黄河水氢、氧同位素组成特征及其气候变化响应

摘要
图/表
参考文献(34)
相关文章 (15)

全文: PDF (1078 KB) HTML (1 KB)
输出: BibTeX | EndNote (RIS)

摘要

于2012年7~8月采集黄河流域干流和支流河水样品，通过分析水体氢氧同位素组成的时间和空间变化特征，研究了河水主要来源的变化以及其对流域气候变化的响应.结果表明：除源头河水外，黄河干流河水δD值变化范围为-97.2‰~-62.9‰，均值为-72.2‰， δ¹⁸O值范围为-13.0‰~-8.7‰，均值为-9.9‰， d盈余值为4.1‰~11.0‰，均值为7.0‰；支流河水δD值范围为-103.8‰~-30.5‰，均值为-68.9‰， δ¹⁸O值范围为-13.7‰~-1.5‰，均值为-9.2‰， d盈余值为-18.5‰~13.2‰，均值为4.5‰.黄河干流兰州段以上以及中游河水氢氧同位素均值均偏负，而兰州至头道拐和下游河水氢氧同位素均值偏正，但河水氘盈余均值呈现由上游到下游逐渐降低的趋势.黄河干流和支流河水Na⁺/Cl^-摩尔比值范围为0.94~3.02，源头区黄河干流河水Na⁺/Cl^-摩尔比均值为1.02，兰州段以上均值为1.58，兰州至头道拐间均值为1.30，中游均值为1.79，下游均值为1.41.河水Na⁺/Cl^-摩尔比值与河水δ¹⁸O值呈较好的负相关关系，表明黄河河水受大气降水补给，地下水补给以及蒸发作用等控制.与前人研究结果对比发现，2000年以来黄河河水年径流量逐渐增加，上游河水受二次蒸发过程影响在降低，中游和下游河水受蒸发作用影响在减弱，显示区域气候干旱状况有所降低.

	服务

	把本文推荐给朋友
	加入我的书架
	加入引用管理器
	E-mail Alert
	RSS
	作者相关文章
	范百龄
	张东
	陶正华
	赵志琦

关键词 ：黄河流域, 氢氧同位素, 大气降水, 气候变化

Abstract：

To better understand the source changes and the response of river water to climate change, waters in mainstream and tributaries in Yellow River Basin were sampled from July to August 2012, and temporal and spatial variations of hydrogen and oxygen isotope values in water samples were analyzed. The results showed that (1) Excluding source water, the values for hydrogen, oxygen isotope, and d excess in mainstream waters in Yellow River ranged from-97.2‰ to-62.9‰ with mean value of-72.2‰, and from-13.0‰ to-8.7‰ with mean value of-9.9‰, and from 4.1‰ to 11.0‰ with mean value of 7.0‰, respectively. For tributary water, the values for hydrogen and oxygen isotope varied from-103.8‰ to-30.5‰ with mean value of-68.9‰ and from-13.7‰ to-1.5‰ with mean value of-9.2‰, respectively, and the d excess varied between-18.5‰ and 13.2‰ with mean value of 4.5‰; (2) The hydrogen and oxygen isotope values in water from the upper-stream of Lanzhou station and middle-stream of Yellow river were more negative than those of water from upper-stream between Lanzhou station and Toudaoguai station and the low-stream, while the d excess values decreased gradually along the flow path; (3) The Na⁺/Cl^- molar ratios varied from 0.94 to 3.02. The mean value of Na⁺/Cl^- molar ratio was 1.02 in source water, and 1.58 in mainstream water above Lanzhou station, and 1.30 in mainstream water between Lanzhou station and Toudaoguai station, and 1.79 in middle-stream water and 1.41 in low-stream water. The negative correlation between Na⁺/Cl^- molar ratio and oxygen isotope values of river water indicated that the Yellow River waters were mainly controlled by atmospheric deposition, groundwater recharge and evaporation; (4) Compared with results of previous studies, it was found that since 2000, the annual water flux of Yellow River increased gradually, the second-evaporation effect on the upper-stream river water decreased, and the evaporation effect on middle and low stream water also decreased, indicating that the climate in Yellow River Basin was becoming less dry.

