|
|
Assessment of the effect of the reduction of the residential coal combustion on the atmospheric BaP pollution in Beijing-Tianjin-Hebei region. |
HAN Mei-li1,2, LIU Shi-jie2, LIU Min1, LU Min1, YAN Wen-jun3, HE You-jiang2, DANG Hong-yan2, DAI Xue-zhi2, ZHANG Zhong-zhi2, DU Xiao-hui2, MENG Fan2 |
1. College of Geographic Sciences, East China Normal University, Shanghai 200241, China;
2. Atmospheric Environment Institute, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;
3. Gansu Meteorological Bureau, Lanzhou 730000, China |
|
|
Abstract The regional air quality model CMAQ was used to simulate and evaluate the effect of residential coal combustion emission reduction policies on atmospheric BaP pollution in Beijing-Tianjin-Hebei (BTH) region. The simulations included a base scenario (the year of 2014) and two scenarios of emission reductions. The simulation results:the annual average concentration of atmospheric BaP in BTH in the base scenario was 2.54ng/m3, which was more than twice of the national air quality standard (1ng/m3).The levels of monthly average concentration of atmospheric BaP were in the order:January, April, October, July, reflecting the impact of coal for heating in winter on atmospheric BaP concentration. The atmospheric BaP concentration of southern BTH region was higher than that of the northern region over BTH region, the reason was probably the higher BaP emissions in the south of BTH than in the north. The emissions reduction of rediential coal in January has the most significant effect on reducing concentration of atmospheric BaP and depotion.The concentrations of atmospheric BaP in January over Beijing, Baoding and Langfang in low (scenario1) and high (scenario2) were reduced by 30% and 40% respectively compared with the base scenario.The emissions reduction of rediential coal combustion in April, July and October had little effect on the changes of atmospheric BaP concentration and depotion. Taking control measures of residential coal consumption in all BTH region could more effectively reduce the concentration of atmospheric BaP concentration in this area.
|
Received: 12 January 2018
|
|
|
|
|
[1] |
Lin Y, Ma Y, Qiu X, et al. Sources, transformation, and health implications of PAHs and their nitrated, hydroxylated, and oxygenated derivatives in PM2.5 in Beijing[J]. Geophysical Research Atmospheres, 2015,120(14):7219-7228.
|
[2] |
Xue X, You Y, Wu J, et al. Exposure measurement,riskassessment and source identification for exposure of traffic assistants to particle-bound PAHs in Tianjin.China[J]. Environmental Sciences, 2014,26:448-457.
|
[3] |
Zhu Y, Yang L, Yuan Q, et al. Airborne particulate polycyclic aromatic hydrocarbon (PAH) pollution in a background site in the North China Plain:concentration, size distribution, toxicity and sources[J]. Science of the Total Environment, 2014,466-467:357-368.
|
[4] |
Matthias V, Aulinger A, Quante M. CMAQ simulations of the Benzo(a)pyrene distribution over Europe for 2000 and 2001[J]. Atmospheric Environment, 2009,43(26):4078-4086.
|
[5] |
José R S, Pérez J L, Callén M S, et al. BaP(PAH)air quality modelling exercise over Zaragoza (Spain) using an adapted version of WRF-CMAQ model[J]. Environmental Pollution, 2013,183:151-158.
|
[6] |
Bewersdorff I, Aulinger A, Volker M, et al. Modeling of benzo(a)pyrene concentrations in north sea coastal areas:contribution of ship emissions[J]. Hrvatski meteorološki casopis, 2008,43(43/2):586-590.
|
[7] |
Zhang H, Ying Q. Secondary organic aerosol from polycyclic aromatic hydrocarbons in Southeast Texas[J]. Atmospheric Environment, 2012,55:279-287.
|
[8] |
王超,张霖琳,刀胥,等.京津冀地区城市空气颗粒物中多环芳烃的污染特征及来源[J]. 中国环境科学, 2015,35(1):1-6.
|
[9] |
Okuda T, Okamoto K, Tanaka S, et al. Measurement and source identification of polycyclic aromatic hydrocarbons (PAHs) in the aerosol in Xi'an, China, by using automated column chromatography and applying positive matrix factorization (PMF)[J]. Science of the Total Environment, 2010,408(8):1909-1914.
|
[10] |
汪祖丞,刘敏,杨毅,等.上海城区多环芳烃的多介质归趋模拟研究[J]. 中国环境科学, 2011,31(6):984-990.
