|
|
Data selection and variation characteristics of atmospheric CH4 observed at Shangdianzi station in Beijing |
XIA Ling-jun1, LIU Li-Xin2 |
1. Jiangxi Climate Center, Nanchang 330096, China;
2. Meteorological Observation Center of China Meteorological Administration, Beijing 100081, China |
|
|
Abstract Based on transport characteristics of air mass 72h back trajectories and statistical data filtered method, measurement data of atmospheric CH4 obtained at Shangdianzi (SDZ) regional background station in Beijing during 2010 and 2014 were analyzed for non-pollution and pollution events. About 42% of the complete data set was filtered as pollution data, and the remainders not polluted by local emission sources were flagged as "representative background data". Variations of background CH4 concentrations at SDZ station can be obtained based on the "representative background data". The annual mean background CH4 concentrations varied from 1884.0×10-9 in 2010 to 1916.4×10-9 in 2014 observed at SDZ, with the averaged growth rate of 8.5×10-9/a. Background atmospheric CH4presented obvious seasonal fluctuations, the higher and lower levels of seasonal CH4 cycle appeared in Jan-Feb and Jun-Jul, respectively, with the peak-to-peak amplitude of 32.8×10-9. The seasonal variations of atmospheric CH4 might be owing to the variations of OH concentration in atmosphere. Furthermore, the annual and "detrended" monthly CH4 background concentrations observed at SDZ were higher than those of MBL at the same latitude and WLG global baseline station.
|
Received: 25 April 2017
|
|
|
|
|
[1] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2015[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2016-10-24.
|
[2] |
Wuebbles D J, Hayhoe K. Atmospheric methane and global change[J]. Earth-Science Reviews, 2002,57(3/4):177-210.
|
[3] |
Zhang B, Chen G Q. Methane Emissions by Chinese Economy:Inventory and Embodiment Analysis[J]. Energy Policy, 2010, 38(8):4304-4316.
|
[4] |
Fu C, Yu G. Estimation and spatiotemporal analysis of methane emissions from agriculture in China[J]. Environmental Management, 2010,46(4):618-632.
|
[5] |
邵立明,仲跻胜,张后虎,等.生活垃圾填埋场春夏季CH4释放及影响因素[J]. 环境科学研究, 2009,22(1):83-88.
|
[6] |
方双喜,李邹,周凌晞,等.云南香格里拉本底站大气CH4体积分数及变化特征[J]. 环境科学学报, 2012,32(10):2568-2574.
|
[7] |
刘萍,余家燕,鲍雷,等.重庆市城区大气中CO2和CH4的浓度特征分析[J]. 西南师范大学学报(自然科学版), 2016, 41(5):146-150.
|
[8] |
许鑫王豪,赵一飞,邹欣庆,等.中国滨海湿地CH4通量研究进展[J]. 自然资源学报, 2015,30(9):1594-1605.
|
[9] |
吴建国,周巧富.青海南部高原积雪期与生长季高寒草甸土壤CO2、CH4和N2O通量的观测[J]. 2016,37(8):2914-2923.
|
[10] |
刘霞,胡海清,赵希宽,等.大兴安岭地区岛状沼泽CH4和N2O排放及其影响因子[J]. 自然资源学报, 2014,29(9):1565-1575.
|
[11] |
刘鹏,张国庆,王剑琼,等.瓦里关大气二氧化碳和甲烷时间变化特征[J]. 环境科学, 2014,35(9):3256-3262.
|
[12] |
方双喜,周凌晞,许林,等.我国4个WMO/GAW本底站大气CH4浓度及变化特征[J]. 环境科学, 2012,33(9):2917-2923.
|
[13] |
Liu L X, Zhou L X, Vaughn B, et al. Background variations of atmospheric CO2 and carbon stable isotopes at Waliguan (WLG) and Shangdianzi (SDZ) stations in China[J]. Journal of Geophysical Research, 2014,119(9):5602-5612.
