基于多模型和多源数据的京津冀地区BVOCs排放清单

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Abstract In order to systematically study the spatial and temporal distributions of biogenic volatile organic compounds (BVOCs) emissions in the Beijing-Tianjin-Hebei (BTH) region, this paper calculated county-level emissions of BVOCs and major components in the BTH region in 2018 based on three methods, including the stock production, land use remote sensing interpretation data, and MEGAN model. The results based on the three methods showed that the total BVOCs emissions in the BTH region were 741400t, 844800t, and 777300t, respectively. The emissions in Beijing, Tianjin, and Hebei were 118000t, 32000t and 637000t, the emissions of isoprene, monoterpenes, and others were 291900t, 225800t, and 274100t, and the emissions of forest land, cropland and grassland accounted for 68.42%, 23.07% and 3.89%, respectively. From the perspective of temporal distributions, BVOCs emissions were characterized by a single peak. Summer showed the highest emissions of 526400t, accounting for 66.64% of the whole year, while winter showed the lowest emissions of 15900t, accounting for 2.01% of the whole year. From the perspective of spatial distributions, BVOCs emissions based on different methods presented similar spatial distribution characteristics of high emissions in north and low emissions in south. The emissions along Taihang Mountains and Yanshan Mountains were dominated by forest land and grassland, while those in the southeastern Hebei Plain was dominated by farmland. From the perspective of methods, the emissions obtained with the light-temperature model based on remote sensing interpretation were relatively high, and the proportion of other BVOCs obtained with the dynamic model was relatively high. This study provides data support for the comprehensive understanding of BVOCs emission characteristics and the planning of continuous air quality improvement strategies in the BTH region.

Key words： BVOCs spatiotemporal distribution storage capacity leaf area index MEGAN model

Received: 06 March 2023

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X51

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	LI Ao-zhe
	DUAN Wen-jiao
	QI Hao-yun
	CAI Bin

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LI Ao-zhe,DUAN Wen-jiao,QI Hao-yun等. BVOCs emission inventory in the Beijing-Tianjin-Hebei region based on multiple models and data sources[J]. CHINA ENVIRONMENTAL SCIENCECE, 2023, 43(10): 5052-5061.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2023/V43/I10/5052

