调水调沙对黄河口颗粒态金属分布的影响

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Abstract Suspended particulate matter (SPM) samples were collected in the Huanghe (Yellow River) estuary before, during and after the Water-Sediment Regulation Scheme (WSRS) in June-July 2009. The concentrations of metal elements (Al, Fe, Mn, Cr, Cu, Ni, V, Zn) were determined by ICP-AES after digestion. Multivariate statistical methods were used to discuss the impact of the WSRS on the variability of particulate heavy metal concentrations and the pollution status in the Huanghe estuary. The results indicated that the concentrations of particulate heavy metals increased during the WSRS and decreased with the increase in salinity in the estuary. The variability of particulate metal concentrations reduced significantly after the normalization by Al, indicating the effects of grain size. Enrichment factor (EF) results showed that Cu and Zn were relatively enriched and the pollution was intensified after the WSRS. Concentrations of particulate metals in the study area were mainly controlled by source geology and provenance, as well as affected by human activity.

Key words： particulate heavy metal distribution pollution water-sediment regulation event Huanghe (Yellow River) estuary

Received: 18 September 2017

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	FU Xiao-ming
	REN Jing-ling
	XIN Cheng-lin
	ZHANG Gui-ling
	LIU Zhe

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FU Xiao-ming,REN Jing-ling,XIN Cheng-lin等. Impacts of water-sediment regulation event on the distributions of particulate metals in the Huanghe (Yellow River) estuary[J]. CHINA ENVIRONMENTAL SCIENCECE, 2018, 38(5): 1867-1877.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2018/V38/I5/1867

