|
|
A study of 210Po in atmospheric aerosol of Shenzhen and its committed effective dose |
SU Ling-ling1, LIU Guo-qing1, DING Min-xia1,2, FENG Jiang-ping2, ZHANG Hong1 |
1. Institute of applied nuclear technology, College of physics and energy, Shenzhen University, Shenzhen 518060, China;
2. Shenzhen Environmental Monitoring Center, Shenzhen 518049, China |
|
|
Abstract The activity concentration of 210Po in atmospheric aerosol of Shenzhen and its committed effective dose through inhalation were studied. The activity concentrations of 210Po in total suspended particle (TSP) and PM2.5 were in the range of 0.01~0.20mBq/m3 (with an average of 0.08mBq/m3) and 0.03~0.38mBq/m3 (with an average of 0.12mBq/m3), respectively. The activity concentration of 210Po showed significant positive correlation with the atmospheric concentration of PM2.5, whereas it showed poor relationship with the amount of rainfall.It is suggested that the atmosphericparticle was the key factor that control the activity concentration of 210Po in the air. The calculated average annual committed effective dose of 210Po through inhalation was 4.53×10-6Sv.
|
Received: 29 October 2016
|
|
|
|
|
[1] |
Moore H E, Martell E A, Poet S E.Sources of Polonium-210 in Atmosphere[J]. Environmental Science & Technology, 1976, 10(6):586-591.
|
[2] |
Yan G, Cho HM, Lee I, et al. Significant Emissionsof 210Po by Coal burning into the Urban Atmosphere ofSeoul, Korea[J]. Atmospheric Environment, 2012,54:80-85.
|
[3] |
张静,李鹏翔,李周,等.大气气溶胶中210Pb和210Po 活度浓度及来源[J]. 辐射防护通讯, 2015,35(6):17-22.
|
[4] |
岳玉美,宋刚,张志强,等.广州市北部土壤天然放射性水平研究[J]. 中国环境科学, 2011,31(4):657-661.
|
[5] |
单健.大气颗粒物滞留时间的测量方法研究及应用[D]. 衡阳:南华大学, 2010.
|
[6] |
Baskaran M, Shaw G E. Residence time of arctic haze aerosols using the Concentrations and activity ratios of Po-210, Pb-210 and Be-7[J]. Aerosol Sci, 2001,32:443-452.
|
[7] |
Ram K, Sarin M M. Atmospheric 210Pb, 210Po and 210Po /210Pb activity ratio in urban aerosols:temporal variability and impact of biomass burning emission[J]. Tellus Series B-chemical & Physical Meteorology, 2012,64(1):1-11.
|
[8] |
李加兴,潘竞舜,文富平,等.大气气溶胶滞留时间计算和分析[J]. 辐射防护通讯, 2013,33(3):25-28.
|
[9] |
张晔,曹钟港,王克斌,等.气溶胶中钋-210的分析[J]. 辐射防护, 2015,35(4):239-242.
|
[10] |
McNeary D, BaskaranM. Residence times and temporal variations of 210Po in aerosols and precipitation from southeastern Michigan[J]. United States, Geophys, 2007,112(D4):1-11.
|
[11] |
Persson B R R, Holm E.7Be, 210Pb and 210Po in the surface air from the Arctic to Antarctica[J]. Environ, 2014,138:364-374.
|
[12] |
Gjelsvik R, Brown J, Holm E, et al. Polonium-210 and other Radio nuclides in Terrestrial and Freshwater Environments, NKS-B/GAPRAD, Norwegian Radiation Protection Authority[M]. Norway, 2009.
|
[13] |
UNSCEAR Sources. Effects and Risks of Ionizing Radiation[M]. UNSCEAR 1988Report, New York:UN, 1988.
|
[14] |
曹钟港,王克斌,杨阳,等.大气气溶胶210Pb与210Po 水平及剂量评价[C]. 全国核化学与放射化学学术研讨会, 2014:212-213.
|
[15] |
JiaG, JiaJ. Atmospheric residence times of the fine-aerosol in the region of south Italy estimated from the activity concentration ratios of 210Po /210Pb in air particulates[J]. Analytical & Bioanalytical Techniques, 2014,5:51-59.
|
[16] |
Silva A A. Seasonal variations of Pb-214 and Po-210 concentrations in the surface air in São José dos Campos Brazil[J]. Atmos. Res, 2007,86(1):88-92.
|
[17] |
Daish S R, Dale A A, Dale C J, et al. The temporal variations of 7Be, 210Pb and 210Po in air in England[J]. Journal of Environmental radioactivity, 2005,84(3):457-467.
|
[18] |
Dlugosz-Lisiecka M. The sources and fate of 210po in the urban air:A review[J]. Environment International, 2016,94:325-330.
|
[19] |
Poet S E, Moore H E, Martell E A. 222Rn, 210Pb, 210Bi and 210Po Profiles and Aerosol Residence Times Versus Altitude[J]. Journal of Geophysical Research Atmospheres, 1972,77(33):6515-6527.
|
[20] |
刘国卿,罗奇,潘远海,等.深圳市大气7Be含量分布及其示踪意义[J]. 地球化学, 2014,43(1):32-38.
|
[21] |
Eckerman K, Harrison J, Menzel H G. ICRP Publication 119:International Commission on Radiation Protection Compendium of dose coefficients based on ICRP Publication 60[M]. Netherlands:Elsevier Ltd, 2012:1-130.
|
|
|
|