, Lu B, et al. Characterization of PM10 source profiles for fugitive dust in Fushun-a city famous for coal[J]. Atmospheric Environment, 2011,44:5351-5365.
|
[14] |
Ho K F, Lee S C, Chow J C, et al. Characterization of PM10 and PM2.5 source profiles for fugitive dust in Hong Kong[J]. Atmospheric Environment, 2003,37(8):1023-1032.
|
[15] |
冯银厂,白志鹏,朱 坦,等.大气颗粒物二重源解析技术原理与应用[J]. 环境科学, 2002,(S1):108-110.
|
[16] |
Silva P J, Carlin R A, Prather K A. Single particle analysis of suspended soil dust from Southern California[J]. Atmospheric Environment, 2000,34(11):1811-1820.
|
[17] |
Dall'Osto M, Harrison R M, Highwood E J, et al. Variation of the mixing state of Saharan dust particles with atmospheric transport[J]. Atmospheric Environment, 2010,44(26):3135-3146.
|
[18] |
Fitzgerald E, Ault A P, Melanie Zauscher, et al. Comparison of the mixing state of long-range transported Asian and African mineral dust[J]. Atmospheric Environment, 2015,115:19-25.
|
[19] |
李 梅,李 磊,黄正旭,等.运用单颗粒气溶胶质谱技术初步研究广州大气矿尘污染[J]. 环境科学研究, 2011,24(6):632-636.
|
[20] |
中国环境监测总站, 北京市环境保护监测中心,上海市环境监测中心,等.环境空气颗粒物来源解析监测方法指南(试行)[EB/OL].http://www.cnemc.cn/publish/112/news/news_40443.html,2014-02-28.
|
[21] |
Song X H, Hopke P K, Fergenson D P, et al. Classification of Single Particles Analyzed by ATOFMS Using an Artificial Neural Network, ART-2A[J]. Analytical Chemistry, 1999,71(4):860- 865.
|
[22] |
姬亚芹,朱 坦,白志鹏,等.天津市土壤风沙尘元素的分布特征和来源研究[J]. 生态环境, 2005,14(4):518-522.
|
[23] |
Toner S M, Sodeman D A, Prather K A. Single particle characterization of ultrafine and accumulation mode particles from heavy duty diesel vehicles using aerosol time-of-flight mass spectrometry[J]. Environmental Science & Technology, 2006,40(40):3912-3921.
|
[24] |
Shields L G, Suess D T, Prather K A. Determination of single particle mass spectral signatures from heavy-duty diesel vehicle emissions for PM2.5, source apportionment[J]. Atmospheric Environment, 2007,41(18):3841-3852.
|
[25] |
Chow J C, Watson J G, Kuhns H, et al. Source profiles for industrial, mobile, and area sources in the Big Bend Regional Aerosol Visibility and Observational study[J]. Chemosphere, 2004,54(2):185-208.
|
[26] |
Dall'Osto M, Beddows D C S, Gietl J K, et al. Characteristics of tyre dust in polluted air:Studies by single particle mass spectrometry (ATOFMS)[J]. Atmospheric Environment, 2014,94:224-230.
|
[27] |
杜 娟,宋韶华,张志朋,等.桂林市细颗粒物典型排放源单颗粒质谱特征研究[J]. 环境科学学报, 2015,35(5):1556-1562.
|
[28] |
王 玮,张 晶,汤大钢,等.可吸入颗粒物(IP)源解析[R]. 北京:中国环境科学研究院, 1999.
|
[29] |
刘桂建,杨萍玥,彭子成.煤灰基本特征及其微量元素的分布规律[J]. 煤炭转化, 2003,26(2):81-86.
|
[30] |
付怀于,闫才青,郑 玫,等.在线单颗粒气溶胶质谱SPAMS对细颗粒物中主要组分提取方法的研究[J]. 环境科学, 2014,(11):4070-4077.
|
|
|
|