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Characterization of contaminated construction sites in key regions |
QIAO Fei, WANG Jin-guo, ZHENG Shi-yu, WEI Yun-bo, ZHUANG Chao, YANG Dong |
Department of Earth Science and Engineering, Hohai University, Nanjing 211100, China |
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Abstract In this paper, three key regions of industrial development in China were investigated(i.e., Beijing-Tianjin-Hebei, Yangtze River Delta and Pearl River Delta regions), based on the 496contaminated sites included in the List of Soil Contamination Risk Control and Remediation of Construction Sites from 2018 to 2021. Statistical analysis was conducted on the regional distribution, soil-groundwater excess contamination characteristics, industry contamination correlation and geological conditions of the sites. The results showed that: The contaminated sites of Beijing-Tianjin-Hebei region were mainly located in Beijing-Tianjin and southern Hebei Province. The number of contaminated sites of Yangtze River Delta is the largest and the sites were widely distributed. The contaminated sites of Pearl River Delta is densely located in the Pearl River Estuary. Generally,soil contamination was dominated by the combined contamination of organic pollutants and heavy metals(48.43%), while groundwater was dominated by organic contamination(42.49%). High risk industries were chemical raw material and chemical manufacturing, metal smelting and rolling processing industry, with the risk load index greater than 0.25. The industry types of medium risk contaminated sites were plastics and rubber products industry, machinery manufacturing, metal products industry, electrical machinery and equipment manufacturing, and leather and fur manufacturing industry. The rest industry types of contaminated sites are low risk. The characteristics of the site soil-groundwater contamination were closely related to the historical industries. For example, the chemical raw materials and chemicals manufacturing industry, having the most diverse contaminations with halogenated hydrocarbons (12% of the total) and benzene (10.4% of the total), accounted for a heavier proportion than the rest of the industries. At the same time, heavy metal contamination in groundwater was serious in all industries, and conventional indicators such as ammonia nitrogen should also be noted. The maximum soil depth of exceedance for all types of typical contaminants was generally 0~5m at soil depth. The maximum soil depth of exceedance for heavy metals was greater than organic contamination. In terms of soil properties, the excess contamination was concentrated in low permeability layers such as clayey soils.
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Received: 10 April 2022
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[1] |
Peng J Y, Zhang S, Han Y, et al. Soil heavy metal pollution of industrial legacies in China and health risk assessment[J]. Science of The Total Environment, 2021,11:151632.
|
[2] |
Wu H T, Gai Z Q, Guo Y X, et al. Does environmental pollution inhibit urbanization in China? A new perspective through residents' medical and health costs[J]. Environmental Research, 2020,182(3):109128.1-109128.9.
|
[3] |
姜凯凯.城市更新背景下土地产权的退出障碍与治理对策——基于空间要素循环的视角[J]. 城市发展研究, 2021,28(8):100-106. Jiang K K. The obstacles on the withdrawal of property rights and the discussion on governance countermeasures under the background of urban renewal:Based on the circulation of urban spatial elements[J]. Urban Development Studies, 2021,28(8):100-106.
|
[4] |
Liu G, Niu J, Zhang C, et al. Characterization and assessment of contaminated soil and groundwater at an organic chemical plant site in Chongqing, Southwest China[J]. Environmental Geochemistry and Health, 2016,38(2):607-618.
|
[5] |
李翔,汪洋,鹿豪杰,等.京津冀典型区域地下水污染风险评价方法研究[J]. 环境科学研究, 2020,33(6):1315-1321. Li X, Wang Y, Lu H J, et al. Groundwater pollution risk assessment method in a typical area of Beijing-Tianjin-Hebei Region[J]. Research of Environmental Sciences, 2020,33(6):1315-1321.
|
[6] |
Zhou Y, Chen Y, Hu Y. Assessing efficiency of urban land utilisation under environmental constraints in Yangtze River Delta, China[J]. Environmental Research and Public Health, 2021,18(23):12634.
|
[7] |
Shan T H, Li X R, Huang F C, et al. Research on industrial structure transfer under the coordinated development of Beijing, Tianjin and Hebei[J]. Journal of Physics:Conference Series,2019,1176:042014.
|
[8] |
金远亮,侯德义,田莉,等.基于用地规划的污染地块修复多目标优化研究[J]. 中国环境科学, 2021,41(2):787-800. Jin Y L, Hou D Y, Tian L, et al. Multi-objective optimization for brownfield remediation on the basis of land use planning[J]. China Environmental Science, 2021,41(2):787-800.
