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The vertical change in extinction effect of particles during a haze episode in Chengdu |
SUN Yong-liang1, ZHAO Tian-liang1, QIU Yu-jun1, LUO lei2, XIA Jun-rong1, CHEN Hong3, XIE Na3 |
1. Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China; 2. Chengdu Plateau Meteorological Research Institution, China Meteorological Administration, Chengdu 610031, China; 3. Chengdu Meteorological Bureau, Chengdu 610031, China |
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Abstract Based on the intensive vertical observation of particle size spectrum and synchronous lidar observation during a heavy haze event in Chengdu over January 4~7, 2017, as well as the extinction coefficients calculated using the Mie scattering theory and compared with the lidar observation, the extinction coefficients of particle in sizes and the contributions to the total extinction were estimated. The results showed that during the heavy haze episode, the magnitudes of extinction coefficients of particles with different sizes in heights was ranked with PM1 > PM2.5~10 > PM1~2.5 > PM > 10 within the boundary layer, and the PM1 was the major factor dominating the particle extinction with the contribution of 49.50%~69.44%. In atmospheric boundary layer, extinction of all size particles presented the pronounced vertical and diurnal variations. In the daytime, the high extinction coefficients were located at the altitude below 600m and between 700 and 1100m. In the nighttime, the extinction coefficients vertically decreased more significantly with the high values around 1100m. Additionally, the extinction coefficients and the extinction contributions of PM>1 below 200m in the nighttime were obviously greater than those in the daytime. In general, the extinction contribution rates of PM1 increased with the decreasing contribution rates of PM>1 in total particle extinction following vertical heights.
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Received: 12 October 2017
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[1] |
Hinds W C. Aerosol technology:properties, behavior, and measurement of airborne particles[J]. Journal of Aerosol Science, 1998,31(9):1121-1122.
|
[2] |
王继志,杨元琴.北京城市能见度及雾特征分析[J]. 应用气象学报, 2002,13(s1):160-169.
|
[3] |
陈义珍,赵丹,柴发合,等.广州市与北京市大气能见度与颗粒物质量浓度的关系[J]. 中国环境科学, 2010,30(7):967-971.
|
[4] |
吴兑,邓雪娇,毕雪岩,等.细粒子污染形成灰霾天气导致广州地区能见度下降[J]. 热带气象学报, 2007,23(1):1-6.
|
[5] |
Molnár A, Mészáros E. On the relation between the size and chemical composition of aerosol particles and their optical properties[J]. Atmos. Environ., 2001,35(30):5053-5058.
|
[6] |
韩茜,魏文寿,刘新春,等.乌鲁木齐不同分级气溶胶理化特征及其对大气消光的影响[J]. 沙漠与绿洲气象, 2015,9(6):68-72.
|
[7] |
王琼,毕晓辉,张裕芬,等.杭州市大气颗粒物消光组分的粒径分布特征研究[J]. 中国环境科学, 2012,32(1):10-16.
|
[8] |
沈艳,张泽锋,李艳伟,等.南京北郊一次霾过程中气溶胶理化特征变化研究[J]. 环境科学学报, 2016,36(7):2314-2323.
|
[9] |
尚倩,李子华,杨军,等.南京冬季大气气溶胶粒子谱分布及其对能见度的影响[J]. 环境科学, 2011,32(9):2750-2760.
|
[10] |
于兴娜,马佳,朱彬,等.南京北郊秋冬季相对湿度及气溶胶理化特性对大气能见度的影响[J]. 环境科学, 2015,(6):1919-1925.
|
[11] |
谭建成,林国杨,陈政豪,等.利用激光雷达测量都市上空气溶胶的浓度分布[J]. 光散射学报, 2008,20(4):375-378.
|
[12] |
胡欢陵,吴永华,谢晨波,等.北京地区夏冬季颗粒物污染边界层的激光雷达观测[J]. 环境科学研究, 2004,17(1):59-66.
