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Aerosol transmission characteristics of spring in Wutai mountain |
YAN Shi-ming1, WANG Yan1, ZHANG Yue-jun1, GAO Xing-ai1, WANG Shu-min1, DONG Jian2, LIU Zheng-dong2 |
1. Shanxi Institute of Meteorological Sciences, Taiyuan 030002, China;
2. Wutai Mountain Meteorological Station, Xinzhou 035515, China |
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Abstract Statistical characteristics of spring aerosol particle concentration and mass concentration over the Wutai mountain in Shanxi province based upon the particle concentration and mass concentration data observed by Grimm180 aerosol instrument over the Wutai mountain in Shanxi province. The Global Data Assimilation System (GDAS) data provided by the National Environmental Prediction Center (NCEP) from March to May 2018, cluster analysis and potential source contribution factor analysis (PSCF) were also utilized to reveal the main transmission path affecting the aerosol concentration variation, as well as the potential contribution source area. There were mainly 6 types of transmission routes affecting the aerosol concentration over the Wutai mountain in spring, of which the first, fourth, second and fifth were northwestern and westward, accounting for 62.5% of the total trajectory; while the third and sixth type were in the southern and eastern directions, accounting for 24.7% of the total trajectory. The statistical analysis of different transmission paths showed that the first and fourth types had the greatest influence on the concentration of PN10, PN>10 and PM10, whose potential contribution source areas were mainly located in western Inner Mongolia and the Loess Plateau in northern Shaanxi Province, in which the PSCF values reached 0.6 or more; whereas the sixth and third type of routes had a larger impact on the PN0.5, PN1.0, and PM1.0 concentration, of which the potential contribution source areas were mainly within the south-central and central Shaanxi Province, Beijing-Tianjin-Hebei region and northern Henan Province, in which the PSCF values were above 0.8. The high-value zone of fine particle PSCF was mainly located in the eastern and southern region around the Wutai mountain with the transmission height lowering than 2km. As the particle size increased, the high-value zone of PSCF became the northwestern and southeastern region, and the transmission height was within 2~4km of the free troposphere, through which the proportion of transportation at northwestern region increased gradually, and the high-value zone got farther and farther away from Wutai mountain station.
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Received: 19 July 2019
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[1] |
Seinfeld J H, Pandis S N. Atmospheric chemistry and physics:From air pollution to climate change, atmospheric chemistry and physics[M]. John Wiley & Sons, New York, 1998:1326.
|
[2] |
Hussein T, Maso M D, Petäjä T, et al. Evaluation of an automatic algorithm for fitting the particle number size distributions[J]. Boreal Environment Research, 2005,10(5):33-355.
|
[3] |
Kulmala M H, Vehkam K, Pet T J, et al. Formation and growth rates of ultrafine atmospheric particles:a review if observations[J]. Journal of Aerosol Science, 2004,35(2):143-176.
|
[4] |
Huebert B J. An overview of ACE-Asia:strategies for quantifying the relationships between Asian aerosols and their climatic impacts[J]. Journal of Geophysical Research, 2003,108(D23):8633.
|
[5] |
沈小静.泰山大气气溶胶数谱分布特征及光学特性研究[D]. 北京:中国气象科学院研究生院, 2012. Shen X J. Characteristics of particle number size distribution and optical properties at Mt. Tai[D]. Beijing:Chinese Academy of Meteorological Sciences, 2012.
|
[6] |
Gao X, Cao X, Tian P, et al. Combined observation of a dust storm over the Loess Plateau using a dual-wavelength lidar and an aethalometer[J]. Atmospheric Pollution Research, 2017,8:1103-1112.
|
[7] |
郑山,刘兴荣,程宁,等.空气污染与恶性肿瘤住院人数的关联性分析[J]. 环境与职业医学, 2016,33(6):601-605. Zheng S, Liu X G, Cheng N, et al. Association between air pollution and hospitalization due to malignantneoplasms[J]. Journal of Environmental & Occupational Medicine, 2016,33(6):601-605.
|
[8] |
苏捷,赵普生,陈一娜.北京地区不同天气条件下气溶胶数浓度粒径分布特征研究[J]. 环境科学, 2016,37(4):1208-1218. Su J, Zhao P S, Chen Y N. Characteristics of Number Concentration Size Distributions of Aerosols Under Different Weather Processes in Beijing[J]. Environmental Science, 2016,37(4):1208-1218.
|
[9] |
刘慧,夏敦胜,陈红,等.2017年兰州市大气污染物输送来源及传输特征模拟分析[J]. 环境科学研究, 2019,32(6):993-1000. Liu H, Xia D S, Chen H, et al. Simulation Analysis of Sources and Transmission Characteristics of Air Pollutants in Lanzhou City in 2017[J]. Research of Environmental Sciences, 2019,32(6):993-1000.