|
[11] |
刘敏,王兰辉.城市地表系统POPs多介质循环过程与模拟研究进展[J]. 中国环境科学, 2013,33(11):2018-2026.
|
[12] |
Liu S, Lu Y, Wang T, et al. Using gridded multimedia model to simulate spatial fate of Benzo[a]pyrene on regional scale[J]. Environment International, 2014,63:53-63.
|
[13] |
Zhu Y, Tao S, Price O R, et al. Environmental distributions of Benzo[a]pyrene in China:Current and future emission reduction scenarios explored using a spatially explicit multimedia fate model[J]. Environmental Science & Technology, 2015,49:13868-13877.
|
[14] |
闫文君,刘敏,刘世杰,等.基于CMAQ模式的中国大气BaP迁移转化模拟研究[J]. 中国环境科学, 2016,36(6):1681-1689.
|
[15] |
China Environmental Bulletin. Ministry of environmental protection of the People's Republic of China[Z]. 2014,2015-11-08.
|
[16] |
Ravindra K, Sokhi R, Grieken R V. Atmospheric polycyclic aromatic hydrocarbons:Source attribution, emission factors and regulation[J]. Atmospheric Environment, 2008,42:2895-2921.
|
[17] |
Wang W T, Jariyasopit N, Schrlau J, et al. Concentration and photochemistry of PAHs, NPAHs, and OPAHs and toxicity of PM2.5 during the Beijing Olympic Games[J]. Environmental Science & Technology, 2011,45:6887-6895.
|
[18] |
丁峰,张阳,李鱼.京津冀大气污染现状及防治方向探讨[J]. 环境保护, 2014,42(21):55-57.
|
[19] |
陈颖军,冯艳丽,支国瑞,等.民用煤室内燃烧条件下多环芳烃的排放特征[J]. 地球化学, 2007,36(1):49-54.
|
[20] |
段凤魁,贺克斌,马永亮.北京PM2.5中多环芳烃的污染特征及来源研究[J]. 环境科学学报, 2009,29(7):1363-1371.
|
[21] |
王焕新,张续,马琳,等.北京市昌平区大气颗粒物中多环芳烃暴露及人群健康风险评价[J]. 环境与健康, 2016,33(11):999-1003.
|
[22] |
Shen H, Huang Y, Wang R, et al. Global atmospheric emissions of polycyclic aromatic hydrocarbons from 1960 to 2008 and future predictions[J]. Environmental Science & Technology, 2013,47:6415-6424.
|
[23] |
毕新慧,盛国英,谭吉华,等.多环芳烃(PAHs)在大气中的相分布[J]. 环境科学学报, 2004,24(1):101-106.
|
[24] |
吴胜刚,刘屹岷,邹晓蕾,等.WRF模式对青藏高原南坡夏季降水的模拟分析[J]. 气象学报, 2016,74(5):744-756.
|
[25] |
张树才,沈亚婷,王开颜,等.北京东南郊大气中多环芳烃的沉降[J]. 2007,20(4):28-33.
|
[26] |
Niu X Y, Ho S S H, Ho K F, et al. Atmospheric levels and cytotoxicity of polycyclic aromatic hydrocarbons and oxygenated-PAHs in PM2.5 in the Beijing-Tianjin-Hebei region[J]. Environmental Pollution, 2017,231(1):1075-1084.
|
[27] |
国家气象科学数据共享服务平台[EB/OL]. http://data.cma.cn/data/cdcdetail/dataCode/SURF_CLI_CHN_MUL_MON.html.
|
[28] |
冯利红,赵岩,李建平,等.天津市部分地区冬季大气PM2.5中多环芳烃污染特征分析[J]. 环境与健康, 2015,32(9):802-804.
|
[29] |
曹文文,张振江,赵若杰,等.室内空气PM10中PAHs对老年人的致癌风险评价[J]. 中国环境科学, 2013,33(2):345-350.
|
[30] |
Wang W, Simonich S, Giri B, et al. Atmospheric concentrations and air-soil gas exchange of polycyclic aromatic hydrocarbons (PAHs) in remote, rural village and urban areas of Beijing-Tianjin region, North China[J]. Science of the Total Environment, 2011,409(15):2942-2950.
|
[31] |
GB 3095-2012《环境空气质量标准》[S]. http://kjs.mep.gov.cn/hjbhbz/bzwb/dqhjbh/dqhjzlbz/201203/W020120410330232398521.pdf.
|
|
|
|