海拉尔盆地地下水铀的分布特征及富集规律

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Abstract 12 surface water samples and 67 groundwater samples were collected from the Hailar Basin. The distribution characteristics and occurrence patterns of uranium in groundwater of samples were analyzed using Durov diagrams, contour maps, uranium form calculation theory, as well as mathematical statistics. Results show that the Helhongde sag area of the Hailar Basin is mainly HCO₃-Ca·Na type, the Wagang uplift, Wuerxun sag and Beier sag area are mainly Cl-Na type and HCO₃-Na type, and the Bayanshan uplift area was mainly HCO₃-Ca·Na type. Hongqi Ranch and Xinbaolige depression were mainly Cl-Na type. The distribution of uranium in the study area ranged from 17 to 425μg/L, with an average of 80μg/L and a standard deviation of 70μg/L, which may indicate a regional groundwater uranium pollution. UO₂(CO₃)₃^4- and UO₂(CO₃)₂^2- are the dominate forms of uranium in groundwater, which is consistent with the redox environment of Eh, indicating a favorable environment for uranium mineralization in groundwater in the southeast of Hulunbuir Lake. Uranium mineralization prefers HCO₃^-type uranium-containing groundwater where uranyl bicarbonate is dominant, and the uranyl carbonate complex should be the dominate form. The dissolution of uranium is related to the increase of HCO₃^-. Uranium in groundwater may have participated in the mixed leaching of carbonate rock and sulfate rock. UO₂(CO₃)₃^4-, UO₂(CO₃)₂^2-, U₄O₉and bituminous ore are in a saturated state, while the concentrations of total Fe and (Ca²⁺+Mg²⁺) were low. Various water chemical indicators are indicative of uranium enrichment, so they can be regarded as references for potential uranium sources.

Key words： Hailar groundwater uranium hydrogeochemistry

Received: 03 June 2020

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X523

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	Articles by authors
	ZHANG Hai-yang
	GAO Bai
	GE Qin
	HUA En-xiang
	HUANG Shao-hua
	YI Ling
	SHEN Wei
	LIN Cong-ye

Cite this article:

ZHANG Hai-yang,GAO Bai,GE Qin等. The distribution and enrichment of Uranium in groundwater of Hailar Basin[J]. CHINA ENVIRONMENTAL SCIENCECE, 2021, 41(1): 223-231.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2021/V41/I1/223

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