|
[9] |
马娇阳,田稳,王坤,等.污染场地土壤重金属的生物可给性及毒性研究[J]. 中国环境科学, 2021,41(10):4885-4893. Ma J Y, Tian W, Wang K, et al. Bioaccessibility and their toxic effects of heavy metal in field soils from an electronic disassembly plant[J]. China Environmental Science, 2021,41(10):4885-4893.
|
[10] |
蒋姝睿,王玥,王萌,等.区域视角下中国工业行业与工业污染关系[J]. 中国环境科学, 2017,37(11):4380-4387. Jiang S R, Wang Y, Wang M, et al. Industrial sectors and pollution in China based on the regional perspective[J]. China Environmental Science, 2017,37(11):4380-4387.
|
[11] |
Jia X, Hu B, Marchant B P, et al. A methodological framework for identifying potential sources of soil heavy metal pollution based on machine learning:A case study in the Yangtze Delta, China[J]. Environmental Pollution, 2019,250:601-9.
|
[12] |
Gworek B,Baczewska-Dabrowska A H, Kalinowski R, et al. Ecological risk assessment for land contaminated by petrochemical industry[J]. PloS One. 2018,13(10):e0204852.
|
[13] |
何梦林,肖海麟,陈小方,等.化工园区基于排放环节的VOCs排放特征研究[J]. 中国环境科学, 2017,37(1):38-48. He M L, Xiao H L, Chen X F, et al. Emission characteristics of volatile organic compounds in chemical industry park based on emission links[J]. China Environmental Science, 2017,37(1):38-48.
|
[14] |
Long Z J, Zhang W, Shi Z L, et al. Reducible fraction dominates the mobility of vanadium in soil around an iron smelter[J]. Bulletin of Environmental Contamination and Toxicology, 2020,105(6):915-920.
|
[15] |
Wang S, Ma Z, Yu W, et al. Migration mechanism of petroleum hydrocarbon pollutants in groundwater system:A case study from groundwater system in Jinan refinery[A].//IEEE.20104th International Conference on Bioinformatics and Biomedical Engineering[C]. 2010:1-4.
|
[16] |
朱辉,叶淑君,吴吉春,等.中国典型有机污染场地土层岩性和污染物特征分析[J]. 地学前缘, 2021,28(5):26-34. Zhu H, Ye S J, Wu J C, et al. Characteristics of soil lithology and pollutants in typical contamination sites in China[J]. Earth Science Frontiers, 2021,28(5):26-34.
|
[17] |
Xu L L, Zhang L Z, Liu B L. Survey and evaluation of heavy metal elements pollution of Changchun suburb land[J]. Advanced Materials Research, 2013,634-638:130-133.
|
[18] |
谭海剑,黄祖照,宋清梅.粤港澳大湾区典型城市污染地块土壤污染特征研究[J]. 环境科学研究, 2021,34(4):976-986. Tan H J, Huang Z Z, Song Q M. Characterization of soil contaminations in brownfield sites in a typical city in Guangdong-Hong Kong-Macao Greater Bay Area[J]. Research of Environmental Sciences, 2021,34(4):976-986.
|
[19] |
马新月,罗帅,王东,等.重庆市场地土壤污染特征分析及行业来源识别[J]. 生态环境学报, 2020,29(4):810-818. Ma X Y, Luo S, Wang D, et al. Analysis of soil pollution characteristics and identification of industry sources in contaminated sites in Chongqing city, China[J]. Ecology and Environmental Sciences, 2020,29(4):810-818.
|
[20] |
Yang Q, Li Z, Lu X, et al. A review of soil heavy metal pollution from industrial and agricultural regions in China:Pollution and risk assessment[J]. Science of the Total Environment, 2018,642(nov.15):690-700.
|
[21] |
Yu G, Chen F, Zhang H, et al. Pollution and health risk assessment of heavy metals in soils of Guizhou, China[J]. Ecosystem Health and Sustainability, 2021,7(1):1859948.
|
[22] |
刘丽丽,邓一荣,林挺,等.粤港澳大湾区典型化工地块地下水分层调查与风险评估[J]. 环境污染与防治, 2021,43(1):67-78. Liu L L, Deng Y R, Li T, et al. Multi-layer sampling and health risk assessment of groundwater for a typical chemical contaminated site in Guangdong-Hong Kong-Macao Greater Nay Area[J]. Environmental Pollution & Control, 2021,43(1):67-78.
|
[23] |
Hayek M, Novak M, Arku G, et al. Mapping industrial legacies:building a comprehensive brownfield database in geographic information systems[J]. Planning Practice & Research, 2010,25(4):461-475.
