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Spatiotemporal characteristics of ambient air pollutants in five border cities of Yunnan province: variations |
LANG Li-jun1, CUI Xiang-fen1, SHI Jian-wu1, HUANG Jian-hong1, NING Ping1, HAO Ji-ming1,2 |
1. Faculty of Environment Science and Engineering, Kunming University of Science and Technology, Kunming 650500, China; 2. School of Environment, Tsinghua University, Beijing 100084, China |
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Abstract The pollution characteristics, spatiotemporal variation and spatial heterogeneity was explored based on ambient particulate matter (PM with diameter £2.5µm [PM2.5], £10µm [PM10]) and gaseous pollutants (Ozone [O3], sulfur dioxide [SO2], nitrogen dioxide [NO2], carbon monoxide [CO]) data collected from 2015 to 2021 in five border cities of Yunnan province. Annual average concentrations of ambient air pollutants fluctuate enormously and that of PM10 (42.6±8.2)µg/m3 and PM2.5 (25.4±4.2)µg/m3 exceed the Grade Ⅱ limit value recommended the Chinese Ambient Air Quality Standards (GB 3095-2012). The monthly average concentrations showed a U-shaped trend for PM, NO2 and O3-8h, and their concentrations peaked in March. PM and NO2 concentrations followed a comparable seasonal pattern: spring>winter>autumn>summer. By contrast, seasonal average concentration of O3-8h decreased as: spring>summer>autumn>winter and that of CO was the lowest in winter. In addition, SO2 showed no obvious seasonal variation. Sen-MK results indicated a general trend of descending in daily average concentrations of ambient air pollutants and PM10 had the highest decline rate at 11×10-3µg/m3 per day, while an inverse trend of O3-8h. The coefficient of variation (COD) revealed that the spatial distribution of ambient air pollutants is extremely uneven, especially for SO2 with COD>0.2 but that of O3-8h was more uniform in spring. Person correlation analysis supported a strong correlation between PM and NO2, CO as well as O3-8h, and correlations between PM and other pollutants are stronger in Xishuangbanna (BN) than other studied cities.
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Received: 07 March 2022
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