[1]	孙银川,严晓瑜,缑晓辉,等.中国典型城市O3与前体物变化特征及相关性研究[J]. 环境科学研究, 2020,33(1):44-53. Sun Y C, Yan X Y, Gou X H. Characteristics and correlation of ozone and its precursors in typical cities in China[J]. Research of Environmental Sciences, 2020,33(1):44-53.
[2]	姜华,常宏咪.我国臭氧污染形势分析及成因初探[J]. 环境科学研究, 2021,34(7):1576-1582. Jiang H, Chang H M. Analysis of China's ozone pollution situation, preliminary investigation of causes and prevention and control recommendations[J]. Research of Environmental Sciences, 2021, 34(7):1576-1582.
[3]	成翔,赵继峰,肖洋,等.工业聚集区大气VOCs组成特征及对臭氧生成的影响[J]. 环境工程技术学报, 2020,10(5):823-830. Cheng X, Zhao J F, Xiao Y, et al. Composition characteristics of atmospheric VOCs and the influence on ozone formation in an industrial cluster area[J]. Journal of Environmental Engineering Technology, 2020,10(5):823-830.
[4]	李琦,等.西安人为源VOCs排放特征及其对O3和SOA生成潜势的影响[J]. 环境科学研究, 2019,32(2):253-262. Li Q, et al. Emission characteristics of anthropogenic VOCs in Xi'an City and its contribution to ozone formation potential and secondary organic aerosols formation potential[J]. Research of Environmental Sciences, 2019,32(2):253-262.
[5]	张蔷,等.北京森林BVOCs排放特征及对区域空气质量的影响[J]. 中国环境科学, 2021,41(2):622-632. Zhang Q, et al. Emission characteristics of VOCs from forests and its impact on regional air quality in Beijing[J]. China Environmental Science, 2021,41(2):622-632.
[6]	Guenther A, et al. A global model of natural volatile organic compound emissions[J]. Journal of Geophysical Research:Atmospheres, 1995,100(D5):8873-8892.
[7]	Evans R C, et al. Estimates of isoprene and monoterpene emission rates in plants[R]. Botanical gazette, 1982,143(3):304-310.
[8]	Anastasi C, Hopkinson L, Simpson V J. Natural hydrocarbon emissions in the United Kingdom[J]. Atmospheric Environment. 1991,25(7):1403-1408.
[9]	谢军飞,李延明.植物源挥发性有机化合物排放清单的研究进展[J]. 环境科学, 2013,34(12):4779-4786. Xie J F, Li Y M. Research advances on volatile organic compounds emission inventory of plants[J]. Environmental Science, 2013, 34(12):4779-4786.
[10]	谭峥铮,卢召艳,石广明,等.湖南省天然源挥发性有机物排放时空特征研究[J]. 环境科学学报, 2021,41(5):1774-1783. Tan Z Z, Lu Z Y, Shi G M, et al. The characteristics of biogenic volatile organic compounds of Hunan Province[J]. Acta Scientiae Circumstantiae. 2021,41(5):1774-1783.
[11]	陆成伟,等.基于动态模型的四川盆地植物挥发性有机物排放[J]. 环境化学, 2018,37(4):836-842. Lu C W, et al. Emission of biogenic volatile organic compounds in Sichuan Basin using a dynamic model[J]. Environ Chem, 2018, 37(4):836-842.
[12]	亓浩雲,等.2000~2020年京津冀BVOCs排放量估算及时空分布特征[J]. 中国环境科学, 2022,42(4):1501-1509. Qi H Y, et al. Estimation of BVOCs emissions from Beijing, Tianjin and Hebei from 2000 to 2020 and its temporal and spatial distribution characteristics[J]. China Environmental Science, 2022,42(4):1501-1509.
[13]	Wang H, et al. A long-term estimation of biogenic volatile organic compound (BVOC) emission in China from 2001-2016:the roles of land cover change and climate variability[J]. Atmospheric chemistry and physics, 2021,21(6):4825-4848.
[14]	高超,等.中国生物源挥发性有机物(BVOCs)时空排放特征研究[J]. 环境科学学报, 2019,39(12):4140-4151. Gao C, et al. Spatiotemporal distribution of biogenic volatile organic compounds emissions in China[J]. Acta Scientiae Circumstantiae, 2019,39(12):4140-4151.
[15]	Guenther A P. Zimmerman and M. Wildermuth. Natural volatile organic compound emission rate estimates for U.S. woodland landscapes[J]. Atmospheric Environment, 1994,28(6):1197-1210.
[16]	Guenther A, et al. A global model of natural volatile organic compound emissions[J]. Journal of Geophysical Research, 1995, 100(D5):8873.
[17]	Steinbrecher R, et al. Intra-and inter-annual variability of VOC emissions from natural and semi-natural vegetation in Europe and neighbouring countries[J]. Atmospheric Environment, 2009,43(7):1380-1391.
[18]	赵静,白郁华,王志辉,等.我国植物VOCs排放速率的研究[J]. 中国环境科学, 2004,(6):15-18. Zhao J, Bai Y H, Wang Z H, Zhang S Y. Studies on the emission rates of plants VOCs in China[J]. China Environmental Science, 2004, (6):15-18.
[19]	Jing X, et al. Emission patterns of biogenic volatile organic compounds from dominant forest species in Beijing, China[J]. Journal of Environmental Sciences, 2020,95(9):73-81.
[20]	Klinger L F, et al. Assessment of volatile organic compound emissions from ecosystems of China[J]. Journal of Geophysical Research:Atmospheres, 2002,107(D21):ACH-1-ACH 16-21.
[21]	樊冲.河北省森林植物源挥发性有机物排放量研究[D]. 北京:北京林业大学, 2019. Fan C. Study on biogenic volatile organic compounds emission from forest plants in Hebei Province[D]. Beijing Forestry University, 2019.
[22]	Simpson D, et al. Inventorying emissions from nature in Europe[J]. Journal of Geophysical Research:Atmospheres, 1999,104(D7):8113-8152.
