春节前后华北平原农村地区黑碳浓度及来源

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Abstract To obtain the mass concentrations, diurnal variations and sources of black carbon (eBC) aerosol around the Chinese spring festival (SF) in rural regions of the North China Plain, one-month (2018-2-12~2018-3-12) online continuous measurement of black carbon was conducted at a rural site in Henan province. During the SF, the eBC concentration was highest, (8.22±4.17)μg/m³, suggesting intensive emissions from anthropogenic activities. Before the SF, the contribution of biomass burning was the largest (41.1±5.3)%, and then gradually decreased down to (26.8±12.0)%. During the study period, the calculated AAE value (1.40±0.16) indicated that the contribution of biomass burning to eBC was close to that of fossil fuel in this area. Compared with some urban sites, the AAE value in this study was higher. Before and after the SF, the eBC mass concentrations show significant diurnal variations, with 2 peak values occurring at 07:00~09:00 and around 20:00 (local time). During the SF, the diurnal variation of eBC mass concentration did not fluctuate obviously. According to the concentration-weighted trajectories analysis, the main potential source regions of eBC were Shanxi, Shaanxi, Anhui, and Jiangsu provinces during the SF. In other two periods, Henan and Hubei provinces could be the main impact regions. This study is meaningful to identify the impact of BC emitted from rural combustion sources on regional haze formation and evolution, and it can also supply the dataset for corresponding modeling of BC's impacts on climate, air quality and human health.

Key words： black carbon aerosol the spring festival sources rural region North China Plain

Received: 22 January 2019

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	LIU Xi
	KONG Shao-fei
	ZHENG Shu-rui
	ZHENG Huang
	YAN Qin
	WU Jian
	CHENG Yi
	WU Fang-qi
	NIU Zhen-zhen
	ZENG Xin
	CHEN Nan
	XU Ke
	QI Shi-hua

Cite this article:

LIU Xi,KONG Shao-fei,ZHENG Shu-rui等. Levels and sources of black carbon around the spring festival at a rural site of the North China Plain[J]. CHINA ENVIRONMENTAL SCIENCECE, 2019, 39(8): 3169-3177.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2019/V39/I8/3169

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