Key words： Yellow River Basin hydrogen and oxygen isotope atmospheric deposition climate change

收稿日期: 2016-09-27

PACS:	X522
	P597

基金资助:

国家自然科学基金资助项目（41173030，41573095）

通讯作者: 张东,副教授,zhangdong@hpu.edu.cn;赵志琦,研究员,zhaozhiqi@vip.skleg.cn E-mail: zhangdong@hpu.edu.cn;zhaozhiqi@vip.skleg.cn

作者简介: 范百龄(1986-),男,安徽安庆人,副教授,博士,主要从事地表物质循环研究.发表论文8篇.

引用本文:

范百龄, 张东, 陶正华, 赵志琦. 黄河水氢、氧同位素组成特征及其气候变化响应[J]. 中国环境科学, 2017, 37(5): 1906-1914. FAN Bai-ling, ZHANG Dong, TAO Zheng-hua, ZHAO Zhi-qi. Compositions of hydrogen and oxygen isotope values of Yellow River water and the response to climate change. CHINA ENVIRONMENTAL SCIENCECE, 2017, 37(5): 1906-1914.

链接本文:

http://manu36.magtech.com.cn/Jweb_zghjkx/CN/ 或 http://manu36.magtech.com.cn/Jweb_zghjkx/CN/Y2017/V37/I5/1906

