The sorption properties of tylosin by black carbon-humic acid complex
DONG Hao1, GUO Xue-tao1, WU Hui-jun1, YANG Chen2, PENG Dan3, GAO Liang-min1, HU You-biao1
1. School of Earth and Environment, Anhui University of Science and Technology, Huainan 232001, China;
2. College of Environment and Energy, South China University of Technology, Guangzhou 510006, China;
3. School of Traffic and Environment, Shenzhen Institute of Information Technology, Shenzhen 518172, China
Based on tylosin was wsed as one representative organic pollutant, the sorption characteristics and mechanism of tylosin on different sources of nano black carbon-humic acid complexes was invesitigated. Results showed that the sorption capacity of black carbon and humic acid complex was higher than that of black carbon and humic acid; the sorption equilibrium could be obttained within 24hours; the sorption kinetics of tylosin on both black carbon and black carbon-humic acid complex fitted the pseudo-second-order kinetics model; the sorption isotherms could fit well with the Henry model and Freundlich model; the sorption capacity of tylosin on black carbon and humic acid complex would be altered in different solution chemistries (i.e., pH and ionic strength of solutions). Ion-exchange, hydrogen-bond, and hydrophobic play a main role in the sorption of tylosin on black carbon and humic acid complex.
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Guo X T, Yang C, Dang Z, et al. The influences of pH and ionic strength on the sorption of tylosin on goethite[J]. Environmental Science and Pollution Research, 2014,21(4):2572-2580.
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Zheng H, Wang Z Y, Zhao J, et al. Sorption of antibiotic sulfamethoxazole varies with biochars produced at different temperatures[J]. Environmental Pollution, 2013,181:60-67.
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Guo X T, Yang C, Zhang J, et al. Sorption and photodegradation of tylosin and sulfamethazine by humic acid-coated goethite[J]. RSC Advances, 2015,5(122):100464-100471.
Ruan Z H, Wu J H, Xie J, et al. Facile preparation of rosin-based biochar coated bentonite for supporting α-Fe2O3 nanoparticles and its application for Cr(vi) adsorption[J]. Journal of Materials Chemistry A, 2015,3(8):4595-4603.
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Luo L, Lou L P, Cui X Y, et al. Sorption and desorption of pentachlorophenol to black carbon of three different origins[J]. Journal of Hazardous Materials, 2011,185(2/3):639-646.
[15]
Lin K, Ding J, Wang H, et al. Goethite-mediated transformation of bisphenol A[J]. Chemosphere, 2012,89(7):789-795.
Lian F, Sun B B, Chen X, et al. Effect of humic acid (HA) on sulfonamide sorption by biochars[J]. Environmental Pollution, 2015,204:306-312.
[18]
Zhang Q, Zhao L, Dong Y H, et al. Sorption of norfloxacin onto humic acid extracted from weathered coal[J]. Journal of Environmental Management, 2012,102:165-172.
[19]
Guo X T, Dong H, Yang C, et al. Application of goethite modified biochar for tylosin removal from aqueous solution[J]. Colloids and Surfaces A:Physicochemical and Engineering Aspects, 2016,502:81-88.
[20]
Zhang J, He M C, Lin C Y, et al. Phenanthrene sorption to humic acids, humin, and black carbon in sediments from typical water systems in China[J]. Environmental Monitoring and Assessment, 2010,166(1-4):445-459.
[1]
Guo X T, Ge J H, Yang C, et al. Sorption behavior of tylosin and sulfamethazine on humic acid:kinetic and thermodynamic studies[J]. RSC Advances, 2015,5(72):58865-58872.
Rakshit S, Sarkaret D, Punamiya P, et al. Kinetics of oxytetracycline sorption on magnetite nanoparticles[J]. International Journal of Environmental Science and Technology, 2014,11(5):1207-1214.
[5]
Marc T, Joseph J P, Carles H, et al. Predicting contaminant adsorption in black carbon (biochar)-amended soil for the veterinary antimicrobial sulfamethazine[J]. Environmental Science & Technology, 2013,47(12):6197-6205.
[6]
Ji L L, Zhu D Q, Wan Y Q, et al. Adsorption of tetracycline and sulfamethoxazole on crop residue-derived ashes:Implication for the relative importance of black carbon to soil sorption[J]. Environmental Science & Technology, 2011,45(13):5580-5586.
[7]
Lou L P, Luo L, Hu B L, et al. The sorption of pentachlorophenol by aged sediment supplemented with black carbon produced from rice straw and fly ash[J]. Bioresource Technology, 2012,112:61-66.
[8]
Jia M, Wang F, Bian Y R, et al. Effects of pH and metal ions on oxytetracycline sorption to maize-straw-derived biochar[J]. Bioresource Technology, 2013,136:87-93.
[9]
Guo X T, Yang C, Dang Z, et al. The influences of pH and ionic strength on the sorption of tylosin on goethite[J]. Environmental Science and Pollution Research, 2014,21(4):2572-2580.
[10]
Zheng H, Wang Z Y, Zhao J, et al. Sorption of antibiotic sulfamethoxazole varies with biochars produced at different temperatures[J]. Environmental Pollution, 2013,181:60-67.
[11]
Guo X T, Yang C, Zhang J, et al. Sorption and photodegradation of tylosin and sulfamethazine by humic acid-coated goethite[J]. RSC Advances, 2015,5(122):100464-100471.
Ruan Z H, Wu J H, Xie J, et al. Facile preparation of rosin-based biochar coated bentonite for supporting α-Fe2O3 nanoparticles and its application for Cr(vi) adsorption[J]. Journal of Materials Chemistry A, 2015,3(8):4595-4603.
[14]
Luo L, Lou L P, Cui X Y, et al. Sorption and desorption of pentachlorophenol to black carbon of three different origins[J]. Journal of Hazardous Materials, 2011,185(2/3):639-646.
[15]
Lin K, Ding J, Wang H, et al. Goethite-mediated transformation of bisphenol A[J]. Chemosphere, 2012,89(7):789-795.
Lian F, Sun B B, Chen X, et al. Effect of humic acid (HA) on sulfonamide sorption by biochars[J]. Environmental Pollution, 2015,204:306-312.
[18]
Zhang Q, Zhao L, Dong Y H, et al. Sorption of norfloxacin onto humic acid extracted from weathered coal[J]. Journal of Environmental Management, 2012,102:165-172.
[19]
Guo X T, Dong H, Yang C, et al. Application of goethite modified biochar for tylosin removal from aqueous solution[J]. Colloids and Surfaces A:Physicochemical and Engineering Aspects, 2016,502:81-88.
[20]
Zhang J, He M C, Lin C Y, et al. Phenanthrene sorption to humic acids, humin, and black carbon in sediments from typical water systems in China[J]. Environmental Monitoring and Assessment, 2010,166(1-4):445-459.
