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Factors of high total phosphorus concentration in the Nanchang typical area of Poyang Lake |
ZHU Li-ying1,2, ZHENG Li-bing1,2, WANG Ya-wei1,2, ZHANG Hong3,4, SHU Li-min3,4, GUI Shuang-lin5, XIA Song5, YAN Bing5, LIU Ji-bao1,2, HU Da-zhou1,2,4, TAO Mao-liang6, GAO Jie7, WEI Yuan-song1,2,4 |
1. State Key Joint Laboratory of Environment Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; 2. Laboratory of Water Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; 3. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; 4. University of Chinese Academy of Sciences, Beijing 100049, China; 5. Institute of Energy Research, Jiangxi Academy of Sciences, Nanchang 330029, China; 6. Xinjian Municipal Ecology and Environment Bureau of Nanchang City, Nanchang 330100, China; 7. Nanchang Municipal Ecological and Environment Monitoring Center, Nanchang 330038, China |
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Abstract In this study, the Nanjishan national monitoring site (NJS site) and its confluence area were selected to explore causes of the high TP concentration through the field investigation of the water environmental factors and sediments. Results indicated that the TP exceedance in the surface water mainly occurred in the low lake water level period (LLP) and lake discharges period (LDP), with the exceedance multiples of 3.06 and 2.78 times, respectively; and TP concentration was significantly correlated with dissolved organic matter (DOM) and turbidity. Three-dimensional fluorescence spectroscopy (3D-EEM) regional integration method and parallel factor analysis (PARAFAC) showed that the DOM consisted of three components, which were dominated by humus-like substances such as fulvic acid (partition III, components C1 and C2), and the main source of which was the degradation of wetland plant litter, with the highest proportion (55.74%) in the LLP. The proportion of protein-like substances (partition I and component C3) increased to more than 35% during the RDP due to inputs of the confluence tributaries and the neighboring disc-shaped lake. TP showed a significant positive correlation (P<0.05) with humic organic matter and a significant negative correlation (P<0.05) with proteic organic matter, indicating that TP and humic organic matter have a common origin. TP and turbidity showed a significant positive correlation (P<0.05), and the highest turbidity was observed in LLP (mean value of 320.83NTU), during which the tributaries and the disc-shaped lake were cut off. The sediment substrate in the study area was chalky, dominated by fine components, and the median grain size DX(50) belonged to fine chalky (2~16μm); the range of sorting coefficients was 2.11~2.75, with poor sorting; the sediment samples were mostly located in the bottom-side suspended and homogeneous suspended transport area, with weak sedimentary hydrodynamics and weak transport capacity; the suspended particulate matter that was not easily deposited, resulting in high turbidity. The average TP content of 0~5cm surface sediment was high (527.89mg/kg), and sediment P was released to the overlying water, with the largest P release flux (0.21mg/(m2·d)) in the NJS site, indicating that surface sediments was one of the important influences on TP concentrations in the site waters.
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Received: 26 July 2023
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Corresponding Authors:
魏源送,研究员,yswei@rcees.ac.cn
E-mail: yswei@rcees.ac.cn
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