|
[24] |
席北斗,李娟,汪洋,等.京津冀地区地下水污染防治现状、问题及科技发展对策[J]. 环境科学研究, 2019,32(1):1-9. Xi B D, Li J, Wang Y, et al. Strengthening the innovation capability of groundwater science and technology to support the coordinated development of Beijing-Tianjin-Hebei Region:Status Quo,Problems and Goals[J].Research of Environmental Sciences, 2019,32(1):1-9.
|
[25] |
生态环境部.关于发布《建设用地土壤污染风险管控和修复名录及修复施工相关信息公开工作指南》的公告[EB/OL]. https://www.mee.gov.cn/xxgk2018/xxgk/xxgk01/202112/t20211224_965184.html. Ministry of Ecology and Environment. Announcement on the publication of the "Directory of soil pollution risk control and restoration for construction land and the guidelines for the disclosure of information related to restoration construction"[EB/OL]. https://www.mee.gov.cn/xxgk2018/xxgk/xxgk01/202112/t20211224_965184.html.
|
[26] |
GB/T 4754-2017国民经济行业分类[S]. GB/T 4754-2017 Industrial classification for national economic activities[S].
|
[27] |
HJ 25.1-2019建设用地土壤污染状况调查技术导则[S]. HJ 25.1-2019 Technical guidelines for investigation on soil contamination of land for construction[S].
|
[28] |
Gu Y G.Heavy metal fractionation and ecological risk implications in the intertidal surface sediments of Zhelin Bay, South China[J]. Marine Pollution Bulletin, 2018,129:905-912.
|
[29] |
GB 36600-2018土壤环境质量建设用地土壤污染风险管控标准(试行)[S]. GB 36600-2018 Soil environmental quality-Risk control standard for soil contamination of development land(On Trail)[S].
|
[30] |
EPA U.Regional Screening Level Summary Table[R]. Washington DC:2017.
|
[31] |
GB/T 14848-2017地下水质量标准[S]. GB/T 14848-2017 Standard for groundwater quality[S].
|
[32] |
Dutch Ministry of Housing, Spatial Planning and Environment. Dutch target and intervention values[Z]. Hague,Netherlands, 2000.
|
[33] |
Liu S H,Zeng G M,Niu Q Y,et al.Bioremediation mechanisms of combined pollution of PAHs and heavy metals by bacteria and fungi:A mini review[J]. Bioresource Technology, 2017,224:25-33.
|
[34] |
Wu S H, Zhou S L, Bao H J, et al. Improving risk management by using the spatial interaction relationship of heavy metals and PAHs in urban soil[J]. Journal of Hazardous Materials, 2019,364(FEB.15):108-116.
|
[35] |
Zheng Y, Luo X L, Zhang W, et al. Transport mechanisms of soil-bound mercury in the erosion process during rainfall-runoff events[J]. Environmental Pollution, 2016,215:10-17.
|
[36] |
张小红,王亚娟,陶红,等.宁夏土壤中PAEs污染特征及健康风险评价[J]. 中国环境科学, 2020,40(9):3930-3941. Zhang X H, Wang Y J, Tao H, et al. Study on pollution characteristics and health risk assessment of phthalates in soil of Ningxia[J]. China Environmental Science, 2020,40(9):3930-3941.
|
[37] |
Groffman A R, Crossey L J J C G. Transient redox regimes in a shallow alluvial aquifer[J]. Chemical Geology, 1999,161(4):415-442.
|
[38] |
Du S H,Su X S,Zhang W J. Effective storage rates analysis of groundwater reservoir with surplus local and transferred water used in Shijiazhuang City, China[J]. Water and Environment Journal, 2012, 27(2):157-169.
|
[39] |
Jiang M H, Sun G Y. Study on the dynamic trajectory of industrial gravity center of the leading industry of the Yangtze River Delta from 1999~2012[C]//IEEE. International Conference on Management Science & Engineering, 2014:695-701.
|
[40] |
林广宇.地下水位变动带石油烃污染物的迁移转化规律研究[D]. 长春:吉林大学, 2014. Lin G Y. Study on migration and transformation of petroleum hydrocarbons in zone of intermittent saturation[D]. Changchun:Jilin University, 2014.
|
[41] |
刘长礼,庞雅婕,王翠玲,等.黏性土对垃圾渗滤液中多环芳烃吸附机理与规律[J]. 地质论评, 2018,64(4):905-912. Liu C L, Pang Y J, Wang C L, et al. Research on the mechanisms and disciplines of clayed soils adsorb PAHs in landfill leachate[J]. Geological Review, 2018,64(4):905-912.
|
|
|
|