全球近地层臭氧时空分布特征及其来源解析

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Abstract Based on observational data from the Acid Deposition Monitoring Network in East Asia (EANET) and World Data Centre for Greenhouse Gases (WDCGG), the seasonal variation characteristics of surface ozone in various regions was compared. By MOZART-4model and the online tagging method, combined with the analysis of O₃ budget, the contribution of various effects to ozone were confirmed in different regions. The model-simulated O₃ and its precursors agreed well with observed values and other researches in the troposphere. The analyses of O₃ budgets at surface showed the values of budgets were relatively low (-3×10^-9~ 3×10^-9/d), and the chemistry was net loss of O₃ over clean background regions (most near ocean). Over continental region, the chemistry was net production of O₃(~ 33.8×10^-9/d), and the main sources of surface O₃ were from inside of troposphere, while the contributions of stratospheric O₃ were relatively low (~ 10×10^-9). Over polar and clean region, the contributions of stratospheric O₃ showed obvious seasonal changes with the largest in winter (~ 20.7×10^-9) and the lowest in summer (~2×10^-9), which account for the O₃ seasonal variations.

Key words： tropospheric ozone global atmospheric chemistry model online tagging ozone ozone budget seasonal variation

Received: 15 December 2020

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	FEI Dong-dong
	HOU Xue-wei
	WEI Lei

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FEI Dong-dong,HOU Xue-wei,WEI Lei. Quantitative sources of global surface ozone and spatial and temporal distribution characteristics[J]. CHINA ENVIRONMENTAL SCIENCECE, 2021, 41(7): 3004-3016.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2021/V41/I7/3004

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