卫星观测资料改进活性VOCs源排放及其对臭氧模拟影响

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Abstract Introduced is a methodology of improving bottom-up volatile organic compound (VOC) emissions by using space-based formaldehyde measurements. The regression equation between satellite observations and pollutant emissions was established which used the bottom-up emission inventories of INTEX-B for anthropogenic VOCs, FINNv1for the biomass burning source, and MEGAN for the biogenic source. The anthropogenic emissions were enhanced by 1.51, 1.87, and 1.93 times in the Beijing-Tianjin-Hebei region, the Yangtze River Delta, and the Pearl River Delta, respectively, whereas the biomass burning emissions were enhanced by 12.2, 6.15, and 2.27 times, and the biogenic emissions were enhanced by 1.66, 1.31, and 1.21 times, respectively, as constrainted by a continuous 3-year record (2005~2007) of OMI satellite measurements. The improved emissions are in good agreement with previous results. Using the improved emission inventories, O₃ simulations with the WRF Chem model were conducted, showing that simulated O₃ was increased in different seasons in the above three regions, with large increases (more than 20×10^-9) in major cities and surrounding areas of the three regions in each season, consistent with the VOC-sensitive urban areas in China. The methodology presented in this paper can be further improved and widely used in air pollution research, especially in the improvement of emission inventories.

Key words： satellite observation HCHO column volatile organic compound emission inventory

Received: 02 November 2020

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X511

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	WANG Feng
	WANG Jian-wei
	ZHAI Jing
	HOU Can

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WANG Feng,WANG Jian-wei,ZHAI Jing等. Emission improvements of reactive VOCs based on satellite observations and their impact on ozone simulations[J]. CHINA ENVIRONMENTAL SCIENCECE, 2021, 41(6): 2504-2514.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2021/V41/I6/2504

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