盘锦市夏冬季PM<sub>2.5</sub>中碳组分污染特征及来源分析

Abstract
Figure/Table
References
Related Citation (15)

Download: PDF (411 KB) HTML (1 KB)
Export: BibTeX | EndNote (RIS)

Abstract In order to study the characteristics and sources of carbon components in PM_2.5 during summer and winter in Panjin City, PM_2.5 samples were collected from three sites in July 2016 and January 2017. The results showed that the average concentrations of PM_2.5, Organic Carbon (OC) and Element Carbon (EC) were (46.14±12.70), (8.58±2.82) and (2.89±1.54) μg/m³ in summer, and (91.01±43.51), (24.50±15.51) and (7.31±5.00) μg/m³in winter, respectively. The correlations between OC and EC in development zone and NO.2 middle school were not significant in summer while OC was strongly correlated with EC at all sampling sites in winter. The SOC concentrations were calculated based on the Minimum R Squired method, which were 4.65μg/m³ in summer and 8.42μg/m³ in winter, accounting for 54.19% and 34.36% of the total OC, respectively. By means of ratio analysis and principal component analysis, the main sources of carbon components were gasoline vehicle exhaust and coal-fired emissions in summer, and vehicle exhaust, coal-fired emissions and biomass burning in winter.

Key words： Panjin city PM_2.5 carbon component source apportionment

Received: 06 January 2019

PACS:

X513

	Service

	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	GUO Ji-liang
	JI Ya-qin
	MA Yan
	WANG Shi-bao
	ZHANG Lei
	LI Yue-yang
	ZHAO Jing-qi

Cite this article:

GUO Ji-liang,JI Ya-qin,MA Yan等. Pollution characteristics and sources of carbon components in PM_2.5 during summer and winter in Panjin city[J]. CHINA ENVIRONMENTAL SCIENCECE, 2019, 39(8): 3201-3206.

URL:

