阴离子嵌段磁性混凝剂去除低浓度亚甲基蓝

Abstract
Figure/Table
References
Related Citation (15)

Download: PDF (2941 KB) HTML (1 KB)
Export: BibTeX | EndNote (RIS)

Abstract Template anionic polyacrylamide (TAPAM) with anionic block structure was synthesized by template method, then modified with polydopamine (PDA) and grafted with Fe₃O₄ nanoparticles by chelation, named TAPAM-PDA-Fe₃O₄. Compared with PDA and APAM-Fe₃O₄ in the removal of methylene blue, the results illustrated that TAPAM-PDA-Fe₃O₄ showed the highest removal rate and the dominant effect of π-π stacking under neutral/alkaline conditions(7.03O₄ could effectively remove methylene blue at low concentrations.When the initial concentration of methylene blue was 4mg/L and the pH value was 9, the maximum removal efficiency reached 97.5%.

Key words： magnetic coagulation coagulant water treatment preparation UV irradiation

Received: 18 December 2020

PACS:

X703.5

	Service

	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	ZHENG Huai-li
	YU Zhi-shuang
	ZHAO Rui
	LI Hong
	SUN Qiang
	HU Ya-dan
	JIANG Jun-yi

Cite this article:

ZHENG Huai-li,YU Zhi-shuang,ZHAO Rui等. Removal of low concentration methylene blue by anionic block magnetic coagulant[J]. CHINA ENVIRONMENTAL SCIENCECE, 2021, 41(8): 3567-3575.

URL:

