南京北郊霾天气溶胶化学组分粒径分布特征

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Abstract

Particles were collected during winter and spring by ray β dust instrument, Andersen cascade sampler and analyzed by ion chromatography and carbon analyzer. The results showed that the proportion of SO₄^2-、NO₃^-and NH₄⁺ in fine particles was the highest (77.4%) during hazy days. The spectral of most ions for hazy days showed trimodal distributions. The industrial emission, biomass burning and secondary reaction were the most important pollution sources of ions. OC and EC were enriched in fine particles. A good relation (R²=0.76) between OC and EC suggested that the same source in PM_2.1~10. Ratios of OC and EC indicated that the main sources of carbonaceous particles were vehicle exhaust, coal combustion and biomass burning during hazy days.

Key words： haze aerosol pollution source Nanjing

Received: 14 January 2018

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	Articles by authors
	ZHANG Cheng
	YU Xing-na
	AN Jun-lin
	LI Yan
	ZHAO Rui-dong
	ZHAO Bo
	XIAO Wei-sheng

Cite this article:

ZHANG Cheng,YU Xing-na,AN Jun-lin等. Distribution characteristics of chemical components in aerosol during haze days in north suburban Nanjing[J]. CHINA ENVIRONMENTAL SCIENCECE, 2018, 38(8): 2873-2881.

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http://www.zghjkx.com.cn/EN/ OR http://www.zghjkx.com.cn/EN/Y2018/V38/I8/2873

