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Temporal and spatial distribution characteristics of lower troposphere carbon dioxide in Hefei Science Island |
YANG Jie1,2, HU Shun-xing1, YUAN Ke-e1, SUN Pei-yu1,3, HUANG Jian1, WANG Yi-nan4 |
1. Key Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China; 2. University of Science and Technology of China, Hefei 230026, China; 3. Graduate University of Chinese Academy of Sciences, Beijing 100049, China; 4. Key Laboratory of Middle Atmosphere and Global Environment Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China |
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Abstract Based on the carbon dioxide volume mixing ratio concentration profiles of Hefei Science Island from 2013 to 2016,the distribution characteristics of carbon dioxide in the subtropical monsoon climate and the characteristics of carbon dioxide source and sink in Hefei science island were analyzed from the night,season and year respectively.The concentration of carbon dioxide in the atmosphere decreased with the increase of altitude,the carbon dioxide concentration of 390m was about 95% that of 15m.The concentration of carbon dioxide gradually increased at night (about 5%),while there was a tendency to decrease at drawn.When the measurement height was more than 100m,the obvious seasonal change was shown,with the minimum in summer and the maximum in winter,which the difference in concentration of about 10×10-6.With a yearly growth rate of about 2.1648×10-6,the annual distribution of the concentration of carbon dioxide from 2013 to 2016 had no significant difference in the gradient change of the height above 100m,the correlation coefficient was above 0.9,and the volume mixing ratio concentration increased.Through data analysis from three different timescales,it could be concluded that the concentration of carbon dioxide near the ground was greatly influenced by the atmospheric environment.The seasonal distribution of carbon dioxide concentration was the result of a combination of atmospheric movement and the activities of plants and animals.In the process of long-term carbon dioxide cycling,there was a current that the near-surface carbon dioxide transported to a higher altitude.
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Received: 30 August 2017
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[1] |
Wagner G A, Plusquellic D F. Ground-based, integrated path differential absorption LIDAR measurement of CO2, CH4, and H2O near 1.6μm[J]. Applied Optics, 2016,55(23):6292-6310.
|
[2] |
Refaat T F, Singh U N, Yu J, et al. Evaluation of an airborne triple-pulsed 2μm IPDA lidar for simultaneous and independent atmospheric water vapor and carbon dioxide measurements[J]. Applied Optics, 2015,54(6):1387-1398.
|
[3] |
麦博儒,邓雪娇,安兴琴,等.基于卫星遥感的广东地区对流层二氧化碳时空变化特征[J]. 中国环境科学, 2014,34(5):1098-1106.
|
[4] |
Feldman D R, Collins W D, Gero P J, et al. Observational determination of surface radiative forcing by CO2 from 2000 to 2010[J]. Nature, 2015,519(7543):339-343.
|
[5] |
Grady J K, Jeffrey Y B, Fabien G, et al. Side-line tunable laser transmitter for differential absorption lidar measurements of CO2:design and application to atmospheric measurements0[J]. Applied Optics, 2008,47(7):944-956.
|
[6] |
马安娜,陆健健.长江口崇西湿地生态系统的二氧化碳交换及潮汐影响[J]. 环境科学与研究, 24(7):716-721.
|
[7] |
张林海,仝川,曾从盛.河口湿地近地面大气CO2浓度日变化和季节变化[J]. 环境科学, 2014,35(3):879-884.
|
[8] |
浦静姣,徐宏辉,顾骏强,等.长江三角洲背景地区CO2浓度变化特征研究[J]. 中国环境科学, 2012,32(6):973-979.
|
[9] |
周聪,施润和,高炜.对流层中层与近地面大气二氧化碳浓度的比较研究[J]. 地球信息科学学报, 2015,17(11):1286-1293.
|
[10] |
孙培育,苑克娥,胡顺星,等.拉曼激光雷达探测合肥西郊低对流层大气二氧化碳垂直分布的统计分析[J]. 光学学报, 2016,36(11):1-8.
|
[11] |
于海利,胡顺星,吴晓庆,等.拉曼激光雷达探测低对流层大气二氧化碳分布[J]. 光学学报, 2012,32(8):21-26.
|
[12] |
苑克娥,张世国,胡顺星,等.拉曼散射激光雷达反演二氧化碳测量结果的可靠性分析[J]. 红外与激光工程, 2014,43(4):1135-1139.
|
[13] |
吴晓庆,林晓庆,朱行听,等.合肥地区近地面辐射通量和二氧化碳统计分析与湍流通量的惯性耗散法估算[J]. 大气与环境光学学报, 2011,(1):69-74.
|
|
|
|