麦田O<sub>3</sub>干沉降过程及不同沉降通道分配的模拟

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Abstract

Terrestrial ecosystems are not only the major sink for ozone, but also a critical control of surface-level ozone budget. However, due to its deleterious effects, plant functioning is affected by the ozone absorbed. It is thus very necessary to predict total ozone deposition to ecosystems and partition the different deposition pathways (stomatal pathway and non-stomatal pathway). Based on observations of the ozone dry deposition of winter wheat and bare-soil field in Nanjing by the eddy-correlation system, the Surfatm-O₃ dry deposition model were added in order to modify and validate parameters of the leaf stomatal resistance (R_s^leaf), soil resistance (R_soil) and cuticular resistance (R_cut). Then the simulations of the total ozone flux (F_O3) of main growth stages in Winter Wheat, dry deposition velocity (V_d) and their distributions of different deposition pathways were carried out, and the impacts of chemical reactions between NO from the soil and ozone on the ozone dry deposition process were also analyzed indirectly. The results showed the simulations and measurements of F_O3 and V_d had the similar trend, and the average values of measured V_d and modelled V_d were 0.39 and 0.37cm/s, respectively. Compared with measurements, the simulations underestimated by 5.3%. The average non-stomatal deposition pathway (cuticular deposition and soil deposition) is the main pathway of ozone dry deposition, accounting for 68.8% of the total ozone flux, in which cuticular deposition was accounted for 46.7% of non-stomatal deposition. The average green and yellow leaf stomatal deposition accounted for 28.6% and 2.6% of the total ozone flux respectively. During the daytime, the proportion of non-stomatal deposition decreased to 58.8%, and the ratios of green and yellow leaf stomatal deposition increased, accounting for 37.7% and 3.5% of the total ozone flux, respectively. During the nighttime, cuticular deposition and soil deposition accounted for 64.3% and 35.7% of total ozone flux, respectively. The soil NO emission affected the dry ozone deposition process by ozone chemical reaction, which should be considered in the future ozone dry deposition model.

Key words： Surfatm-O₃ model winter wheat field ozone dry deposition different deposition pathways simulation

Received: 19 June 2017

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	Articles by authors
	XU Jing-xin
	ZHENG You-fei
	MAI Bo-ru
	ZHAO Hui
	CHU Zhong-fang
	HUANG Ji-qing
	YUAN Yue

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XU Jing-xin,ZHENG You-fei,MAI Bo-ru等. Simulating and partitioning ozone flux in winter wheat field: the Surfatm-O₃ model[J]. CHINA ENVIRONMENTAL SCIENCECE, 2018, 38(2): 455-470.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2018/V38/I2/455

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