[1]	吴兑.大城市区域霾与雾的区别和灰霾天气预警信号发布[J]. 环境科学与技术, 2008,31(9):1-7.
[2]	高歌.1961~2005年中国霾日气候特征及变化分析[J]. 地理学报, 2008,63(7):761-768.
[3]	Nel A. Atmosphere. Air pollution-related illness:effects of particles[J]. Science, 2005,308(5723):804.
[4]	Kang C M, Lee H S, Kang B W, et al. Chemical characteristics of acidic gas pollutants and PM2.5 species during hazy episodes in Seoul, South Korea[J]. Atmospheric Environment, 2004,38(28):4749-4760.
[5]	于兴娜,马佳,朱彬,等.南京北郊秋冬季相对湿度及气溶胶理化特性对大气能见度的影响[J]. 环境科学, 2015,36(6):1919-1925.
[6]	Kim K W, Kim Y J, Bang S Y. Summer time haze characteristics of the urban atmosphere of Gwangju and the rural atmosphere of Anmyon, Korea[J]. Environmental Monitoring & Assessment, 2008,141(1-3):189-199.
[7]	陈欢欢,吴兑,谭浩波,等.珠江三角洲2001~2008年灰霾天气过程特征分析[J]. 热带气象学报, 2010,26(2):147-155.
[8]	师远哲,安俊琳,王红磊,等.南京青奥会期间不同天气条件下大气气溶胶中水溶性离子的分布特征[J]. 环境科学, 2016,37(12):4475-4481.
[9]	Li Q F, Wang L L, Jayanty R K M, et al. Organic and elemental carbon in atmospheric fine particulate matter in an animal agriculture intensive area in North Carolina:estimation of secondary organic carbon concentrations[J]. Open Journal of Air Pollution, 2013,2(1):7-18.
[10]	Huang L, Brook J R, Zhang W, et al. Stable isotope measurements of carbon fractions (OC/EC) in airborne particulate:a new dimension for source characterization and apportionment[J]. Atmospheric Environment, 2006,40(15):2690-2705.
[11]	黄怡民,刘子锐,陈宏,等.北京夏冬季霾天气下气溶胶水溶性离子粒径分布特征[J]. 环境科学, 2013,34(4):1236-1244.
[12]	翟宇虹,黄晓锋,张丽,等.深圳大气气溶胶中水溶性有机物粒径分布特征[J]. 中国环境科学, 2015,35(11):3211-3216.
[13]	蒋斌,陈多宏,王伯光,等.鹤山大气超级站旱季单颗粒气溶胶化学特征研究[J]. 中国环境科学, 2016,36(3):670-678.
[14]	叶香,姜爱军,张军,等.南京市大气能见度的变化趋势及特征[J]. 气象科学, 2011,31(3):325-331.
[15]	葛顺,汤莉莉,秦玮,等.南京地区秋季灰霾天气特征及其水溶性离子分析[J]. 环境科学与技术, 2015,38(2):99-104.
[16]	周瑶瑶,马嫣,郑军,等.南京北郊冬季霾天PM2.5水溶性离子的污染特征与消光作用研究[J]. 环境科学, 2015,36(6):1926-1934.
[17]	陈杨,汤莉莉,王壮,等.南京冬季重霾天气过程与颗粒物污染特征[J]. 环境科学与技术, 2015,38(6):74-82.
[18]	GB 3095-2012环境空气质量标准[S].
[19]	吕睿,于兴娜,马佳,等.南京北郊冬春季大气颗粒物中含氮无机水溶性离子组分特征[J]. 生态环境学报, 2017,26(1):129-135.
[20]	邹嘉南,安俊琳,王红磊,等.亚青会期间南京污染气体与气溶胶中水溶性离子的分布特征[J]. 环境科学, 2014,35(11):4044-4051.
[21]	陈永桥,张逸,张晓山.北京城乡结合部气溶胶中水溶性离子粒径分布和季节变化[J]. 生态学报, 2005,25(12):3231-3236.
[22]	Wang Y, Zhuang G, Tang A, et al. The ion chemistry and the source of PM2.5, aerosol in Beijing[J]. Atmospheric Environment, 2005,39(21):3771-3784.
[23]	刘景云,刘子锐,温天雪,等.石家庄秋季一次典型霾污染过程水溶性离子粒径分布特征[J]. 环境科学, 2016,37(9):3258-3267.
[24]	吴琳,沈建东,冯银厂,等.杭州市灰霾与非灰霾日不同粒径大气颗粒物来源解析[J]. 环境科学研究, 2014,27(4):373-381.
[25]	银燕,童尧青,魏玉香,等.南京市大气细颗粒物化学成分分析[J]. 大气科学学报, 2009,32(6):723-733.
[26]	Sun Y, Zhuang G, Wang Y, et al. The air-borne particulate pollution in Beijing-concentration, composition, distribution and sources[J]. Atmospheric Environment, 2004,38(35):5991-6004.
[27]	Mukerjee S, Shadwick D S, Smith L A, et al. Techniques to assess cross-border air pollution and application to a US-Mexico border region[J]. Science of the Total Environment, 2001,276(1-3):205.
[28]	Zhang R, Jing J, Tao J, et al. Chemical characterization and source apportionment of PM2.5 in Beijing:seasonal perspective[J]. Atmospheric Chemistry & Physics Discussions, 2013,13(14):7053-7074.
[29]	Zheng X, Liu X, Zhao F, et al. Seasonal characteristics of biomass burning contribution to Beijing aerosol[J]. Science in China Series B:Chemistry, 2005,48(5):481-488.
[30]	王红磊,朱彬,安俊琳,等.亚青会期间南京市气溶胶中OC和EC的粒径分布[J]. 环境科学, 2014,35(9):3271-3279.
[31]	李杏茹,王英锋,郭雪清,等.2008年奥运期间北京不同粒径大气颗粒物中元素碳和有机碳的变化特征[J]. 环境科学, 2011,32(2):313-318.
[32]	Turpin B J, Cary R A, Huntzicker J J. An In Situ, Time-Resolved Analyzer for Aerosol Organic and Elemental Carbon[J]. Aerosol Science & Technology, 1990,12(1):161-171.
[33]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of Emissions from Air Pollution Sources. 2. C1through C30Organic Compounds from Medium Duty Diesel Trucks[J]. Environmental Science Technology, 1999,33(10):1578-1587.
[34]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of Emissions from Air Pollution Sources. 5. C1-C32Organic Compounds from Gasoline-Powered Motor Vehicles[J]. Environmental Science & Technology, 2002,36(6):1169.
[35]	Chen Y, Zhi G, Feng Y, et al. Measurements of emission factors for primary carbonaceous particles from residential raw-coal combustion in China[J]. Geophysical Research Letters, 2006,33(20):382-385.
[36]	Schauer J J, Kleeman M J, Cass G R, et al. Measurement of Emissions from Air Pollution Sources. 3. C1-C29Organic Compounds from Fireplace Combustion of Wood[J]. Environmental Science & Technology, 2001,35(9):1716.
[37]	He L Y, Hu M, Huang X F, et al. Measurement of emissions of fine particulate organic matter from Chinese cooking[J]. Atmospheric Environment, 2004,38(38):6557-6564.
[38]	Qiu X, Duan L, Gao J, et al. Chemical composition and source apportionment of PM10 and PM2.5 in different functional areas of Lanzhou, China[J]. 环境科学学报(英文版), 2016,40(2):75.
[39]	段卿,安俊琳,王红磊,等.南京北郊夏季大气颗粒物中有机碳和元素碳的污染特征[J]. 环境科学, 2014,35(7):2460-2467.
[40]	Turpin B J, Huntzicker J J. Identification of secondary organic aerosol episodes and quantitation of primary and secondary organic aerosol concentrations during SCAQS[J]. Atmospheric Environment, 1995, 29(23):3527-3544.
[41]	范忠雨,李友平,杨铮铮,等.成都市PM2.5中有机碳和元素碳的污染特征及来源[J]. 四川环境, 2016,35(2):76-81.
[42]	李英红,段菁春,郑乃嘉,等.兰州大气细颗粒物中有机碳与元素碳的污染特征[J]. 中国科学院大学学报, 2015,32(4):490-497.
[43]	刘凤娴,彭林,白慧玲,等.朔州市市区PM2.5中元素碳、有机碳的分布特征[J]. 环境科学, 2015,36(3):787-793.
[44]	张懿华,王东方,赵倩彪,等.上海城区PM2.5中有机碳和元素碳变化特征及来源分析[J]. 环境科学, 2014,35(9):3263-3270.