[1]	丁悌平,高建飞,石国钰,等.长江水氢、氧同位素组成的时空变化及其环境意义 [J]. 地质学报, 2013,87(5):661-676.
[2]	李亚举,张明军,王圣杰,等.我国大气降水中稳定同位素研究进展 [J]. 冰川冻土, 2011,33(3):624-633.
[3]	章新平,刘晶淼,田立德,等.亚洲降水中δ18O沿不同水汽输送路径的变化 [J]. 地理学报, 2004,59(5):699-708.
[4]	Craig H. Isotopic variations in meteoric waters [J]. Science, 1961,133(3465):1702-1703.
[5]	陈粉丽,张明军,马潜,等.兰州及其周边区域大气降水δ18O特征及其水汽来源 [J]. 环境科学, 2013,34(10):3755-3763.
[6]	余武生,马耀明,孙维贞,等.青藏高原西部降水中δ18O变化特征及其气候意义 [J]. 科学通报, 2009,54(15):2131-2139.
[7]	Hoefs J. Stable isotope geochemistry [M]. Springer-Verlag, 1980:102-107.
[8]	Allison G B. The relationship between 18O and deuterium in water in sand columns undergoing evaporation [J]. Journal of Hydrology, 1982,55:163-169.
[9]	苏小四,林学钰,廖资生,等.黄河水δ18O、δD和3H的沿程变化特征及其影响因素研究 [J]. 地球化学, 2003,32(4):349-357.
[10]	王文科,孔金玲,段磊,等.黄河流域河水与地下水转化关系研究 [J]. 中国科学E辑:技术科学, 2004,34(S1):23-33.
[11]	陈静生,王飞越,何大伟.黄河水质地球化学 [J]. 地学前缘, 2006,13(1):58-73.
[12]	李春晖,郑小康,杨志峰,等.黄河天然径流量变化趋势及其影响分析 [J]. 北京师范大学学报(自然科学版), 2009,45(1):80-85.
[13]	穆兴民,李靖,王飞,等.黄河天然径流量年际变化过程分析 [J]. 干旱区资源与环境, 2003,17(2):1-5.
[14]	苏小四,吴晓芳,林学钰,等.黄河水主要化学组分与δ13C的沿程变化特征 [J]. 人民黄河, 2006,28(5):29-31,80.
[15]	高建飞,丁悌平,罗续荣,等.黄河水氢、氧同位素组成的空间变化特征及其环境意义 [J]. 地质学报, 2011,85(4):596-602.
[16]	苏小四,林学钰.包头平原地下水水循环模式及其可更新能力的同位素研究 [J]. 吉林大学学报(地球科学版), 2003,33(4):503-508,529.
[17]	汪敬忠,吴敬禄,曾海鳌,等.内蒙古河套平原水体同位素及水化学特征 [J]. 地球科学与环境学报, 2013,35(4):104-112.
[18]	高晶,郝爱兵,魏亚杰,等.河套平原中东部地下水的环境同位素特征分析 [J]. 水文地质工程地质, 2009,36(3):55-58.
[19]	王健,王亮,张龙军.地下水灌溉回水对黄河流域化学风化CO2消耗估算的影响 [J]. 中国海洋大学学报(自然科学版), 2014,44(9):89-97.
[20]	Wang L, Hu F, Yin L, et al. Hydrochemical and isotopic study of groundwater in the Yinchuan plain, China [J]. Environmental Earth Sciences, 2013,69(6):2037-2057.
[21]	曹金亮,韩颖,袁新华,等.天桥泉域岩溶水系统水动力场、水化学场特征分析 [J]. 中国岩溶, 2005,24(4):312-317.
[22]	韩颖.晋陕蒙接壤地区岩溶地下水与黄河水环境同位素特征分析 [J]. 中国岩溶, 2002,21(4):52-58.
[23]	林良俊,王金生.晋陕峡谷地区岩溶地下水的同位素及水化学分析 [J]. 工程勘察, 2004,(4):27-30.
[24]	林良俊,王金生,林学钰.晋陕峡谷地区北段岩溶地下水流特征分析 [J]. 地球学报, 2004,25(6):665-670.
[25]	张江华,梁永平,王维泰,等.硫同位素技术在北方岩溶水资源调查中的应用实例 [J]. 中国岩溶, 2009,28(3):235-241.
[26]	臧红飞,贾振兴,郑秀清,等.柳林泉域岩溶水水化学及碳硫同位素特征 [J]. 水电能源科学, 2013,31(12):28-32.
[27]	Fan B L, Zhao Z Q, Tao F X, et al. Characteristics of carbonate, evaporite and silicate weathering in Huanghe River basin: A comparison among the upstream, midstream and downstream [J]. Journal of Asian Earth Sciences, 2014,96:17-26.
[28]	张东,刘丛强,汪福顺,等.农业活动干扰下地下水无机碳循环过程研究 [J]. 中国环境科学, 2015,35(11):3359-3370.
[29]	李孝廉,郝俊卿,王雁林.黄河流域三水转化关系及其模式探讨 [J]. 干旱区地理, 2010,33(4):607-614.
[30]	Yao Z, Liu J, Huang H, et al. Characteristics of isotope in precipitation, river water and lake water in the Manasarovar basin of Qinghai-Tibet Plateau [J]. Environmental Geology, 2009,57(3): 551-556.
[31]	Cui B L, Li, X Y. Stable isotopes reveal sources of precipitation in the Qinghai Lake Basin of the northeastern Tibetan Plateau [J]. Science of Total Environment, 2015,527-528:26-37.
[32]	李小飞,张明军,王圣杰,等.黄河流域大气降水氢、氧稳定同位素时空特征及其环境意义 [J]. 地质学报, 2013,87(2):269-277.
[33]	Li F, Pan G, Tang C, et al. Recharge source and hydrogeochemical evolution of shallow groundwater in a complex alluvial fan system, southwest of North China Plain [J]. Environmental Geology, 2007,55(5):1109-1122.
[34]	Froehlich K, Gibson J J, Aggarwal P. Deuterium excess in precipitation and its climatological significance [C]//Study of Environmental Change Using Isotope Techniques. Proc. Intern. Conf. 2001:54-66.