http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2019/V39/I8/3201

[1]	刘新民,邵敏,曾立民,等.珠江三角洲地区气溶胶中含碳物质的研究[J]. 环境科学, 2002,23(S1):54-59. Liu X M, Shao M, Zeng L M, et al. Study on EC and OC Compositions of Ambient Particles in Pearl River Delta Region[J]. Environmental Science, 2002,23(S1):54-59.
[2]	Huang L, Brook J R, Zhang W, et al. Stable isotope measurements of carbon fractions (OC/EC) in air borne particulate:a new dimension for source characterization and apportionment[J]. Atmospheric Environment, 2006,40(15):2690-2705.
[3]	王果,迪丽努尔•塔力甫,买里克扎提•买合木提,等.乌鲁木齐市PM2.5和PM2.5~10中碳组分季节性变化特征[J]. 中国环境科学, 2016,36(2):356-362. Wang G, Dilnur T, Mailikezhati M, et al. Seasonal changes of carbonaceous species in PM2.5, PM2.5~10 in Urumqi[J]. China Environmental Science, 2016,36(2):356-362.
[4]	Glasius M, Hansen A M K, Claeys M, et al. Composition and sources of carbonaceous aerosols in Northern Europe during winter[J]. Atmospheric Environment, 2018,173:127-141.
[5]	吴琳,冯银厂,戴莉,等.天津市大气中PM10、PM2.5及其碳组分污染特征分析[J]. 中国环境科学, 2009,29(11):1134-1139. Wu L, Feng Y C, Dai L, et al. Characteristics of PM10, PM2.5 and their carbonaceous species in Tianjin City[J]. China Environmental Science, 2009,29(11):1134-1139.
[6]	王伟,姬亚芹,赵哲,等.鞍山城区夏季PM2.5中碳组分污染特征及来源[J]. 环境工程技术学报, 2015,5(2):91-96. Wang W, Ji Y Q, Zhao Z, et al. Pollution characteristics of carbon fractions in PM2.5 and their sources in urban area of Anshan City in summer[J]. Journal of Environmental Engineering Technology, 2015,5(2):91-96.
[7]	安欣欣,张大伟,冯鹏,等.北京城区夏季PM2.5中碳组分和二次水溶性无机离子浓度特征[J]. 环境化学, 2016,35(4):713-720. An X X, Zhang D W, Feng P, et al. Characteristics of carbon components and secondary water-soluble inorganic ions in PM2.5 in summer in urban Beijing[J]. Environmental Chemistry, 2016,35(4):713-720.
[8]	元洁,刘保双,程渊,等.2017年1月天津市区PM2.5化学组分特征及高时间分辨率来源解析研究[J]. 环境科学学报, 2018,38(3):1090-1101. Yuan J, Liu B S, Cheng Y, et al. Study on characteristics of PM2.5 and chemical components and source apportionment of high temporal resolution in January 2017 in Tianjin urban area[J]. Acta Scientiae Circumstantiae, 2018,38(3):1090-1101.
[9]	程渊,刘保双,毕晓辉,等.天津市区夏冬季环境空气PM2.5中碳组分污染特征及来源研究[J]. 环境科学学报, 2018,38(9):3394-3405. Cheng Y, Liu B S, Bi X H, et al. Character and source analysis of carbonaceous aerosol in PM2.5 during summer-winter period, Tianjin urban area[J]. Acta Scientiae Circumstantiae, 2018,38(9):3394-3405.
[10]	王杨君,董亚萍,冯加良,等.上海市PM2.5中含碳物质的特征和影响因素分析[J]. 环境科学, 2010,31(8):1755-1761. Wang Y J, Dong Y P, Feng J L, et al. Characteristics and influencing factors of carbonaceous aerosols in PM2.5 in Shanghai, China[J]. Environmental Science, 2010,31(8):1755-1761.
[11]	朱李华,陶俊,张仁健,等.冬夏季广州城区碳气溶胶特征及其与O3和气象条件的关联[J]. 环境科学学报, 2010,30(10):1942-1949. Zhu L H, Tao J, Zhang R J, et al. Characteristics of the carbonaceous aerosol in PM2.5 and its relation to O3and meteorological conditions in the urban Guangzhou area in winter and summer[J]. Acta Scientiae Circumstantiae, 2010,30(10):1942-1949.
[12]	成海容,王祖武,冯家良,等.武汉市城区大气PM2.5的碳组分与源解析[J]. 生态环境学报, 2012,21(9):1574-1579. Cheng H R, Wang Z W, Feng J L, et al. Carbonaceous species composition and source apportionment of PM2.5 in urban atmosphere of Wuhan[J]. Ecology and Environmental Sciences, 2012,21(9):1574-1579.
[13]	张承中,丁超,周变红,等.西安市冬、夏两季PM2.5中碳气溶胶的污染特征分析[J]. 环境工程学报, 2013,7(4):1477-1481. Zhang C Z, Ding C, Zhou B H, et al. Pollution characteristics of carbon aerosol in PM2.5 of Xi'an during winter and summer[J]. Chinese Journal of Environmental Engineering, 2013,7(4):1477-1481.
[14]	云龙龙,陆钒,张天舒,等.无锡市冬季典型天气PM2.5中碳组分的污染特征[J]. 环境科学, 2014,35(9):3280-3286. Yun L L, Lu F, Zhang T S, et al. Pollution characteristics of carbonaceous aerosols in PM2.5 during typical winter days in Wuxi City[J]. Environmental Science, 2014,35(9):3280-3286.
[15]	Weber C, Sundvor I, Figenbaum E. Comparison of regulated emission factors of Euro 6LDV in Nordic temperatures and cold start conditions:Diesel-and gasoline direct-injection[J]. Atmospheric Environmental, 2019,206:208-217.