[1]	张丽洁,王贵,姚德,等.近海沉积物重金属研究及环境意义[J]. 海洋地质前沿, 2003,19(3):6-9.
[2]	刘广深,曾毅强.陆地生态系统中汞的迁移与富集研究的重要意义[J]. 四川环境, 1996,13(4):216-217.
[3]	Li X, Wai O W H, Li Y S, et al. Heavy metal distribution in sediment profiles of the Pearl River estuary, South China[J]. Applied Geochemistry, 2000,15(5):567-581.
[4]	Turner A, Millward G E. Suspended Particles:Their Role in Estuarine Biogeochemical Cycles[J]. Estuarine Coastal & Shelf Science, 2002,55(6):857-883.
[5]	陈静生,王飞越,陈江麟.论小于63μm粒级作为水体颗粒物重金属研究介质的合理性及有关粒级转换模型研究[J]. 环境科学学报, 1994,14(4):419-425.
[6]	刘昌岭,张经.颗粒态重金属通过河流与大气向海洋输送[J]. 海洋环境科学, 1996,15(4):68-76.
[7]	Nesbitt H W, Young G M. Early proterozoic climates and plate motions inferred from major element chemistry of lutites[J]. Nature, 1982,299(5885):715-717.
[8]	王开荣.黄河调水调沙对河口及其三角洲的影响和评价[J]. 泥沙研究, 2005,6:29-33.
[9]	Huang W W, Jing Z, Zhou Z H. Particulate element inventory of the Huanghe (Yellow River):A large, high-turbidity river[J]. Geochimica Et Cosmochimica Acta, 1992,56(10):3669-3680.
[10]	Yang S, Jung H S, Li C. Two unique weathering regimes in the Changjiang and Huanghe drainage basins:geochemical evidence from river sediments[J]. Sedimentary Geology, 2004,164(1):19-34.
[11]	Qiao S, Yang Z, Pan Y, et al. Metals in suspended sediments from the Changjiang (Yangtze River) and Huanghe (Yellow River) to the sea, and their comparison[J]. Estuarine Coastal & Shelf Science, 2007,74(3):539-548.
[12]	水利部黄河水利委员会编.黄河泥沙公报[Z]. 2010.
[13]	Wang Z W, Ren J L, Zhang G L, et al. Behavior of dissolved aluminum in the Huanghe (Yellow River) and its estuary:Impact of human activities and sorption processes[J]. Estuarine Coastal & Shelf Science, 2015,153:86-95.
[14]	Bordas F, Bourg A. Effect of Solid/Liquid Ratio on the Remobilization of Cu, Pb, Cd and Zn from Polluted River Sediment[J]. Water, Air, & Soil Pollution, 2001,128(3):391-400.
[15]	Atkinson C A, Jolley D F, Simpson S L. Effect of overlying water pH, dissolved oxygen, salinity and sediment disturbances on metal release and sequestration from metal contaminated marine sediments[J]. Chemosphere, 2007,69(9):1428-1437.
[16]	黄薇文,张经,陆贤崑.黄河口地区底质中重金属的分布特征、污染评价及其与泥沙运动的关系[J]. 环境科学, 1985,6(4):31-36.
[17]	何江,王新伟,李朝生,等.黄河包头段水-沉积物系统中重金属的污染特征[J]. 环境科学学报, 2003,23(1):53-57.
[18]	Zhang J, Huang W W, Liu M G, et al. Drainage basin weathering and major element transport of two large Chinese rivers (Huanghe and Changjiang)[J]. Journal of Geophysical Research, 1990, 95(C8):13277-13288.
[19]	辛成林,任景玲,张桂玲,等.黄河下游水体悬浮颗粒物中金属元素的地球化学行为[J]. 中国环境科学, 2015,35(10):3127-3134.
[20]	Sondi I, Jura?i? M, Pravdi? V. Sedimentation in a disequilibrium river-dominated estuary:the Raša River Estuary (Adriatic Sea, Croatia)[J]. Sedimentology, 1995,42(5):769-782.
[21]	Che Y, He Q, Lin W Q. The distributions of particulate heavy metals and its indication to the transfer of sediments in the Changjiang Estuary and Hangzhou Bay, China[J]. Marine Pollution Bulletin, 2003,46(1):123-31.
[22]	Soto-Jiménez M F, Páez-Osuna F. Distribution and Normalization of Heavy Metal Concentrations in Mangrove and Lagoonal Sediments from Mazatlán Harbor (SE Gulf of California)[J]. Estuarine Coastal & Shelf Science, 2001,53(3):259-274.
[23]	黄薇文,张经,刘敏光,等.黄河口底质中重金属的存在形式[J]. 中国海洋大学学报自然科学版, 1985,15(1):137-145.
[24]	张晓琳.长江口、黄河口及邻近海域重金属的分布特征及影响因素研究[D]. 青岛:中国海洋大学, 2013:27-39.
[25]	辛成林,任景玲,张桂玲,等.海南东部河流、河口及近岸水域颗粒态重金属的分布及污染状况[J]. 环境科学, 2013,34(4):1315-1323.
[26]	Prego R, Belzunce M J, Cobelo A, et al. Particulate metal in the Ulla River estuary:State and sources of contamination (Arosa Ria, NW Iberian Peninsula)[J]. Ciencias Marinas, 2008,34(3):381-388.
[27]	Song Y X, Ji J F, Mao C P, et al. Heavy metal contamination in suspended solids of Changjiang River-environmental implications[J]. Geoderma, 2010,159(3/4):286-295.
[28]	Zhang J, Liu C L. Riverine composition and estuarine geochemistry of particulate metals in China-Weathering features, anthropogenic impact and chemical fluxes[J]. Estuarine Coastal & Shelf Science, 2002,54(6):1051-1070.
[29]	Singh M, Müller G, Singh I B. Geogenic distribution and baseline concentration of heavy metals in sediments of the Ganges River, India[J]. Journal of Geochemical Exploration, 2003,80(1):1-17.
[30]	Yi?iterhan O, Murray J W. Trace metal composition of particulate matter of the Danube River and Turkish rivers draining into the Black Sea[J]. Marine Chemistry, 2008,111(1):63-76.
[31]	Presley B J, Trefry J H, Shokes R F. Heavy metal inputs to Mississippi Delta sediments[J]. Water, Air, & Soil Pollution, 1980,13(4):481-494.
[32]	田均良,李雅琦,陈代中.中国黄土元素背景值分异规律研究[J]. 环境科学学报, 1991,11(3):253-262.
[33]	茅志昌.长江河口盐水入侵锋研究[J]. 海洋与湖沼, 1995,26(6):643-649.
[34]	Zhang J, Huang W W, Wang Q. Concentration and partitioning of particulate trace metals in the Changjiang (Yangtze River)[J]. Water, Air, & Soil Pollution, 1990,52(1):57-70.
[35]	易中周.重金属污染物在水体中的络合效应[J]. 红河学院学报, 1999,1(4):12-14.
[36]	Turner A. Trace-metal partitioning in estuaries:importance of salinity and particle concentration[J]. Marine Chemistry, 1996, 54(1/2):27-39.
[37]	Loring D H. Normalization of heavy-metal data from estuarine and coastal sediments[J]. Ices Journal of Marine Science, 1991, 48(1):101-115.
[38]	刘素美,张经.沉积物中重金属的归一化问题-以Al为例[J]. 海洋学研究, 1998,16(3):48-55.
[39]	Sutherland R A. A comparison of geochemical information obtained from two fluvial bed sediment fractions[J]. Environmental Geology, 2000,39(3):330-341.
[40]	Li Y H. Geochemical cycles of elements and human perturbation[J]. Geochimica Et Cosmochimica Acta, 1981,45(11):2073-2084.
[41]	刘成,王兆印,何耘,等.环渤海湾诸河口潜在生态风险评价[J]. 环境科学研究, 2002,15(5):33-37.
[42]	Sutherland R A. Bed sediment-associated trace metals in an urban stream, Oahu, Hawaii[J]. Environmental Geology, 2000, 39(6):611-627.
[43]	水利部黄河水利委员会,黄河水资源公报[Z]. 2010.
[44]	钟晓兰,周生路,赵其国,等.长三角典型区土壤重金属有效态的协同区域化分析、空间相关分析与空间主成分分析[J]. 环境科学, 2007,28(12):2758-2765.
[45]	朱爱萍,陈建耀,江涛,等.北江流域横石河-翁江沿岸土壤重金属污染特征分析[J]. 中国环境科学, 2015,35(2):506-515.