|
|
Variation characteristics of pollutant concentration in autumn and winter from 2013 to 2019 in Baoding City |
LI Huan-huan1,2, NIU Can2, ZHANG Kai1, LI Jie1, ZHI Min-kang1, LUO Yu-qian1, WANG Tao2, LU Shan-shan3 |
1. State Key Laboratory of Environmental Standards and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; 2. College of Public Health, Hebei University, Baoding 071000, China; 3. Baiyangdian River Basin Ecological Environment Monitoring Center, Hebei University, Baoding 071051, China |
|
|
Abstract In order to deeply understand the air quality of Baoding, Morlet wavelet analysis and Mann-Kendall non-parametric test were utilized for revealling the variation trends, multi-scale changes and mutation characteristics of six conventional air pollutions (PM10, PM2.5, SO2, NO2, CO and O3-8h) annual average concentration and pollution characteristics. Except for O3-8h, the annual average concentrations of pollutants decreased year by year, and the proportion of severe pollution days in the whole year decreased from 31% to 6.6%, showing an overall improvement trend in Baoding. However, the severe pollution days in autumn and winter of 2013~2019 accounted for 81%~97%, and the air pollution in autumn and winter still needs to be paid great attention. The wavelet analysis revealed the obviously periodic variations of pollutant concentrations during autumn and winter time in Baoding City. The periodic oscillations appeared at 20d (quasi-biweekly), 50~90d (intra-seasonal oscillations), and 90~110d (seasonal oscillations). In this time scale, the low-frequency oscillations for the pollutant concentrations were closely related to the low-frequency oscillations of atmospheric condition. The most severe pollution often occurred in December, January and February, which were mainly related to the source emission intensity and relatively stable atmospheric conditions. The mutation points of each pollutant pollution sequence were concentrated in October and March. In the autumn and winter of 2019~2020, NO2 showed the obvious decreasing trend, and the mutation point was one month earlier than previous years, which was directly related to the significant reduction in vehicle emissions during the epidemic, while the times of mutation point for SO2 and CO in the autumn and winter of 2013~2014 and 2015~2016 were similar, this may be related to the incomplete combustion of scattered coal for residential heating in winter. Since the implementation of control measures in Baoding in 2015, such as coal-to-gas, coal-to-electricity, and special treatment of low-quality scattered coal, the difference in the time of the mutation point between the two air pollutions indicated that clean heating measures had obvious effects on reducing the concentration of SO2 and improving air quality.
|
Received: 20 December 2020
|
|
|
|
|
[1] |
Fu G Q, Xu W, Yang R F, et al. The distribution and trends of fog and haze in the North China Plain over the past 30 years[J]. Atmospheric Chemistry and Physics, 2014,14(21):11949-11958.
|
[2] |
Wang M, Shao M, Chen W, et al. Trends of non-methane hydrocarbons (NMHC) emissions in Beijing during 2002~2013[J]. Atmospheric Chemistry and Physics, 2015,14(3):85-94.
|
[3] |
Fu F, Purvis-Roberts K L, Williams B. Impact of the COVID-19 pandemic lockdown on air pollution in 20 major cities around the world[J]. Atmosphere, 2020,11(11):1189.
|
[4] |
Wu Q, Wang Z, Chen H, et al. An evaluation of air quality modeling over the Pearl River Delta during November 2006[J]. Meteorology & Atmospheric Physics, 2012,116(3/4):113-132.
|
[5] |
Guo J, He J, Liu H, et al. Impact of various emission control schemes on air quality using WRF-Chem during APEC China 2014[J]. Atmospheric Environment, 2016,140:311-319.
|
[6] |
Meng Y, Li R, Zhao Y, et al. Chemical characterization and sources of PM2.5 at a high-alpine ecosystem in the Southeast Tibetan Plateau, China[J]. Atmospheric Environment, 2020,235:117645.