|
[13] |
韩道文,刘文清,刘建国,等.气溶胶质量浓度空间垂直分布的反演方法[J]. 中国激光, 2006,33(11):1567-1573.
|
[14] |
张春光,张玉钧,韩道文,等.气溶胶质量浓度垂直分布反演模型的研究[J]. 激光技术, 2009,33(3):303-306.
|
[15] |
刘东,戚福弟,金传佳,等.合肥上空卷云和沙尘气溶胶退偏振比的激光雷达探测[J]. 大气科学, 2003,27(6):1093-1100.
|
[16] |
Sassen K. The polarization lidar technique for cloud research:A review and current assessment.[J]. Bulletin of the American Meteorological Society, 1991,72(12):1848-1866.
|
[17] |
Pal S R, Carswell A I. Polarization properties of lidar scattering from clouds at 347nm and 694nm.[J]. Applied Optics, 1978, 17(15):2321-8.
|
[18] |
Iwasaka Y, Hayashida S. The effects of the volcanic eruption of St. Helens on the polarization properties of stratospheric aerosols-Lidar measurement at Nagoya[J]. Meterological Society of Japan, 1981, 59(4):611-614.
|
[19] |
Schotland R M, Sassen K, Stone R. Observations by lidar of linear depolarization ratios for hydrometeors.[J]. Journal of Applied Meteorology, 2010,10(5):1011-1017.
|
[20] |
Fernald F G. Analysis of atmospheric lidar observations:some comments[J]. Applied Optics, 1984,23(5):652.
|
[21] |
杨欣,陈义珍,刘厚凤,等.北京2013年1月连续强霾过程的污染特征及成因分析[J]. 中国环境科学, 2014,34(2):282-288.
|
[22] |
Hartmann M. Light scattering by small particles. Von H. C. VANDE HULST. New York:Dover Publications, Inc. 1981. Paperback, 470S. 103Abb. und 46Tab. US $ 7.50[J]. Acta Polymerica, 1984,35(4):338-338.
|
[23] |
李丽芳,张记龙,李晓,等.近红外波段气溶胶的消光特性研究[J]. 激光与红外, 2013,43(1):24-28.
|
[24] |
Hansen J E, Travis L D. Light scattering in planetary atmospheres[J]. Space Sci. Rev., 1974,16:527-610.
|
[25] |
吴兑.霾与雾的识别和资料分析处理[J]. 环境化学, 2008, 27(3):327-330.
|
[26] |
葛应,刘志红,汤志亚.成都市气溶胶消光系数特征分析[J]. 四川环境, 2015,34(1):38-43.
|
[27] |
蒋燕,贺光艳,罗彬,等.成都平原大气颗粒物中无机水溶性离子污染特征[J]. 环境科学, 2016,37(8):2863-2870.
|
[28] |
张彩艳,吴建会,张普,等.成都市冬季大气颗粒物组成特征及来源变化趋势[J]. 环境科学研究, 2014,27(7):782-789.
|
[29] |
严国梁,韩永翔,张祥志,等.南京地区一次灰霾天气的微脉冲激光雷达观测分析[J]. 中国环境科学, 2014,34(7):1667-1672.
|
[30] |
杜川利,唐晓,李星敏,等.城市边界层高度变化特征与颗粒物浓度影响分析[J]. 高原气象, 2014,33(5):1383-1392.
|
[31] |
Sorbjan, Zbigniew. The atmospheric boundary layer[M]//Atmospheric boundary layer flows:Oxford University Press, 2002:225-250.
|
[32] |
Liu J, Zhu L, Wang H, et al. Dry deposition of particulate matter at an urban forest, wetland and lake surface in Beijing[J]. Atmospheric Environment, 2016,125:178-187.
|
[33] |
叶兴南, 陈建民. 灰霾与颗粒物吸湿增长[J]. 自然杂志, 2013,35(5):334-341.
|
[34] |
吴丹,曹双,汤莉莉,等.南京北郊大气颗粒物的粒径分布及其影响因素分析[J]. 环境科学, 2016,37(9):3268-3279.
|
|
|
|