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Methane diffusion flux and its driving factors in Zhushan Bay of Lake Taihu |
LIU Zhen-jing1,2, XIAO Qi-tao2, HU Zheng-hua1, ZHANG Mi3, WANG Wei3, XIAO Wei3 |
1. School of Applied Meteorology, Nanjing University of Information Science and Technology, Nanjing 210044, China; 2. Key Laboratory of Watershed Geographic Science, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; 3. Yale-NUIST Center on Atmospheric Environment, Nanjing University of Information Science and Technology, Nanjing 210044, China |
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Abstract To identify the influence of input of pollutants and eutrophication on the temporal and spatial variations of the CH4 diffusion flux, monthly field measurements of CH4 flux was conducted in Zhushan Bay from November 2011 to August 2013. For comparison, the CH4 flux in the Central Zone of the lake with less impact from human activities was also determined. Results showed that the CH4 diffusion flux in Zhushan Bay with a mean value of (0.193±0.049) mmol/(m2·d) was significantly (P<0.01) higher than that ((0.024±0.005) mmol/(m2·d)) in the Central Zone. Meanwhile, the highest CH4 flux occurred at the sampling site with river discharge in Zhushan Bay. Further, the CH4 diffusion flux in the Central Zone showed apparent temporal variation, and the flux was positively correlated with water temperature (R2=0.53, P<0.01). However, the CH4 flux showed a poor correlation with water temperature in Zhushan Bay (P>0.05).In addition, both the dissolved CH4 concentration and CH4 flux in Zhushan Bay were positively correlated with the dissolved CH4 concentration in the inflowing river (concentration: R2=0.75, P<0.05; flux: R2=0.64, P<0.05). The results indicated that the external input of pollutants might weaken the effect of temperature on CH4 flux in Zhushan Bay, leading to the eutrophic Zhushan Bay being a significant source of atmospheric CH4.
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Received: 26 May 2021
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