|
[7] |
Sibel Cukurluoglu, Ulker Guner Bacanli. Time series analysis for the sulphur dioxide and particulate matter concentrations in the Aegean Region of Turkey[J]. International Journal of Global Warming, 2014,6(2/3):175-193.
|
[8] |
Rahman S, Chen S, Saleem N, et al. Financial development and its moderating role in environmental Kuznets curve:evidence from pakistan[J]. Environmental Science and Pollution Research, 2019,26(19):1-16.
|
[9] |
Wu Y, Guo J, Zhang X, et al. Synergy of satellite and ground based observations in estimation of particulate matter in eastern China[J]. Science of the Total Environment, 2012,433(1):20-30.
|
[10] |
F Chevallier, J J Morcrette, F Chéruy, et al. Use of a neural-network-based long-wave radiative-transfer scheme in the ECMWF atmospheric model[J]. Quarterly Journal of the Royal Meteorological Society, 2000,126(563):761-776.
|
[11] |
李梓铭,孙兆彬,邵勰,等.北京城区PM2.5不同时间尺度周期性研究[J]. 中国环境科学, 2017,37(2):407-415. Li Z M, Sun Z B, Shao X, et al. Using Morlet wavelet analysis to analyze multiple time scale periodically in PM2.5 in Beijing[J]. China Environmental Science, 2017,37(2):407-415.
|
[12] |
Domingues M O, Mendes O, Costa A M D. On wavelet techniques in atmospheric sciences[J]. Advances in Space Research, 2005,35(5):831-842.
|
[13] |
Hermida L, Lopez L, Merino A, et al. Hailfall in southwest france:relationship with precipitation, trends and wavelet analysis[J]. Atmospheric Research, 2015,156:174-188.
|
[14] |
Anil Kumar, Uttam Kumar Rawat, Preeti Singh. Wavelet analysis of atmospheric aerosols as ambient air pollutants[J]. Invertis Journal of Science & Technology, 2018,11(3):132-137.
|
[15] |
孙春媛,李令军,赵文吉,等.基于小波变换的北京市PM2.5时空分布特征及成因分析[J]. 生态环境学报, 2016,25(8):1343-1350. Sun C Y, Li L J, Zhao W J, et al. Temporal and spatial characteristic and factors analysis of PM2.5 on the basis of wavelet transformation in Beijing[J]. Ecology and Environmental Sciences, 2016,25(8):1343-1350.
|
[16] |
鲁凤,钱鹏,胡秀芳,等.基于小波分析与Mann-Kendall法的上海市近12年空气质量变化[J]. 长江流域资源与环境, 2013,22(12):1614-1620. Lu F, Qian P, Hu X F, et al. Air quality changes of Shanghai in recent 12 years based on wavelet analysis and mann-kendall method[J]. Resources and Environment in the Yangtze Basin, 2013,22(12):1614-1620.
|
[17] |
吴小玲,张斌,刘祖涵,等.基于小波变换的上海市近10年SO2指数的变化[J]. 环境科学, 2009,30(8):2193-2198. Wu X L, Zhang B, Ai N S, et al. Wavelet analysis on SO2 pollution index changes of Shanghai in recent 10years[J]. Environmental Science, 2009,30(8):2193-2198.
|
[18] |
王海鹏,张斌,刘祖涵,等.基于小波变换的兰州市近十年空气污染指数变化[J]. 环境科学学报, 2011,31(5):1070-1076. Wang H P, Zhang B, Liu Z H, et al. Waveletanalysis of air pollution index changes in Lanzhou during the last decade[J]. Acta Scientiae Circumstantiae, 2011,31(5):1070-1076.
|
[19] |
Xu Y X, Ren J, He L Y, et al. Study on temporal and spatial distribution of air pollutant concentration based on wavelet analysis[J]. International Core Journal of Engineering, 2019,5(8):1895-2414.
