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Distribution and influence factor of Cu、Pb、Hg in surficial sediments and suspended sediments of Hangzhou Bay |
WANG Shan-shan, PAN Cun-hong, LI Hong, HAN Ceng-cui |
Zhejiang Institute of Hydraulices & Estuary, Hangzhou 310020, China |
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Abstract Heavy metals (Cu, Pb, Hg), grain size parameters, total nitrogen, total Phosphorus, total carbon of 18surface sediments and suspended sediments of Hangzhou Bay were measured to obtain the spatial distribution and influencing factors and based on the 3-D current field established by FVCOM and P-M sedimentary dynamic environment analysis, the role of dynamic deposition in the aggregation of heavy metals was emphatically analysed. In the surface sediments, the maximum value of Cu, Hg appeared in the middle of the bay mouth, while the maximum value of Pb appeared at the north side of the Bay mouth, the contents in the top mouth was much lower, middle of bay mouth was important collection area of Hangzhou Bay. The contents of metals in suspended sediments were slightly higher than in surficial sediments, the discreteness was much smaller and the distribution was much more uniform. The differences of heavy metals in suspended particulate matter and surface sediments reflected the interaction of the sediment discharge from the Yangtze River Estuary and the discharge from the north shore of the Gulf of Hangzhou. The hydrodynamic effect of study area was very strong, the sedimentary differentiation caused by the circulation of tidal current was one of the most important reasons for the different concentrations and discrete difference between suspended sediment and surface sediment. Organic matter played an important role in the enrichment of metals in the surface sediments.
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Received: 05 May 2017
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[1] |
张经.应时理.长江口中的颗粒态重金属.-中国主要可口的生物地球化学研究-化学物质的迁移与环境[M]. 北京:海洋出版社, 1996:146-157.
|
[2] |
刘淑民,姚庆祯,刘月良,等.黄河口湿地表层沉积物中重金属的分布特征及其影响因素[J]. 中国环境科学, 2012,32(9):1625-1631.
|
[3] |
何松琴,宋金明,李学刚,等.长江口及邻近海域夏季表层沉积物中重金属等的分布、来源于沉积环境质量[J]. 海洋科学, 2011,35(5):4-9.
|
[4] |
李磊,平仙隐,王云龙,等.长江口及邻近海域沉积物中重金属研究-时空分布及污染分析[J]. 中国环境科学, 2012,32(12):2245-2252.
|
[5] |
刘明,张爱斌,范德江,等.渤海中部底质沉积物重金属环境质量[J]. 中国环境科学, 2012,32(2):279-290.
|
[6] |
张亚楠,贺青,陈金民,等.珠江口及其邻近海域重金属的河口过程和沉积污染风险[J]. 海洋学报, 2013,35(2):178-186.
|
[7] |
张雷,秦延文,马迎群,等.大辽河感潮河段及其近海河口重金属空间分布及污染评价[J]. 环境科学, 2014,35(9):3336-3345.
|
[8] |
陈吉余,恽才兴,虞志英.杭州湾的动力地貌.中国海岸发育过程和演变规律[M]. 上海:上海科学技术出版社, 1989.
|
[9] |
韩曾萃,戴泽蘅,李广炳,等.钱塘江河口治理开发[M]. 北京:中国水利水电出版社, 2003:77-108.
|
[10] |
鲍根德.杭州湾及其邻近陆架沉积物中某些主要元素的地球化学特征[J]. 海洋学报, 1992,14(5):69-74..
|
[11] |
廖先贵,张湘君,应时理,等.中国海洋学文集[C]//杭州湾重金属的来源及其对泥沙运动的指示意义-中国海洋学文集(2).北京:海洋出版社, 1992:64-78.
|
[12] |
应时理,熊健.杭州湾悬浮颗粒物和沉积物中重金属的来源及变化特征.中国主要河口的生物地球化学研究-化学物质的迁移与环境[M]. 北京:海洋出版社, 1997:92-106.
|
[13] |
张弛,高效江,宋祖光,等.杭州湾河口地区表层沉积物中重金属的分布特征及污染评价[J]. 复旦学报(自然科学版), 2008,47(4):535-540.
|
[14] |
杨耀芳,曹维,朱志清,等.杭州湾海域表层沉积物中重金属污染物的累积及其潜在生态风险评价[J]. 海洋开发与管理, 2013,(1):51-58.
|
[15] |
柴小平,胡宝兰,魏娜,等.杭州湾及邻近海域表层沉积物重金属的分布、来源及评价[J]. 环境科学学报, 2015,35(12):3906-3916.
|
[16] |
GB12763-1991海洋调查规范[S].
|
[17] |
GB17378-1998海洋监测规范[S].
|
[18] |
黄厚见,平仙隐,李磊,等.春、夏季长江口海水、沉积物及生物体中重金属含量及其评价[J]. 生态环境学报, 2011,20(5):898-903.
|
[19] |
张晓琳.长江口、黄河口及邻近海域重金属的分布特征及影响因素研究[D]. 青岛:中国海洋大学, 2013.
|
[20] |
吴斌,宋金明,李学刚.黄河口表层沉积物中重金属的环境地球化学特征[J]. 环境科学, 2013,34(4):1324-1332.
