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Model-derived source apportionment and regional transport matrix study of ozone in Jingjinji |
WANG Yan-li, XUE Wen-bo, LEI Yu, WU Wei-ling |
Chinese Academy for Environmental Planning, Beijing, 100012, China |
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Abstract By coupling ozone source apportionment technology (OSAT) with comprehensive air quality model with extensions (CAMx), the regional transport matrix of surface O3 was built and the spatio-temporal distributions were also analyzed in 13 cities of Jing-Jin-Ji Region in July, 2015. Results showed that the major contributor to O3 was transport source (TS>80%), while the local source (LS) contributed only 6.9% in Langfang and 19.7% in Beijing. The transport source included in-region sources (IRS, ranges from 10.3% in Cangzhou to 32.2% in Langfang), out-region sources (ORS, ranges from 37.3% in Chengde to 60.7% in Qinhuangdao), and boundary condition (BC, ranges from 14.4% in Handan to 23.1% in Zhangjiakou). The daily matrix of regional transport in key cities also showed the significance of ORS to O3. There was a positive correlation between LS contribution and the mass concentrations of O3-8h, in particular, the contribution of LS increased significantly during high ozone episode days. Regarding the regional characteristics of transport path to different cities, the ozone levels were influenced by both local and regional emission sources, and joint efforts are required to optimize the O3 reduction scheme.
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Received: 27 March 2017
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