|
[20] |
李慧,王淑兰,张文杰,等.京津冀及周边地区"2+26"城市空气质量特征及其影响因素[J]. 环境科学研究, 2021,34(1):172-184. Li H, Wang S L, Zhang W J, et al. Exposure distribution of air pollutants in Beijing-Tianjin-Hebei region based on monitoring and kriging method[J]. Research of Environmental Sciences, 2021,34(1):172-184.
|
[21] |
梅梅,朱蓉,孙朝阳,等.京津冀及周边"2+26"城市秋冬季大气重污染气象条件及其气候特征研究[J]. 气候变化研究进展, 2019, 15(3):270-281. Mei M, Zhu R, Sun C Y, et al. Study on meteorological conditions for heavy air pollution and its climatic characteristics in "2+26" cities around Beijing-Tianjin-Hebei region in autumn and winter[J]. Climate Change Research, 2019,15(3):270-281.
|
[22] |
刀谞,吉东生,张显,等.京津冀及周边地区采暖季PM2.5化学组分变化特征[J]. 环境科学研究, 2021,34(1):1-10. Dao X, Ji D S, Zhang X, et al. Characteristics of chemical composition of PM2.5 in Beijing-Tianjin-Hebei and its surrounding areas during the heating period[J]. Environmental Science, 2021, 34(1):1-10.
|
[23] |
苟银寅,张凯,李金娟,等.保定市大气污染变化趋势及特征[J]. 环境科学, 2020,41(10):4413-4425. Gou Y Y, Zhang K, Li J J, et al. Variational trend and characteristics of air pollution in Baoding city[J]. Environmental Science, 2020, 41(10):4413-4425.
|
[24] |
郑悦,程方,张凯,等.保定市大气污染特征和潜在输送源分析[J]. 环境科学研究, 2020,33(2):260-270. Zheng Y, Cheng F, Zhang K, et al. Characteristics and potential transport source identification of atmospheric pollution in Baoding city[J]. Research of Environmental Sciences, 2020,33(2):260-270.
|
[25] |
吕文丽,张凯,曹晴,等.烟花爆竹燃放对大气污染物及PM2.5组分影响[J]. 中国环境科学, 2020,40(8):3303-3311. Lü W L, Zhang K, Cao Q, et al. Impacts of fireworks burning on atmospheric pollutants and water-soluble inorganic ions in PM2.5[J]. China Environmental Science, 2020,40(8):3303-3311.
|
[26] |
HJ 633-2012环境空气质量指数(AQI)技术规定(试行)[S]. HJ 633-2012 Technical regulations on ambient air quality index (AQI) (trial)[S].
|
[27] |
Lisa V D H, Deventer M J, Graus M, et al. Aerosol particles during the Innsbruck Air Quality Study (INNAQS):The impact of transient fluxes on total aerosol number exchange[J]. Atmospheric environment, 2018,190(OCT.):389-400.
|
[28] |
Nyikadzino B, Chitakira M, Muchuru S. Rainfall and runoff trend analysis in the Limpopo river basin using the Mann Kendall statistic[J]. Physics and Chemistry of the Earth Parts A/B/C, 2020,117:102870.
|
[29] |
Yue S, Wang C Y. The Mann-Kendall test modified by effective sample size to detect trend in serially correlated hydrological series[J]. Water Resources Management, 2004,18(3):201-218.
|
[30] |
张凯,吕文丽,王婉,等.保定市大气污染来源与燃煤治理成效[J]. 环境科学研究, 2019,2(10):1720-1729. Zhang K, Lü W L, Wang W, et al. Sources of air pollution and effects of coal combustion treatment in Baoding city[J]. Research of Environmental Sciences, 2019,32(10):1720-1729.
|
[31] |
Li K, Jacob D J, Liao H. Anthropogenic dirvers of 2013~2017 trends in summer surface ozone in China[J]. Proceedings of the National Academy of Sciences of the United States of America, 2019,116(2):422-427.
|
[32] |
Tian H, Liu Y, Li Y, et al. An investigation of transmission control measures during the first 50days of the COVID-19 epidemic in China[J]. Science, 2020,368(6491):638-642.