http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2021/V41/I8/3567

[1]	Deng H, Lu J J, Li G X, et al. Adsorption of methylene blue on adsorbent materials produced from cotton stalk[J]. Chemical Engineering Journal, 2011,172(1):326-334.
[2]	Novais R M, Ascensão G, Tobaldi D M, et al. Biomass fly ash geopolymer monoliths for effective methylene blue removal from wastewaters[J]. Journal of Cleaner Production, 2017,171(pt.1):783-794.
[3]	徐继红,段贤扬,何梦奇,等.GA-g-PAMPS/AA/ST凝胶的制备及对亚甲基蓝吸附性能[J]. 中国环境科学, 2020,40(10):4362-4369. Xu J H, Duan X Y, He M Q, et al. Preparation of GA-g-PAMPS/AA/ST hydrogel and adsorption properties for methylene blue[J]. Chinese Environmental Science, 2020,40(10):4362-4369.
[4]	Fan S S, Wang Y, Wang Z, et al. Removal of methylene blue from aqueous solution by sewage sludge-derived biochar:Adsorption kinetics, equilibrium, thermodynamics and mechanism[J]. Journal of Environmental Chemical Engineering, 2017,5(1):601-611.
[5]	Vilar V J P, Botelho C M S, Boaventura R A R. Methylene blue adsorption by algal biomass based materials:Biosorbents characterization and process behaviour[J]. Journal of Hazardous Materials, 2007,147(1/2):120-132.
[6]	Lau Y-Y, Wong Y-S, Teng T-T, et al. Degradation of cationic and anionic dyes in coagulation-flocculation process using bi-functionalized silica hybrid with aluminum-ferric as auxiliary agent[J]. Rsc Advances, 2015,5(43):34206-34215.
[7]	Verma A K, Dash R R, Bhunia P. A review on chemical coagulation/flocculation technologies for removal of colour from textile wastewaters[J]. Journal of Environmental Management, 2012,93(1):154-168.
[8]	郭俊元,陈诚,刘文杰.微生物絮凝剂及与壳聚糖复配处理亚甲基蓝废水[J]. 中国环境科学, 2017,37(9):3346-3352. Guo J Y, Chen C, Liu W J. A bioflocculant and its performances in treatment of methylene blue wastewater by composited with chitosan[J]. Chinese Environmental Science, 2017,37(9):3346-3352.
[9]	Sun Q, Zheng H L, Zheng X Y, et al. Dual polydopamine-anion polyacrylamide polymer system for improved removal of nickel ions and methylene blue from aqueous solution[J]. Science of Advanced Materials, 2019,11(1):116-127.
[10]	Hosseinzadeh H, Khoshnood N. Removal of cationic dyes by poly(AA-co-AMPS)/montmorillonite nanocomposite hydrogel[J]. Desalination and water treatment, 2016,57(14):6372-6383.
[11]	李冬梅,李树彬,林显增,等.NGO/PDA-DAG改性膜制备及抗污染性能研究[J]. 中国环境科学, 2020,40(12):5299-5307. Li D M, Li S S, Lin X Z, et al. Study on the preparation of NGO/PDA-DAG modified membrane and its anti-fouling performance[J]. Chinese Environmental Science, 2020,40(12):5299-5307.
[12]	Mao B Q, An Q D, Zhai B, et al. Multifunctional hollow polydopamine-based composites (Fe3O4/PDA@Ag) for efficient degradation of organic dyes[J]. Rsc Advances, 2016,6(53):47761-47770.
[13]	Ma S, Feng J, Qin W, et al. CuFe2O4@PDA magnetic nanomaterials with a core-shell structure:synthesis and catalytic application in the degradation of methylene blue in water[J]. Rsc Advances, 2015, 5(66):53514-53523.
[14]	Pan X H, Cheng S Y, Su T, et al. Fenton-like catalyst Fe3O4@polydopamine-MnO2 for enhancing removal of methylene blue in wastewater[J]. Colloids and Surfaces B-Biointerfaces, 2019,181:226-233.
[15]	Atta A M, Al-Hussain S A, Al-Lohedan H A, et al. In situ preparation of magnetite/cuprous oxide/poly (AMPS/NIPAm) for removal of methylene blue from waste water[J]. Polymer International, 2018, 67(4):471-480.
[16]	于雯超,郑利兵,魏源送,等.磁混凝对市政污水中抗生素抗性基因和重金属抗性基因的削减效能[J]. 环境科学, 2020,41(2):815-822. Yu W C, Zheng L B, Wei Y S, et al. Removal performance of antibiotic resistance genes and heavy metal resistance genes in municipal wastewater by magnetic-coagulation process[J]. Environmental Science, 2020,41(2):815-822.
[17]	Sun Q, Zheng H L, Hu X B, et al. Magnetic template anion polyacrylamide-polydopamine-Fe3O4 combined with ultraviolet/H2O2 for the rapid enrichment and degradation of diclofenac sodium from aqueous environment[J]. Polymers, 2020,12(1):72-.
[18]	Zheng X Y, Zhang J X, Wang J, et al. Polydopamine coatings in confined nanopore space:Toward improved retention and release of hydrophilic cargo[J]. Journal of Physical Chemistry C, 2015, 119(43):24512-24521.
[19]	Veisi H, Safarimehr P, Hemmati S. Oxo-vanadium immobilized on polydopamine coated-magnetic nanoparticles (Fe3O4):A heterogeneous nanocatalyst for selective oxidation of sulfides and benzylic alcohols with H2O2[J]. Journal of the Taiwan Institute of Chemical Engineers, 2018,88:8-17.
[20]	Bao Y, Ma J Z, Li N. Synthesis and swelling behaviors of sodium carboxymethyl cellulose-g-poly(AA-co-AM-co-AMPS)/MMT superabsorbent hydrogel[J]. Carbohydrate Polymers, 2011,84(1):76-82.
[21]	Zheng H L, Ma J Y, Zhu C J, et al. Synthesis of anion polyacrylamide under UV initiation and its application in removing dioctyl phthalate from water through flocculation process[J]. Separation and Purification Technology, 2014,123:35-44.
[22]	Veisi H, Tamoradi T, Rashtiani A, et al. Palladium nanoparticles anchored polydopamine-coated graphene oxide/Fe3O4 nanoparticles (GO/Fe3O4@PDA/Pd) as a novel recyclable heterogeneous catalyst in the facile cyanation of haloarenes using K4[Fe(CN)6] as cyanide source[J]. Journal of Industrial and Engineering Chemistry, 2020, 90:379-388.