|
[14] |
Fang S X, Tans P P, Dong F, et al., Characteristics of atmospheric CO2 and CH4at the Shangdianzi regional background station in China[J]. Atmospheric Environment, 2016,131:1-8.
|
[15] |
栾天,周凌晞,方双喜,等.龙凤山本底站大气CO2数据筛分及浓度特征研究[J]. 环境科学, 2014,35(8):2864-2870.
|
[16] |
Tsutsumi Y, Mori K, Ikegami M, et al. Long-term trends of greenhouse gases in regional and background events observed during 1998~2004 at Yonagunijima located to the east of the Asian continent[J]. Atmospheric Environment, 2006,40:5868-5879.
|
[17] |
Pu J J, Xu H H, He J, et al. Estimation of regional background concentration of CO2 at Lin'an Station in Yangtze River Delta[J]. China. Atmospheric Environment, 2014,94:402-408.
|
[18] |
Reimann S, Schaub D, Stemmler K, et al. Halogenated greenhouse gases at the Swiss High Alpine Site of Jungfraujoch (3580m asl):Continuous measurements and their use for regional European source allocation[J]. Journal of Geophysical Research, 2004,109,DOI:10.1029/2003JD003923.
|
[19] |
Jin F J, Kim J, Kim K R. Estimation of Potential Source Region in North east Asia through Continuous In-Situ Measurement of Atmospheric CO2 at Gosan, JejuIsland, Korea[J]. Terrestrial Atmospheric and Oceanic Sciences, 2010,21(2):313-323.
|
[20] |
刘立新,周凌晞,张晓春,等.我国4个国家级本底站大气CO2浓度变化特征[J]. 中国科学, 2009,39(2):222-228.
|
[21] |
孟昭阳,丁国安,汤洁,等.北京上甸子本底站2003年秋冬季痕量气体浓度变化特征[J]. 气象科技, 2007,35(4):550-557.
|
[22] |
栾天,周凌晞,方双喜,等.龙凤山站大气CO2浓度2种筛分方法比对研究[J]. 中国环境科学, 2015,35(2):321-328.
|
[23] |
Thoning K W, Tans P P, Komhyr W D. Atmospheric carbon dioxide at Mauna Loa Observatory:2. Analysis of the NOAA GMCC data, 1974-1985[J]. Journal of Geophysical Research, 1989,94(6):8549-8565.
|
[24] |
Liu Z Y, Wen X Y, Brady E C, et al. Chinese cave records and the East Asia summer monsoon[J]. Quaternary Science Reviews, 83:115-128.
|
[25] |
Thompson R L, Stohl A, Zhou L X, et al. Methane emissions in East Asia for 2000-2011 estimated using an atmospheric Bayesian inversion[J]. Journal of Geophysical Research, 2015,120:4352-4369.
|
[26] |
Wang Y S, Zhou L, Wang M X, et al. Trends of atmospheric methane in Beijing[J]. Chemosphere-Global Change Science, 2001,3(1):65-71.
|
[27] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2014[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2015-11-09.
|
[28] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2013[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2014-11-06.
|
[29] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2012[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2013-11-06.
|
[30] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2011[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2012-11-19.
|
[31] |
WMO. GHGs Bulletin:The State of Greenhouse Gases in the Atmosphere Using Global Observations through 2010[EB/OL]. http://www.wmo.int/pages/prog/arep/gaw/ghg/GHGbulletin.html, 2011-11-21.
|
[32] |
Zhou L X, White J W C, Conway T J, et al. Long-term record of atmospheric CO2 and stable isotopic ratios at Waliguan Observatory:Seasonally averaged 1991-2002 source/sink signal, and a comparison of 1998-2002 record to the 11selected sites in the Northern Hemisphere[J]. Global Biogeochemical Cycle, 2006, 20, GB2001, DOI:10.1029/2004GB002431.
|
[33] |
任信荣,王会祥,邵可声,等.北京市大气OH自由基测量结果及其特征[J]. 环境科学, 2002,23(4):24-27.
|
|
|
|