清洁大气背景下贵阳空气质量变化及气象作用

Abstract
Figure/Table
References
Related Citation (15)

Download: PDF (535 KB) HTML (1 KB)
Export: BibTeX | EndNote (RIS)

Abstract Regional changes of urban air quality and meteorological effects were statistically analyzed based on environmental monitoring and meteorological observation data from 2013 to 2016 in the paper. In the recent 4years, annual average concentrations of SO₂, NO₂, O_{3_8h}, PM₁₀, PM_2.5 and CO were respectively (20.78±19.71), (28.32±9.59), (107.59±27.54), (67.56±34.32), (42.53±24.52)μg/m³ and (0.74±0.22) mg/m³ in Guiyang. Except for concentrations of SO₂ close or exceeding central and eastern China, other air compositions kept in low levels. Ambient O₃ concentrations significantly increased, while other air pollutant level declined with the similar patterns of inter-annual, monthly and diurnal variations with central and eastern China. The significant differences of air pollutants existed among industrial, residential and suburban areas with industrial area > residential area > suburb for particulate matter, SO₂, NO₂ and CO as well as suburb > residential area > Industrial area for surface O₃ concentrations, reflecting impact of human activities on air quality. Air compound pollutants O₃ and PM_2.5 presented positive correlation in summer and but negative correlation in winter. Air temperature, boundary layer height, solar radiation and air pressure had significant impacts on pollutant concentrations, while relative humidity and wind speed had the weak influences, differently from wind speed dominating changes of air quality in central and eastern China. In summer, rainy season in Guiyang, PM_2.5 hygroscopic growth was weak in light or moderate precipitation intensity with the obvious aerosol wash-out by large and heavy rainfall; both PM_2.5 hygroscopic growth and removal of precipitation were more remarkable in the dry and cold winter.

Key words： air quality Guiyang atmospheric pollutants meteorological conditions Yunnan-Guizhou Plateau

Received: 04 May 2017

X513

	Service

	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	SHU ZHUO-zhi
	ZHAO Tian-liang
	ZHENG Xiao-bo
	QIU Yu-jun
	SHI Ren-rui
	JIA Meng-wei

Cite this article:

SHU ZHUO-zhi,ZHAO Tian-liang,ZHENG Xiao-bo等. Air quality variations and meteorological drivers of Guiyang city in clean atmospheric environment[J]. CHINA ENVIRONMENTAL SCIENCECE, 2017, 37(12): 4460-4468.

URL:

http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2017/V37/I12/4460

[1]	Flocas H, Kelessis A, Helmis C, et al. Synoptic and local scale atmospheric circulation associated with air pollution episodes in an urban Mediterranean area[J]. Theoretical and Applied Climatology, 2009,95(3):265-277.
[2]	Ragosta M, Caggiano R, Macchiato M, et al. Trace elements in daily collected aerosol:Level characterization and source identification in a four-year study[J]. Atmospheric Research, 2008,89(1/2):206-217.
[3]	Whiteaker J R, Suess D T, Prather K A. Effects of meteorological conditions on aerosol composition and mixing state in Bakersfield, CA[J]. Environmental Science & Technology, 2002,36(11):2345.
[4]	Chan C K, Yao X. Air pollution in mega cities in China[J]. Atmospheric Environment, 2008,42(1):1-42.
[5]	李小飞,张明军,王圣杰,等.中国空气污染指数变化特征及影响因素分析[J]. 环境科学, 2012,33(6):1936-1943.
[6]	Luo Y, Zheng X, Zhao T, et al. A climatology of aerosol optical depth over China from recent 10 years of MODIS remote sensing data[J]. International Journal of Climatology, 2012,34(3):863-870.
[7]	赵子菁,魏永杰,张祥志,等.南京市霾天气与主要气象条件的相关分析[J]. 中国环境科学, 2015,35(12):3570-3580.
[8]	刘咸德,李军,赵越,等.北京地区大气颗粒物污染的风向因素研究[J]. 中国环境科学, 2010,30(1):1-6.
[9]	刘建,吴兑,范绍佳,等.前体物与气象因子对珠江三角洲臭氧污染的影响[J]. 中国环境科学, 2017,37(3):813-820.
[10]	杨孝文,周颖,程水源,等.北京冬季一次重污染过程的污染特征及成因分析[J]. 中国环境科学, 2016,36(3):679-686.
[11]	许亚宣,李小敏,于华通,等.邯郸市大气复合污染特征的监测研究[J]. 环境科学学报, 2015,35(9):2710-2722.
[12]	Parrish D D, Zhu T. Clean Air for Megacities[J]. Science, 2009,326(5953):674-675.
[13]	Zhang Y H, Hu M, Zhong L J, et al. Regional Integrated Experiments on Air Quality over Pearl River Delta 2004(PRIDE-PRD2004):Overview[J]. Atmospheric Environment, 2008,42(25):6157-6173.
[14]	朱彤,尚静,赵德峰.大气复合污染及灰霾形成中非均相化学过程的作用[J]. 中国科学:化学, 2010,40(12):1731-1740.
[15]	马金珠,刘永春,马庆鑫,等.大气非均相反应及其环境效应[J]. 环境化学, 2011,30(1):97-119.
[16]	陈楠,全继宏,田一平,等.灰霾期间武汉城市区域大气污染物的理化特征[J]. 中国环境监测, 2016,32(2):20-25.
[17]	张桂芹,焦红云,齐鸣,等.济南市灰霾期大气复合污染特征分析[J]. 山东建筑大学学报, 2012,27(1):84-87.
[18]	徐鹏,郝庆菊,吉东生,等.重庆市北碚城区大气污染物浓度变化特征观测研究[J]. 环境科学, 2014,35(3):820-829.
[19]	郑小波,王学锋,罗宇翔,等.云贵高原1961-2006年大气能见度和消光因素变化趋势及原因[J]. 生态环境学报, 2010,19(2):314-319.
[20]	Zhao T, Liu D, Zheng X, et al. Revealed variations of air quality in industrial development over a remote plateau of Southwest China:an application of atmospheric visibility data[J]. Meteorology & Atmospheric Physics, 2016,128(6):1-9.
[21]	刘娜,冯新斌, Landis Matthew,等.贵阳市大气颗粒物PM2.5污染特征及气象参数的影响[J]. 地球与环境, 2014,42(3):311-315.
[22]	杜德艳,李金娟,陶芸,等.贵阳市PM2.5微观特征的季节变化分析[J]. 环境科学学报, 2015,35(6):1645-1650.
[23]	Liu S Y, Liang X Z. Observed diurnal cycle climatology of planetary boundary layer height.[J]. Journal of Climate, 2010, 23(21):5790-5809.
[24]	杜川利,唐晓,李星敏,等.城市边界层高度变化特征与颗粒物浓度影响分析[J]. 高原气象, 2014,33(5):1383-1392.
[25]	吉东生,王跃思,孙扬,等.北京大气中SO2浓度变化特征[J]. 气候与环境研究, 2009,14(1):69-76.
[26]	于洲,刘寿东,王咏薇,等.杭州市2014年城区大气污染物浓度变化特征观测分析[J]. 科学技术与工程, 2016,16(16):95-104.
[27]	廖志恒,孙家仁,范绍佳,等.2006~2012年珠三角地区空气污染变化特征及影响因素[J]. 中国环境科学, 2015,35(2):329-336.
[28]	唐宜西,张小玲,徐敬,等.北京城区和郊区本底站大气污染物浓度的多时间尺度变化特征[J]. 环境科学学报, 2016,36(8):2783-2793.
[29]	王红丽.上海市光化学污染期间挥发性有机物的组成特征及其对臭氧生成的影响研究[J]. 环境科学学报, 2015,35(6):1603-1611.
[30]	刘建,吴兑,范绍佳,等.前体物与气象因子对珠江三角洲臭氧污染的影响[J]. 中国环境科学, 2017,37(3):813-820.
[31]	赵辉,郑有飞,魏莉,等.G20峰会期间杭州及周边地区空气质量的演变与评估[J]. 中国环境科学, 2017,37(6):2016-2024.
[32]	周勤迁,潘月鹏,王剑,等.黑龙江海伦农业区冬春PM2.5和气态污染物污染特征[J]. 中国环境科学, 2014,34(4):844-851.
[33]	GB3095-2012环境空气质量标准[S].
[34]	赵辉,郑有飞,徐静馨,等.中国典型城市大气污染物浓度时空变化特征分析[J]. 地球与环境, 2016,44(5):549-556.
[35]	郭胜利,黄军,王希,等.南京市大气颗粒物污染特征及影响因素分析[J]. 科学技术与工程, 2015,15(13):226-231.
[36]	陈源,谢绍东,罗彬.成都市大气细颗粒物组成和污染特征分析(2012-2013年)[J]. 环境科学学报, 2016,36(3):1021-1031.
[37]	刘永林,钟明洋,孙启民,等.重庆市都市功能核心区秋季大气污染物时空分布特征[J]. 环境科学学报, 2016,36(7):2344-2354.
[38]	梁碧玲,张丽,赖鑫,等.深圳市臭氧污染特征及其与气象条件的关系[J]. 气象与环境学报, 2017,33(1):66-71.
[39]	Li Y, Chen Q, Zhao H, et al. Variations in PM10, PM2.5 and PM1.0 in an Urban Area of the Sichuan Basin and Their Relation to Meteorological Factors[J]. Atmosphere, 2015,6(1):150-163.
[40]	贾梦唯,赵天良,张祥志,等.南京主要大气污染物季节变化及相关气象分析[J]. 中国环境科学, 2016,36(9):2567-2577.
[41]	潘月鹏,王跃思,胡波,等.北京奥运时段河北香河大气污染观测研究[J]. 环境科学, 2010,31(1):1-9.
[42]	Jia M, Zhao T, Cheng X, et al. Inverse Relations of PM2.5 and O3 in Air Compound Pollution between Cold and Hot Seasons over an Urban Area of East China[J]. Atmosphere, 2017,8:59.
[43]	Stephens S, Madronich S, Wu F, et al. Weekly patterns of México City's surface concentrations of CO, NOx, PM10 and O3 during 1986-2007[J]. Atmospheric Chemistry & Physics, 2008,8(17):5313-5325.