|
[33] |
杨双艳,武炳义,胡景高,等.大气准双周振荡的研究进展[J]. 大气科学学报, 2015,38(6):855-864. Yang S Y, Wu B Y, Hu J G, et al. Research progress of quasi-biweekly oscillation of atmosphere[J]. Transactions of Atmospheric Sciences, 2015,38(6):855-864.
|
[34] |
杨双艳,武炳义,周顺武,等.大气季节内振荡研究进展[J]. 气象科技, 2012,40(6):938-948. Yang S Y, Wu B Y, Zhou S W, et al. Progress in researches on atmospheric intraseasonal oscillation[J]. Meteorological Science and Technology, 2012,40(6):938-948.
|
[35] |
李崇银.大气中的季节内振荡[J]. 大气科学, 1990,15(1):32-45. Li C Y. Intraseasonal oscillation in the atmosphere[J]. Chinese Journal of Atmospheric Sciences, 1990,15(1):32-45.
|
[36] |
李崇银,程胜,潘静.冬季北半球平流层季节内振荡与对流层季节内振荡的关系[J]. 大气科学, 2006,30(5):744-752. Li C Y, Cheng S, Pan J. The relationship between the intraseasonal oscillations in the northern hemisphere during the boreal winter in the stratosphere and troposphere[J]. Chinese Journal of Atmospheric Sciences, 2006,30(5):744-752.
|
[37] |
Sun Y, Jiang Q, Wang Z, et al. Investigation of the sources and evolution processes of severe haze pollution in Beijing in January 2013[J]. Journal of Geophysical Research Atmospheres, 2014,119(7):4380-4398.
|
[38] |
杨旭.京津冀地区空气污染特征与气象成因及其预报研究[D]. 兰州:兰州大学, 2017. Yang X. Research on characteristics of air pollution and its meteorological reasons and forecasting method in Beijing-Tianjin-Hebei region[D]. Lanzhou:Lanzhou University, 2017.
|
[39] |
Duncan B N, Martin R V, Staudt A C, et al. Interannual and seasonal variability of biomass burning emissions constrained by satellite observations[J]. Journal of Geophysical Research:Atmospheres, 2003, 108(D2):4100.
|
[40] |
徐冉,张恒德,杨孝文,等.北京地区秋冬季大气污染特征及成因分析[J]. 环境科学, 2019,40(8):3405-3414. Xu R, Zhang H D, Yang X W, et al. Concentration characteristics of PM2.5 and the causes of heavy air pollution events in Beijing during autumn and winter[J]. Environmental Science, 2019,40(8):3405-3414.
|
[41] |
Zhang R, Zhang Y, Lin H, et al. NOx emission reduction and recovery during COVID-19 in east China[J]. Atmosphere, 2020,11(4):433.
|
[42] |
Xin H, Aijun D, Jian G, et al. Enhanced secondary pollution offset reduction of primary emissions during COVID-19 lockdown in China[J]. National Science Review, 2020.0:1-9.
|
[43] |
Bauwens M, Compernolle S, Stavrakou T, et al. Impact of coronavirus outbreak on NO2 pollution assessed using TROPOMI and OMI observations[J]. Geophysical Research Letters, 2020,47(11):460-472.
|
[44] |
Le T H, Wang Y, Liu L, et al. Unexpected air pollution with marked emission reductions during the COVID-19 outbreak in China[J]. Science, 2020,369(6504):702-706.
|
[45] |
Huang F, Li X, Wang C, et al. PM2.5 Spatiotemporal variations and the relationship with meteorological factors during 2013~2014 in Beijing, China[J]. Plos One, 2015,10(11):1-17.
|
[46] |
Liu L, Zhang J, Du R G, et al. Chemistry of atmospheric fine particles during the COVID-19 pandemic in a megacity of eastern China[J]. Geophysical Research Letters, 2021,48:1-10.
|
|
|
|