|
|
The characteristics of PM2.5 and its water soluble ions during Spring Festival in PRD in 2012 |
MA Ying1, WU Dui1,2,3, LIU jian2 |
1. Institute of Atmospheric Environmental Safety and Pollution Control, Jinan University, Guangzhou 510632, China; 2. School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China; 3. Guangzhou Institute of Tropical and Marine Meteorology, China Meteorology Administration, Guangzhou 510080, China |
|
|
Abstract Particulate matter (PM) and relevant water-soluble ions were analyzed based on the hourly Marga data from China Meteorological Agency Panyu Atmospheric Components Station during Spring Festival of 2012 in PRD.During fireworks burning period, mass concentrations of PM10, PM2.5 and all water-soluble ions increased rapidly, indicating an occurrence of air pollution. The ratio of PM2.5 to PM10 (PM2.5/PM10) showed a decreasing trend,and thus the increase in PM10 caused by the pollution was more significant than that of PM2.5; however, the average value of PM2.5/PM10 is 0.92, indicating PM2.5 was the absolutely dominant component of PM. The influence of fireworks burning on the concentration of K+, Cl- and SO42- was more significant than on that of NO3- and NH4+. The correlation analysis suggested that the increase of K+, Cl-, Mg2+ and Na+ resulted from the firework burning and SO42-, NO3-和NH4+ was probably from the same source. Finally, firework burning has also contributed to the increase of black carbon.
|
Received: 29 February 2016
|
|
|
|
|
[1] |
罗云峰,周秀骥,李维亮.大气气溶胶辐射强迫及气候效应的研究现状 [J]. 地球科学进展, 1998,13(6):572-581.
|
[2] |
吴兑,毕雪岩,邓雪娇,等.珠江三角洲大气灰霾导致能见度下降问题研究 [J]. 气象学报, 2006,64(4):510-517.
|
[3] |
吴兑,吴晟,李菲,等.粗粒子气溶胶远距离输送造成华南严重空气污染的分析 [J]. 中国环境科学, 2011,31(4):540-545.
|
[4] |
吴兑,邓雪娇,毕雪岩,等.细粒子污染形成灰霾天气导致广州地区能见度下降 [J]. 热带气象学报, 2007,23(1):1-6.
|
[5] |
吴兑,吴晟,李海燕,等.穗港晴沙两重天-2010年3月17-23日珠三角典型灰霾过程分析 [J]. 环境科学学报, 2011,31(4):695-703.
|
[6] |
吴兑,刘啟汉,梁延刚,等.粤港细粒子(PM2.5)污染导致能见度下降与灰霾天气形成的研究 [J]. 环境科学学报, 2012,32(11): 2660-2669.
|
[7] |
廖碧婷,吴兑,陈静,等.华南地区大气气溶胶中EC和水溶性离子粒径分布特征 [J]. 中国环境科学, 2015,35(5):1297-1309.
|
[8] |
王明星,张仁健.大气气溶胶研究的前沿问题 [J]. 气候与环境研究, 2001,1(6):119-123.
|
[9] |
吴兑.南海北部大气气溶胶水溶性成分谱分布特征 [J]. 大气科学, 1995,19(5):616-622.
|
[10] |
Wu Dui, Tie Xuexi, Deng Xuejiao, Chemical characterizations of soluble aerosols in Southern China [J]. Chemosphere, 2006,64(5): 749-757.
|
[11] |
吴兑,常业谛,毛节泰,等.华南地区大气气溶胶质量谱与水溶性成分谱分布的初步研究 [J]. 热带气象学报, 1994,10(1):85-96.
|
[12] |
吴兑,陈位超.广州气溶胶质量谱与水溶性成分谱的年变化特征 [J]. 气象学报, 1994,52(4):499-505.
|
[13] |
吴兑,黄浩辉,邓雪娇.广州黄埔工业区近地层气溶胶分级水溶性成分的物理化学特征 [J]. 气象学报, 2001,59(2):213-219.
|
[14] |
吴兑,邓雪娇,叶燕翔,等.岭南山地气溶胶物理化学特征研究 [J]. 高原气象, 2006,25(5):877-885.
|
[15] |
廖碧婷,吴兑.常越,广州地区SO42-,NO3-,NH4+与相关气体污染特征研究 [J]. 环境科学学报, 2014,34(6):1551-1559.
|
[16] |
李淑贤,邱洪斌,王新明,等.广州秋季灰霾和正常天气PM2.5中水溶性离子特征 [J]. 分子科学学报, 2011,27(3):166-169.
|
[17] |
刘建,吴兑,范绍佳,等.广州地区灰霾与清洁过程的污染特征研究 [J]. 环境科学学报, 2015,35(11):3433-3442.
|
[18] |
Watson J G. Visibility: Science and regulation [J]. Journal of the Air & Waste Management Association, 2002,52(6):628-713.
|
[19] |
沈建东,焦荔,何曦,等,杭州城区春节PM2.5中水溶性离子在线观测 [J]. 中国环境监测, 2014,30(2):151-157.
|
[20] |
赵金平,徐亚,张福旺,等.泉州郊区春节燃放烟花时段大气污染特征 [J]. 环境科学, 2011,32(5):1224-1230.
|
[21] |
李利平,张宁,王振,等.春节燃放爆竹对大气气溶胶水溶性无机离子的影响 [J]. 城市环境与城市生态, 2008,21(5):37-41.
|
[22] |
秦玮,葛顺,张祥志,等.烟花燃放对空气中PM2.5及水溶性离子的影响研究 [J]. 环境监控与预警, 2013,5(3):1-4.
|
[23] |
邹强,姚玉刚,丁铭,等.春节烟花爆竹燃放期间苏州市区PM2.5中水溶性离子特征分析 [J]. 环境监测管理与技术, 2014,26(2):26-29.
|
[24] |
王占山,张大伟,李云婷,等.2014年春节期间北京市空气质量分析 [J]. 环境科学学报, 2015,35(2):371-378.
|
[25] |
赵伟,范绍佳,谢文彰,等.烟花燃放对珠三角地区春节期间空气质量的影响 [J]. 环境科学, 2015,36(12):4365.
|
[26] |
吴兑,毛节泰,邓雪娇,等.,珠江三角洲黑碳气溶胶及其辐射特征的观测 [J]. 中国科学D辑, 2009,39(11):1542-1553.
|
[27] |
秦瑜,赵春生.大气化学基础 [M]. 北京:气象出社, 2003.
|
[28] |
Raveendran K, Ganesh A, Khilar K C. Influence of mineral matter on biomass pyrolysis characteristics [J]. Fuel, 1995,74(12):1812-1822.
|
[29] |
刘臻.青岛大气气溶胶水溶性无机离子分布特征研究 [D]. 青岛:中国海洋大学, 2012.
|
[30] |
张小玲,徐敬,李腊平,等.不同气象条件下烟花爆竹燃放对空气质量的影响研究 [J]. 气象与环境学报, 2008,24(4):6-12.
|
[30] |
Helmenstin A M. The Chemistry of Firecracker Colors [EB/OL]. 2005. http:// chemistry.about.com/library/weekly/aa0.
|
|
|
|