|
[10] |
李正,张昊,叶辉,等.杭州市典型雾霾期污染特征及污染源的HYSPLIT模型分析[J]. 环境科学学报, 2018,38(5):1717-1726. Li Z, Zhang H, Ye H, et al. Characteristics of air pollution during typical haze periods and HYSPLIT model analysis of its source in Hangzhou[J]. Acta Scientiae Circumstantiae, 2018,38(5):1717-1726.
|
[11] |
蒋永成,蒋宗孝,童怀忠,等.厦门市颗粒物输送路径和源区季节特征分析[J]. 环境科学与技术, 2018,41(10):184-191. Jiang Y C, Jiang Z X, Tong H Z, et al. Seasonal characteristics of transport paths and source areas of particulate matter in Xiamen[J]. Environmental Science & Technology, 2018,41(10):184-191.
|
[12] |
李颜君,安兴琴,范广洲.北京地区大气颗粒物输送路径及潜在源分析[J]. 中国环境科学, 2019,39(3):915-927. Li Y J, An X Q, Fan G Z. Transport pathway and potential source area of atmospheric particulates in Beijing[J]. China Environmental Science, 2019,39(3):915-927.
|
[13] |
闫世明,王雁,郭伟,等.太原市秋冬季大气污染特征和输送路径及潜在源区分析[J]. 环境科学, 2019,40(11):4801-4809. Yan S M, Wang Y, Guo W, et al. Characteristics, transportation, pathways, and potential sources of air pollution during autumn and winter in Taiyuan[J]. Environmental Science, 2019,40(11):4801-4809.
|
[14] |
沈利娟,王红磊,银燕,等.泰山顶(1534m)夏季气溶胶粒径分布特征[J]. 环境科学, 2019,40(5):2019-2026. Shen L J, Wang H L, Ying Y, et al. Size distributions of aerosols during the summer at the summit of mountain taishan(1534m) in central East China[J]. Environmental Science, 2019,40(5):2019-2026.
|
[15] |
戴文婷,李建军,成春雷,等.中国中东部高山和城市夏季大气气溶胶浓度及粒径分析[J]. 地球环境学报, 2011,2(1):263-271. Dai W T, Li J J, Cheng C L, et al. Concentrations and size distributions of summertime atmospheric aerosols at urban and alpine sites in east and central China[J]. Journal of Earth Environment, 2011,2(1):263-271.
|
[16] |
Wang G, Li J, Cheng C, et al. Observation of atmospheric aerosols at Mt. Hua and Mt. Tai in central and east China during spring 2009-Part1:EC, OC and inorganic ions[J]. Atmospheric Chemistry and Physics, 2011,11:4221-4235.
|
[17] |
银燕,陈晨,陈魁,等.黄山大气气溶胶微观特性的观测研究[J]. 大气科学学报, 2010,33(3):129-136. Yin Y, Chen C, Chen K, et al. An Observational study of the microphysical properties of atmospheric serosol at Mt. Huang[J]. Transactions of Atmospheric Sciences, 2010,33(3):129-136.
|
[18] |
张磊,金莲姬,朱彬,等. 2011年6~8月平流输送对黄山顶污染物浓度的影响[J]. 中国环境科学, 2013,33(6):969-978. Zhang L, Jin L J, Zhu B, et al. The influence of advective transport on the concentrations of pollutants at the top of mountain Huangshan from June to August, 2011[J]. China Environmental Science, 2013, 33(6):969-978.
|
[19] |
王爱平,朱彬,银燕,等.黄山顶夏季气溶胶数浓度特征及其输送潜在源区[J]. 中国环境科学, 2014,34(4):852-861. Wang A P, Zhu B, Yin Y, et al. Aerosol number concentration properties and potential sources areas transporting to the top of mountain Huangshan in summer[J]. China Environmental Science, 2014,34(4):852-861.
|
[20] |
张小培.黄山顶大气气溶胶粒子来源和输送过程的数值模拟[D]. 南京:南京信息工程大学, 2012. Zhang X P. Numerical simulation of Source & Transport of Aerosol Particles at Mountain Huang[D]. Nanjing:Nanjing University of Information Science & Technology, 2012.
|
[21] |
Jiang H, Yin Y, Yang L H, et al. The characteristics of atmospheric ice nuclei measured at different altitudes in the Huangshan Mountains in Southeast China[J]. Advances in Atmospheric Sciences, 2014,31(2):396-406.
|
[22] |
占明锦,孙俊英,张养梅,等.气团来源对瓦里关地区颗粒物数谱分布的影响[J]. 冰川冻土, 2009,31(4):77-81. Zhan M J, Sun J Y, Zhang Y M, et al. The influence of air mass sources on the particle number concentration and the size distribution at Mt. Waliguan[J]. Journal of Glaciology and Geocryology, 2009, 31(4):77-81.
|
[23] |
Kivekäs N, Sun J, Zhan M, et al. Long term particle size distribution measurements at Mount Waliguan, a high-altitude site in inland China[J]. Atmospheric Chemistry and Physics, 2009,9(15):5461-5474.