[16]	田莎莎,张显,卞思思,等.沈阳市PM2.5污染组分特征及其来源解析[J]. 中国环境科学, 2019,39(2):487-496. Tian S S, Zhang X, Bian S S, et al. Characteristics of PM2.5pollution components and their sources in Shenyang[J]. China Environmental Science, 2019,39(2):487-496.
[17]	张伟,姬亚芹,李金,等.鞍山市夏冬季PM2.5中碳组分化学特征及来源解析[J]. 中国环境科学, 2017,37(5):1657-1662. Zhang W, Ji Y Q, Li J, et al. The characteristics and source apportionment of carbon fractions in PM2.5during summer-winter period in Anshan City[J]. China Environmental Science, 2017,37(5):1657-1662.
[18]	王珍,郭军,陈卓,等.贵阳市秋、冬季PM2.5中碳组分污染特征及来源分析[J]. 地球与环境, 2015,43(3):285-289. Wang Z, Guo J, Chen Z, et al. Characteristics and source analysis of carbonaceous aerosols in PM2.5 of Guiyang City, P.R. China during autumn-winter period[J]. Earth and Environment, 2015,43(3):285-289.
[19]	Turpin B J, Huntzicker J J. Identification of secondary organic aerosol episodes and quantitation of primary and secondary organic aerosol concentrations during SCAQS[J]. Atmospheric Environment, 1995, 29(23):3527-3544.
[20]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of emissions from air pollution sources. 2. C1through C30 organic compounds from medium duty diesel trucks[J]. Environmental Science and Technology, 1999,33(10):1578-1587.
[21]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of emissions from air pollution sources. 5. C1-C32organic compounds from gasoline-powered motor vehicles[J]. Environmental Science and Technology, 2002,36:1169-1180.
[22]	Chen Y J, Zhi G R, Feng Y L, et al. Measurements of emission factors for primary carbonaceous particles from residential raw-coal combustion in China[J]. Geophysical Research Letters, 2006,332(20):382-385.
[23]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of emissions from Air Pollution Sources. 3. C1-C29organic compounds from fireplace combustion of wood[J]. Environmental Science and Technology, 2001,35:1716-1728.
[24]	He L Y, Hu M, Huang X F, et al. Measurement of emissions of fine particulate organic matter from Chinese cooking[J]. Atmospheric Environment, 2004,38:6557-6564.
[25]	Millet D B, Donahue N M, Pandis S N, et al. Atmospheric volatile organic compound measurements during the Pittsburgh Air Quality Study:Results, interpretation, and quantification of primary and secondary contributions[J]. Journal of Geophysical Research-Atmospheres, 2005,110,D07S07:1-17.
[26]	Ji D S, Gao M, Maenhaut W, et al. The carbonaceous aerosol levels still remain a challenge in the Beijing-Tianjin-Hebei region of China:Insights from continuous high temporal resolution measurements in multiple cities[J]. Environment international, 2019,126:171-183.
[27]	Wu C, Yu J Z. Determination of primary combustion source organic carbon-to-elemental carbon (OC/EC) ratio using ambient OC and EC measurements:secondary OC-EC correlation minimization method[J]. Atmospheric Chemistry and Physics, 2016,16(8):5453-5465.
[28]	张灿,周志恩,翟崇治,等.基于重庆本地碳成分谱的PM2.5碳组分来源分析[J]. 环境科学, 2014,35(3):810-819. Zhang C, Zhou Z E, Zhai C Z, et al. Carbon source apportionment of PM2.5 in Chongqing Based on Local Carbon Profiles[J]. Environmental Science, 2014,35(3):810-819.
[29]	Xu H M, Cao J J, Chow J C, et al. Inter-annual variability of wintertime PM2.5 chemical composition in Xi'an, China:evidences of changing source emissions[J]. Science of the Total Environment, 2016,545:546-555.
[30]	Cao J J, Wu F, Chow J C, et al. Characterization and source apportionment of atmospheric organic and elemental carbon during fall and winter of 2003 in Xi'an, China[J]. Atmospheric Chemistry and Physics, 2005,5(11):3127-3137.
[31]	Watson J G, Chow J C, Lowenthal D H, et al. Differences in the carbon composition of source profiles for diesel-and gasoline powered vehicles[J]. Atmospheric Environment, 1994,28(15):2493-2505.