[23]	Geron C D, Guenther A B, Pierce T E. An improved model for estimating emissions of volatile organic compounds from forests in the eastern United States[J]. Journal of Geophysical Research, 1994, 99(D6):12773-12791.
[24]	陈颖,李德文,史奕,等.沈阳地区典型绿化树种生物源挥发性有机物的排放速率[J]. 东北林业大学学报, 2009,37(3):47-49. Chen Y, Li D W, Shi Y, He X Y. Emission rate of biogenic volatile organic compounds from urban trees in Shenyang, China[J]. Journal of Northeast Forestry University, 2009,37(3):47-49.
[25]	张钢锋,谢绍东.基于树种蓄积量的中国森林VOC排放估算[J]. 环境科学, 2009,30(10):2816-2822. Zhang G F, Xie S D. Estimation of VOC emission from forests in China based on the volume of tree species[J]. Environmental Science, 2009,30(10):2816-2822.
[26]	Simon V, et al. The biogenic volatile organic compounds emission inventory in France[J]. Science of The Total Environment, 2006, 372(1):164-182.
[27]	Goldstein A H, et al. Seasonal course of isoprene emissions from a midlatitude deciduous forest[J]. Journal of Geophysical Research:Atmospheres, 1998,103(D23):31045-31056.
[28]	张福春.中国农业物候图集[M]. 1987. Zhang F C. Chinese agricultural phenology atlas[M]. Beijing:Science Press, 1987.
[29]	中国科学院国家计划委员会地理研究所.中国动植物侯观测年报:1987~1988年.第11号[M]. 中国科学技术出版社, 1992. Institute of Geograph. Annual report of animal and plant phenology in China:serial reports with number from 11, 1987~1988[M]. Beijing:Science Press, 1992.
[30]	国家林业和草原局.中国森林资源报告·2014·2018[M]. 中国林业出版社, 2019. State Administration of Forestry and Grassland. China Forest Resources Report·2014·2018[M]. China Forestry Publishing House, 2019.
[31]	方精云,陈安平.中国森林植被碳库的动态变化及其意义[J]. 植物学报, 2001,(9):967-973. Fang J Y, Chen A P. Dynamic forest biomass carbon pools in China and their significance[J]. Journal of Integrative Plant Biology, 2001, (9):967-973.
[32]	方精云,郭兆迪,朴世龙,等.1981~2000年中国陆地植被碳汇的估算[J]. 中国科学(D辑:地球科学), 2007,(6):804-812. Fang J Y, Guo Z D, Piao S L. Estimation of terrestrial vegetation carbon sinks in China from 1981 to 2000. Scientia Sinica:Terrae, 2007,(6):804-812.
[33]	王亚静,王红彦,高春雨,等,毕于运.稻麦玉米秸秆残留还田量定量估算方法及应用[J]. 农业工程学报, 2015,31(13):244-250. Wang Y J, Wang H Y, Gao C Y, Wang L, Bi Y Y. Quantitative estimation method and its application to rice, wheat and corn straw residues left in field[J]. Transactions of the Chinese Society of Agricultural Engineering, 2015,31(13):244-250.
[34]	刘岩,李莉,安静宇,等.长江三角洲2014年天然源BVOCs排放、组成及时空分布[J]. 环境科学, 2018,39(2):608-617. Liu Y, Li L, An J Y, et al. Emissions, chemical composition, and spatial and temporal allocation of the BVOCs in the Yangtze River Delta Region in 2014[J]. Environmental Science, 2018,39(2):608-617.
[35]	Myneni R, Knyazikhin Y, Park T. MYD15A2H MODIS/Aqua Leaf Area Index/FPAR 8-Day L4Global 500m SIN Grid V006[Data set]. NASA EOSDIS Land Processes DAAC, 2022-09-06.
[36]	Friedl M, Sulla-Menashe D. MCD12Q1MODIS/Terra+Aqua Land Cover Type Yearly L3Global 500m SIN Grid V006[Data set]. NASA EOSDIS Land Processes DAAC, 2022-09-06.
[37]	Loreto F, Sharkey T D. On the relationship between isoprene emission and photosynthetic metabolites under different environmental conditions[J]. Planta, 1993,189(3):420-424.
[38]	蔡斌,程昊淼,亓浩雲,等.京津冀夏季不同类型植被对典型城市O3和PM2.5贡献研究[J/OL]. 中国环境科学, 2023,43(6):2734-2743. Cai B, Cheng H M, Qi H Y, et al. Contribution of different types of vegetation to O3 and PM2.5 in typical cities in Beijing-Tianjin-Hebei Region in Summer[J]. China Environmental Science, 2023,43(6):2734-2743.
[39]	Li J, Li L Y, et al. Inventory of highly resolved temporal and spatial volatile organic compounds emission in China[C]//International Conference on Modelling, Monitoring and Management of Air Pollution, 2016.
[40]	张蔷,等.北京森林BVOCs排放现状及动态变化特征分析[J/OL]. 中国环境科学, 2022,42(9):3991-4000. Zhang Q, et al. The current status and characteristics of variations in forest BVOCs emissions in Beijing[J/OL]. China Environmental Science, 2022,42(9):3991-4000.
[41]	井潇溪.北京市森林植物挥发性有机物排放研究[D]. 北京:北京林业大学, 2020. Jing X X. Study on biogenic volatile organic compounds emission from forest plants in Beijing[D]. Beijing Forestry University, 2020.
[42]	袁相洋,许燕,杜英东,等.南京和北京城市天然源挥发性有机物排放差异[J]. 中国环境科学, 2022,42(4):1489-1500. Yuan X Y, Xu Y, Du Y D, Feng Z Z. Differences of biogenic volatile organic compound emissions from urban forests in Nanjing and Beijing[J]. China Environmental Science, 2022,42(4):1489-1500.
[43]	夏春林,肖琳.京津冀天然源挥发性有机物排放研究[J]. 环境科学学报, 2019,39(8):2680-2689. Xia C L, Xiao L. Estimation of biogenic volatile organic compounds emissions in Jing-Jin-Ji[J]. Acta Scientiae Circumstantiae, 2019, 39(8):2680-2689.
[44]	高翔,刘茂辉,徐媛,等.天津市植被排放挥发性有机物估算及时空分布[J]. 西部林业科学, 2016,45(6):108-114. Gao X, Liu M H, Xu Y, et al. Biogenic VOCs Emission in Tianjin City and Its Temporal and Spatial Distribution[J]. Journal of West China Forestry Science, 2016,45(6):108-114.