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PM2.5 and VOCS emission inventories from cooking in Changchun City |
WU Xue-wei1,2, CHEN Wei-wei1, WANG Kun3, XIU Ai-jun1, ZHANG Shi-chun1, ZHAO Hong-mei1, ZHANG Xue-lei1 |
1. Key Laboratory of Wetland Ecology and Environment, Northeast Institute of Geography and Agroecology, Changchun 130102, China;
2. Univeresity of Chinese Academy of Sciences, Beijing 100049, China;
3. Department of Air Pollution Control, Beijing Municipal Institute of Labour Protection, Beijing 100054, China |
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Abstract Cooking activities are one of important sources of atmospheric pollutants, but few corresponding emission inventory has been published. In this study PM2.5 and VOCS emission inventories from cooking in Changchun City, Northeast China are developed. Based on four different bottom-up methods (i.e., based on population, dining out frequency, amount of edible oil and burner numbers), we collected the cooking activity data in Changchun City, Northeast China for the year of 2014. These data include the population, the frequency of dining out, the amount of edible oil, and the number of burners. The emission factors are obtained through literature review. Then the PM2.5 and VOCS emission inventories from cooking based on the four different methods are developed and their spatial-temporal distributions analyzed. The results show the magnitude of annual cooking PM2.5 emissions in Changchun City are from 183 tons to 770 tons and VOCS emissions between 9 tons and 586 tons in 2014. The PM2.5 and VOCS emission from residential cooking were highest, which accounted for 74% to 81% and 28% to 78% of the total amount, while for 8% to 22% and 3% to 26% from cafeteria cooking and for 8% to 22% and 3% to 26% from commercial cooking. The spatial distribution of cooking emissions show that they are higher in Chaoyang District than in Nanguan District, Lvyuan District, Erdao District, Kuancheng District and Shuangyang District. Based on the temporal variation, emissions from cooking mainly occur from 7 am to 8am, 11:30 am to 12:30 pm, 18:00 pm to 20:00 pm during the day and are higher on Wednesday, Saturday and Sunday during the week. The emissions are higher in winter than other seasons, especially in January, February and December, which accounted for 9.23%, 9.47% and 9.98%. Considering the uncertainty of emission inventory, the VOCS emissions inventory based on the population has the highest uncertainty, and based on edible oil amount the lowest uncertainty. The uncertainties of the PM2.5 and VOCS emissions based on edible oil amount are 31% and 61%, which can act as a reference method to calculate regional cooking emission inventory. This study can provide reference and basis for the formulation of cooking emission inventory specifications in China.
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Received: 15 December 2017
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[1] |
王秀艳,史建武,白志鹏,等.沈阳市烹饪油烟中VOCs排放特征分析[J]. 中国人口·资源与环境, 2011,21(127):364-366.
|
[2] |
Abdullahi K L, Delgado-Saborit J M, Harrison R M. Emissions and indoor concentrations of particulate matter and its specific chemical components from cooking:A review[J]. Atmospheric Environment, 2013,71(2):260-294.
|
[3] |
张玉梅,张卫东,王军玲.大气PM2.5源解析"源清单化学质量平衡法(I-CMB)"模型的建立与应用[J]. 大气科学学报, 2015,38(2):279-284.
|
[4] |
温梦婷,胡敏.北京餐饮源排放细粒子理化特征及其对有机颗粒物的贡献[J]. 环境科学, 2007,28(11):2620-2625.
|
[5] |
Wang G. Chemical Characteristics of Fine Particles Emitted from Different Chinese Cooking Styles[J]. Aerosol & Air Quality Research, 2015,15(6S):2357-2366.
|
[6] |
Wang G, Cheng S, Lang J, et al. Characterization of volatile organic compounds from different cooking emissions[J]. Atmospheric Environment, 2016,145:299-307.
|
[7] |
谭德生,邝元成,刘欣,等.餐饮业油烟的颗粒物分析[J]. 环境科学, 2012,33(6):1958-1963.
|
[8] |
崔彤,程婧晨,何万清,等.北京市典型餐饮企业VOCs排放特征研究[J]. 环境科学, 2015,36(5):1523-1529.
|
[9] |
厉曙光,黄昕.家庭厨房烹调油烟污染的危害[J]. 上海预防医学, 2003,15(2):57-59.
|
[10] |
Huang Y, Ho S S, Ho K F, et al. Characteristics and health impacts of VOCs and carbonyls associated with residential cooking activities in Hong Kong[J]. Journal of Hazardous Materials, 2011,186(1):344-351.
|
[11] |
秦之湄,毛名英,唐文雅,等.基于互联网大数据的城市餐饮源清单高时空分辨研究[C]//秦之湄.2016全国环境信息技术与应用交流大会暨中国环境科学学会环境信息化分会年会论文集, 2016:140-147.
|
[12] |
Roe S M, Spivey M D, Lindquist H C, et al. National emissions inventory for commercial cooking[C]//In Proceedings of the 13th International Emission Inventory Conference, Clearwater, FL, USA, 2004:8-10.