|
[24] |
杨毅红,陶俊,朱李华,等.中国西部背景地PM2.5化学组分特征及其对大气散射系数的影响[J]. 环境科学学报, 2017,37(4):1216-1226. Yang Y H, Tao J, Zhu L H, et al.Characterization of chemical compositions of PM2.5 and its impact on scattering coefficients at a background site over Western China[J]. Acta Scientiae Circumstantiae, 2017,37(4):1216-1226.
|
[25] |
Kaiser A, Scheifinger H, Spangl W, et al. Transport of nitrogen oxides, carbon monoxide and ozone to the Alpine Global Atmosphere Watch stations Jungfraujoch (Switzerland), Zugspitze and Hohenpeissenberg (Germany), Sonnblick (Austria) and Mt. Krvavec (Slovenia)[J]. Atmospheric Envirment, 2007,41(40):9273-9287.
|
[26] |
Cui J, Pandey Deolal S, Sprenger M, et al. Free tropospheric ozone changes over Europe as observed at Jungfraujoch (1990-2008):an analysis based on backward trajectories[J]. Journal of Geophysical Research, 2011,116(D10).
|
[27] |
Pratt K A, Prather K A. Aircraft measurements of vertical profiles of aerosol mixing states[J]. Journal of Geophysical Research, 2010, 115(D11).
|
[28] |
Li W J, Zhang D, Shao L, et al. Individual particle analysis of aerosols collected under haze and non-haze conditions at a high-elevation mountain site in the North China plain[J]. Atmospheric Chemistry and Physics, 2011,11(22):11733-11744.
|
[29] |
Draxler R R. Description of the HYSPLIT4 modelling system[R]. NOAA Technical Memorandum, 1997:24.
|
[30] |
Pu W, Shi X, Wang L, et al. Potential source regions of air pollutants at a regional background station in Northern China[J]. Environmental Technology, 2019,40(26):3412-3421.
|
[31] |
Zhang G, Xu H, Qi B, et al. Characterization of atmospheric trace gases and particulate matter in Hangzhou, China[J]. Atmospheric Chemistry and Physics, 2018,18(3):1705-1728.
|
[32] |
翟华,朱彬,赵雪婷,等.长江三角洲初冬一次重污染天气成因分析[J]. 中国环境科学, 2018,38(11):3-11. Zhai H, Zhu B, Zhao X T, et al. Analysis of a heavy air pollution event in early winter in the Yangtze River Delta[J]. China Environmental Science, 2018,38(11):3-11.
|
[33] |
Perrone M G, Vratolis S, Georgieva E, et al. Sources and geographic origin of particulate matter in urban areas of the Danube macro-region:The cases of Zagreb (Croatia), Budapest (Hungary) and Sofia (Bulgaria)[J]. Science of The Total Environment, 2018,619-620:1515-1529.
|
[34] |
Cheng M D, Hopke P K, Barrie L, et al. Qualitative determination of source regions of aerosol in Canadian high Arctic[J]. Environmental Science and Technology, 1993,27(10):2063-2071.
|
[35] |
Polissar A V, Hopke P K, Paatero P, et al. The aerosol at Barrow, Alaska:long-term trends and source locations[J]. Atmospheric Environment, 1999,33(16):2441-2458.
|
[36] |
Cheng I, Xu X, Zhang L. Overview of receptor-based source apportionment studies for speciated atmospheric mercury[J]. Atmospheric Chemistry and Physics, 2015,15(14):7877-7895.
|
[37] |
Wang H, Zhang L, Cao X, et al. A-Train satellite measurements of dust aerosol distributions over Northern China[J]. Journal of Quantitative Spectroscopy and Radiative Transfer, 2013,122:170-179.
|
[38] |
Yu J Y, Wang Y W, Chang C W. Asian dust storm activity and its association with atmospheric circulation from 1995 to 2006[J]. Terrestrial Atmospheric and Oceanic Sciences, 2010,21(2):375-391.
|
[39] |
Tian P, Cao X, Zhang L, et al. Aerosol vertical distribution and optical properties over China from long-term satellite and ground-based remote sensing[J]. Atmospheric Chemistry and Physics, 2017,17:2509-2523.
|
[40] |
李瑞芃.青岛大气颗粒物数浓度分布及特殊天气过程中变化特征研究[D]. 青岛:中国海洋大学, 2012. Li R P. Distribution of atmospheric particle number concentration in Qingdao and variations in different weather conditions[D]. Qingdao:Ocean University of China, 2012.
|
[41] |
郭家瑜,张英杰,郑海涛,等.北京2015年大气细颗粒物的空间分布特征及变化规律[J]. 环境科学学报, 2017,37(7):2409-2419. Guo J Y, Zhang Y J, Zheng H T, et al. Characteristics of spatial distribution and variations of atmospheric fine particles in Beijing in 2015[J]. Acta Scientiae Circumstantiae, 2017,37(7):2409-2419.
|
[42] |
Zhang Y L, Cao F. Fine particulate matter (PM2.5) in China at a city level[J]. Scientific Reports, 2015,5:14884.
|
|
|
|