[23]	Xu K Z, Wu J, Fang Q L, et al. Magnetically separable h-Fe3O4@Au/polydopamine nanosphere with a hollow interior:A versatile candidate for nanocatalysis and metal ion adsorption[J]. Chemical Engineering Journal, 2020,398.
[24]	Li J Y, Long X Y, Yin H X, et al. Magnetic solid-phase extraction based on a polydopamine-coated Fe3O4 nanoparticles absorbent for the determination of bisphenol A, tetrabromobisphenol A, 2,4,6-tribromophenol, and (S)-1,1'-bi-2-naphthol in environmental waters by HPLC[J]. Journal of Separation Science, 2016,39(13):2562-2572.
[25]	Zhang Z X, Mwadini M A, Chen Z L. Polytetrafluoroethylene-jacketed stirrer modified with graphene oxide and polydopamine for the efficient extraction of polycyclic aromatic hydrocarbons[J]. Journal of Separation Science, 2016,39(20):4011-4018.
[26]	An Y Y, Zheng H L, Sun Q, et al. A novel floating adsorbents system of acid orange 7 removal:Polymer grafting effect[J]. Separation and Purification Technology, 2019,227:9.
[27]	Chen X X, Chen B L. Macroscopic and spectroscopic investigations of the adsorption of nitroaromatic compounds on graphene oxide, reduced graphene oxide, and graphene nanosheets[J]. Environmental Science & Technology, 2015,49(10):6181-6189.
[28]	Yang Z L, Gao B Y, Li C X, et al. Synthesis and characterization of hydrophobically associating cationic polyacrylamide[J]. Chemical Engineering Journal, 2010,161(1/2):27-33.
[29]	Zhao C L, Zheng H L, Feng L, et al. Improvement of sludge dewaterability by ultrasound-initiated cationic polyacrylamide with microblock structure:The role of surface-active monomers[J]. Materials, 2017,10(3):18.
[30]	Xing Y X, Zhang J X, Chen F, et al. Mesoporous polydopamine nanoparticles with co-delivery function for overcoming multidrug resistance via synergistic chemo-photothermal therapy[J]. Nanoscale, 2017,9(25):8781-8790.
[31]	Feng L, Zheng H L, Gao B Y, et al. Fabricating an anionic polyacrylamide (APAM) with an anionic block structure for high turbidity water separation and purification[J]. Rsc Advances, 2017,7(46):28918-28930.
[32]	Liu B Z, Zheng H L, Deng X R, et al. Formation of cationic hydrophobic micro-blocks in P(AM-DMC) by template assembly:characterization and application in sludge dewatering[J]. Rsc Advances, 2017,7(10):6114-6122.
[33]	Zheng C F, Zheng H L, Wang Y J, et al. Modified magnetic chitosan microparticles as novel superior adsorbents with huge "force field" for capturing food dyes[J]. Journal of Hazardous Materials, 2019,367:492-503.
[34]	劳德平,丁书强,倪文,等.响应面优化制备粉煤灰基PASC混凝剂性能与表征[J]. 中国环境科学, 2018,38(12):4599-4607. Li Y S, Zheng X Y, Zheng H L, et al. Response surface method optimization of preparation fly ash based polysilicate aluminum chloride coagulant:performance and microstructure characterization[J]. Chinese Environmental Science, 2018,38(12):4599-4607.
[35]	Li X, Zheng H L, Gao B Y, et al. UV-initiated template copolymerization of AM and MAPTAC:Microblock structure, copolymerization mechanism, and flocculation performance[J]. Chemosphere, 2017,167:71-81.
[36]	Guan Q Q, Zheng H L, Zhai J, et al. Preparation, characterization, and flocculation performance of P(acrylamide-co-diallyldimethylammonium chloride) by UV-initiated template polymerization[J]. Journal of Applied Polymer Science, 2015,132(13):7.
[37]	Feng L, Zheng H, Wang Y, et al. Ultrasonic-template technology inducing and regulating cationic microblocks in CPAM:characterization, mechanism and sludge flocculation performance[J]. Rsc Advances, 2017,7(38):23444-23456.
[38]	Albadarin A B, Collins M N, Naushad M, et al. Activated lignin-chitosan extruded blends for efficient adsorption of methylene blue[J]. Chemical Engineering Journal, 2017,307:264-272.
[39]	Pathania D, Sharma S, Singh P. Removal of methylene blue by adsorption onto activated carbon developed from Ficus carica bast[J]. Arabian Journal of Chemistry, 2017,10:S1445-S1451.
[40]	Marrakchi F, Ahmed M J, Khanday W A, et al. Mesoporous-activated carbon prepared from chitosan flakes via single-step sodium hydroxide activation for the adsorption of methylene blue[J]. International Journal of Biological Macromolecules, 2017,98:233-239.
[41]	Islam M A, Ahmed M J, Khanday W A, et al. Mesoporous activated coconut shell-derived hydrochar prepared via hydrothermal carbonization-NaOH activation for methylene blue adsorption[J]. Journal of Environmental Management, 2017,203:237-244.
[42]	Vinothkannan M, Karthikeyan C, kumar G G, et al. One-pot green synthesis of reduced graphene oxide (RGO)/Fe3O4 nanocomposites and its catalytic activity toward methylene blue dye degradation[J]. Spectrochimica Acta Part A:Molecular and Biomolecular Spectroscopy, 2015,136:256-264.
[43]	王刚,李嘉,何宝菊,等.两性高分子絮凝剂聚乙烯亚胺基黄原酸钠除浊性能[J]. 中国环境科学, 2018,38(12):4537-4544. Wang G, Li J, He B J, et al. Removal performance for turbidity by amphoteric macromolecule flocculant with polyethyleneimine-sodium xanthogenate.[J]. Chinese Environmental Science, 2018,38(12):4537-4544.
[44]	邬艳,杨艳玲,李星,等.三种常见混凝机理为主导条件下絮体特性研究[J]. 中国环境科学, 2014,34(1):150-155. Wu Y, Yang Y L, Li X, et al. Study on flocs characteristics under three common dominant coagulation mechanisms[J]. Chinese Environmental Science, 2014,34(1):150-155.