|
[13] |
黄丹雯.烹饪油烟影响PM2.5?[J]. 环境, 2013,(11):69-71.
|
[14] |
北京市政府关于《北京市大气污染防治条例》实施情况的报告(书面)[J]. 北京市人大常委会公报, 2015,260(1):124-130.
|
[15] |
程婧晨,崔彤,何万清,等.北京市典型餐饮企业油烟中醛酮类化合物污染特征[J]. 环境科学, 2015,36(8):2743-2749.
|
[16] |
王桂霞,董雪玲,许立男.餐饮源排放颗粒物的污染特征[C]//王桂霞.Proceedings of conference on environmental pollution and public health (CEPPH 2012). Scientific Research Publishing, USA (美国科研出版社), 2012:691-697.
|
[17] |
秦之湄,唐文雅,尹元畅,等.基于互联网大数据的成都餐饮源细颗粒物排放空间分配研究[J]. 环境科学学报, 2017,38(12):4511-4518.
|
[18] |
尹元畅,蒋燕,王波,等.成都餐饮源PM2.5及VOCs排放因子的探索[J]. 环境监测管理与技术, 2015,27(5):63-67.
|
[19] |
李亚倩,李建军,李海娇.餐饮油烟废气污染及其净化技术进展[J]. 四川化工, 2018,21(1):13-16.
|
[20] |
林立,何校初,邬坚平,等.上海餐饮油烟污染特征研究[J]. 环境科学与技术, 2014,(s2):546-549.
|
[21] |
黄继章,李伟铿,张宝春.广州市餐饮源排放研究[J]. 广州环境科学, 2013,(2):1-2.
|
[22] |
王堃,高佳佳,田贺忠,等.基于POI兴趣点的排放清单空间分配方法[J]. 中国环境科学, 2017,37(6):2377-2382.
|
[23] |
曹国良,张小曳,龚山陵,等.中国区域主要颗粒物及污染气体的排放源清单[J]. 科学通报, 2011,56(3):261-268.
|
[24] |
魏巍,王书肖,郝吉明.中国人为源VOC排放清单不确定性研究[J]. 环境科学, 2011,32(2):305-312.
|
[25] |
长春市统计局.长春统计年鉴-2015[M]. 北京:中国统计出版社, 2015.
|
[26] |
长春市统计局.长春统计年鉴-2014[M]. 北京:中国统计出版社, 2014.
|
[27] |
长春房天下.http://changchun.fang.com/[EB/Z]. 2017-10-14.
|
[28] |
餐饮收入_当期值.http://data.stats.gov.cn/easyquery.htm?cn=A01[EB/Z]. 2017-11-1.
|
[29] |
陈瑶,付静,邵培基.四川师范大学学生食堂消费行为研究[J].管理学家:学术版, 2010,(7):10-19.
|
[30] |
李静,江国虹,潘怡,等.天津居民的就餐饮食行为调查[J]. 营养学报, 2014,36(4):327-330.
|
[31] |
吴芳谷,汪彤,陈虹桥,等.餐饮油烟排放特征[J]. 过程工程学报, 2002,11(2):319-323.
|
[32] |
王秀艳,高爽,周家岐,等.餐饮油烟中挥发性有机物风险评估[J]. 环境科学研究, 2012,25(12):1359-1363.
|
[33] |
Wang X, Shi J, Bai Z, et al. Measurement of VOCs emissions from cooking in the Northeast Area of China[C]//International Conference on Mechanic Automation & Control Engineering. IEEE, 2011:3212-3215.
|
[34] |
柳晓雷,李晓丹,熊安华,等.北京市餐饮油烟排放处理现状和治理对策研究[C]//柳晓雷.中国环境科学学会学术年会论文集(2015), 2015:3112-3116.
|
[35] |
范洪铎.中小餐饮店油烟污染分析及对策[J]. 海峡科学, 2014,(5):23-24.
|
[36] |
饮食业油烟排放标准(试行)[Z]. 2001.
|
[37] |
环评爱好者.http://www.eiafans.com/thread-134416-2-1.html[EB/Z]. 2017-11-13.
|
[38] |
大气挥发性有机物源排放清单编制技术指南(试行)[Z]. 2014.
|
[39] |
张腾,彭林,李颖慧,等.餐饮源油烟中PM2.5的化学组分特征[J]. 环境科学研究, 2016,29(2):183-191.
|
[40] |
舒熳,李云春,曹军骥.不同餐饮源的PM2.5排放特征[C]//2014中国环境科学学会学术年会, 2014:1-8.
|
[41] |
Wang L, Xiang Z, Stevanovic S, et al. Role of Chinese cooking emissions on ambient air quality and human health[J]. Science of the Total Environment, 2017,589:173-181.
|
[42] |
蒋燕,尹元畅,王波,等.成都市川菜烹饪油烟中VOCs排放特征及其对大气环境的影响[J]. 环境化学, 2014,(11):2005-2006.
|
[43] |
周子航,邓也,陆成伟,等.成都市人为源挥发性有机物排放清单及特征[J]. 中国环境监测, 2017,33(3):39-48.
|
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|
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