|
[21] |
甘华阳,梁开,郑志昌.珠江口沉积物的重金属背景值及其污染评价分区[J]. 地球与环境, 2010,38(3):344-350.
|
[22] |
王云,魏复盛.土壤环境元素化学[M]. 北京:中国环境科学出版社, 1995.
|
[23] |
汪庆华,董岩翔,郑文,等.浙江土壤地球化学基准值余环境背景值[J]. 地质通报, 2007,26(5):590-597.
|
[24] |
朱而勤.现代海洋自生矿物[J]. 科学通报, 1981,5:44-52.
|
[25] |
陈静生,周家义,刘玉几.中国水环境重金属研究[M]. 北京:中国环境科学出版社, 1992:168-170.
|
[26] |
Attri M J, Thomas R M. Heavy metal concentrations in sediment from the Thames estuary, UK[J]. Marine Pollution Bulletin, 1995,34(11):742-744.
|
[27] |
Audry S, Schafer J, Blanc G, et al. Fifty-year sedimentary record of heavy metal pollution (Cd, Zn, Cu, Pb) in the Lot River reservoirs (France)[J]. Environ Pollut, 2004.
|
[28] |
陈怀满.环境土壤学[M]. 北京:科学出版社, 2005:219-236.
|
[29] |
张莉,祁士华,瞿程凯,等.福建九龙江流域重金属分布来源及健康风险评价[J]. 中国环境科学, 2014,34(8):2133-2139.
|
[30] |
何海星,于瑞莲,胡恭任,等.厦门西港近岸沉积物重金属污染历史及源解析[J]. 中国环境科学, 2014,34(4):1045-1051.
|
[31] |
朱广伟,张路,罗潋葱,等.大型浅水湖泊沉积物内源营养盐释放模式及其估算方法——以太湖为例[J]. 中国科学D辑, 2005,35(增刊Ⅱ):33-44.
|
[32] |
何桐,谢健,余汉生,等.大亚湾表层沉积物中氮的形态分布特征[J]. 热带海洋学报, 2009,28(2):86-92.
|
[33] |
宋祖光,高效江,张弛.杭州湾潮滩表层沉积物中磷的分布、赋存形态即生态意义[J]. 生态学杂志, 2007,26(6):853-858.
|
[34] |
林以安,唐仁友,李炎.长江口区C、N、P的生物地球化学变化对悬浮体絮凝沉降的影响.中国主要河口的生物地球化学研究——化学物质的迁移淤环境[M]. 北京:海洋出版社, 1996.
|
[35] |
王芳,晏维金.长江输送颗粒态磷的生物可利用性及其环境地球化学意义[J]. 环境科学学报, 2004,24(3):418-422.
|
[36] |
戚晓红.中国近海部分典型海域磷的生物地球化学研究[D]. 青岛:中国海洋大学, 2005.
|
[37] |
赵健,毕春娟,陈振楼,等.动力和盐度影响下长江口近岸沉积物中汞的再悬浮行为[J]. 中国科学(化学), 2011,41(1):105-116.
|
[38] |
Godfred Odame duodu, Ashantha Goonetilleke,et al. Comparison of pollution indices for the assessment of heavy metal in Brisbane River sediment[J]. Environmental Pollution, 2016,219:1077-1091.
|
[39] |
徐粲,高建华,杨旸,等.南黄海辐射沙脊群潮汐水道的悬砂输运特征[J]. 海洋学报, 2014,36(11):150-162.
|
[40] |
刘高伟,程和琴,李九发.长江河口河槽水沙特性及其输运机制研究[J]. 泥沙研究, 2015,4:44-51.
|
[41] |
倪勇强,耿兆铨,朱军政.杭州湾水动力特性研讨[J]. 水动力科学研究与进展, 2003,18(4):439-445.
|
[42] |
谢东风,高抒,潘存鸿,等.杭州湾沉积物宏观输运的数值模拟[J]. 泥沙研究, 2012,3:50-56.
|
[43] |
潘存鸿,曾剑,唐子文,等.钱塘江河口泥沙特性及河床冲淤研究[J]. 水利水运工程学报, 2013,1:1-7.
|
[44] |
Pejrup M. The triangular diagram used for classification of estuarine sediments:a new approach[C]//De boer PL. Tide-influenced sedimentary Environments and Facies.Dordrecht:Reidel, 1988:289-300.
|
[45] |
刘红,何青,王元叶,等.长江口表层沉积物粒度时空分布特征[J]. 沉积学报, 2007,25(3):445-455.
|
[46] |
刘朝,师育新,戴雪荣,等.钱塘江河口区不同河段表层沉积物粒度特征[J]. 华东师范大学学报(自然科学版), 2016,6:182-191.
|
[47] |
章伟艳,张霄宇,金海燕,等.长江口-杭州湾及其邻近海域沉积动力环境及物源分析[J]. 地理学报, 2013,68(5):640-650.
|
[48] |
Rahid M A. Geochemistry of marine Humic, Comounds[M]. New York:Springor-Veriga, 1985:115.
|
|
|
|