选择性催化氧化H<sub>2</sub>S的富氮碳催化剂研究进展

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Abstract In recent years, selective catalytic oxidation (H₂S-SCO) technology, which can efficiently purify H₂S and recover sulfur resources, has received much attention. Research on the development of high-performance, high-selective, and low-cost catalysts is the focus of H₂S-SCO technology, among which the nitrogen-rich carbon-based catalysts (RNCCs), which have the advantages of high activity, metal-free, easy-to-prepare, low cost, and easy to be regenerated, are considered as a class of highly promising catalysts for H₂S-SCO. In this article, the development of metal-based catalysts is introduced, the preparation method, catalytic activity, and physical-chemical properties of RNCC are summarized and generalized, the structure-efficacy relationship of RNCC and the key factors affecting the performance of RNCC are systematically discussed, and the H₂S-SCO reaction mechanism of RNCC is concluded. Finally, the current opportunities and challenges of RNCC are also pointed out, and the future development direction is envisioned.

Key words： nitrogen-rich carbon catalyst H₂S selective catalytic oxidation

Received: 22 September 2023

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X512

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	YANG Jin-tao
	YANG Xue-jin
	NING Ping
	WANG Fang
	SONG Xiao-shuang
	JIA Li-juan
	FENG Jia-yu

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YANG Jin-tao,YANG Xue-jin,NING Ping等. Advances in nitrogen-rich carbon catalysts for selective catalytic oxidation of H₂S[J]. CHINA ENVIRONMENTAL SCIENCECE, 2024, 44(4): 1981-1994.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2024/V44/I4/1981

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