Abstract:A quartz crystal microbalance with dissipation (QCM-D) was used to investigate the initial adsorption behavior of biofilm under four kinds of Na+ concentrations. The rigid model and viscoelastic model were fitted to explore the changes in adsorption mass and viscoelasticity with time. The results indicate that both reversible and irreversible adsorption processes occurred in the initial adsorption of biofilm. The formation of irreversible adsorption was promoted when Na+ concentration was 150mmol/L, due to increased zeta potential and net charge reduction in bacterial surfaces. With an increase in Na+ concentration from 2.5mmol/L to 50mmol/L, the adsorption rate increased gradually, which is consistent with the electrostatic double-layer theory. No significant change in the adsorption rate was observed when the concentration was increased to 150mmol/L. The softness of the absorbed layer in the 150mmol/L group was the highest, followed by the 2.5, 10 and 50mmol/L groups. An increase in the viscoelasticity of the layer was also observed during the early adsorption process. With an increase in Na+ concentration, the adsorption mass kept increasing and the viscoelasticity first increased and then remained unchanged.
刘丰, 王前, 吴华南, 徐期勇. 渗滤液中Na+对生物膜形成初期吸附特性的影响[J]. 中国环境科学, 2022, 42(1): 213-219.
LIU Feng, WANG Qian, WU Hua-nan, XU Qi-yong. Effects of Na+ in leachate on initial adsorption of biofilm. CHINA ENVIRONMENTAL SCIENCECE, 2022, 42(1): 213-219.
韩智勇, 许模, 刘国, 等. 生活垃圾填埋场地下水污染物识别与质量评价[J]. 中国环境科学, 2015, 35(9): 2843-2852. Han Z Y, Xu M, Liu G, et al. Domestic garbage landfill groundwater pollutant identification and quality evaluation [J]. China Environmental Science, 2015, 35(9): 2843-2852.
[2]
胡馨然, 杨斌, 韩智勇, 等. 中国正规、非正规生活垃圾填埋场地下水中典型污染指标特性比较分析[J]. 环境科学学报, 2019, 39(9): 3025-3038. Hu X R, Yang B, Han Z Y, et al. Comparative analysis on characteristics of typical pollution indicators in groundwater of regular and informal domestic waste landfills in China [J]. Journal of Environmental Science, 2019, 39(9): 3025-3038.
[3]
刘东, 孙建亭, 江丁酉, 等. 二妃山垃圾填埋场污染地下水的可能性分析[J]. 地质科技情报, 2002, 21(3): 79-83. Liu D, Sun J T, Jiang D U, et al. Analysis on the possibility of groundwater pollution in Erfei Mountain Landfill [J]. Geological Science and Technology Information, 2002, 21(3): 79-83.
[4]
Sekhohola-Dlamini L, Tekere M. Microbiology of municipal solid waste landfills: A review of microbial dynamics and ecological influences in waste bioprocessing [J]. Biodegradation, 2020, 31(1/2): 1-21.
[5]
王凯, 武道吉, 彭永臻, 等. 垃圾渗滤液处理工艺研究及应用现状浅析[J]. 北京工业大学学报, 2018, 44(1): 1-12. Wang K, Wu D J, Peng Y Z, et al. Critical review of landfill leachate treatment technologies [J]. Journal of Beijing University of Technology, 2018, 44(1): 1-12.
[6]
Luo H, Zeng Y, Cheng Y, et al. Recent advances in municipal landfill leachate: a review focusing on its characteristics, treatment, and toxicity assessment [J]. Science of the Total Environment, 2020, 703: 135468.
[7]
Lappin-Scott H, Costerton J. Microbial biofilms (Biotechnology research) [M]. Cambridge: Cambridge University Press, 1995: 712-739.
[8]
Paksy A, Powrie W, Robinson J P, et al. A laboratory investigation of anaerobic microbial clogging in granular landfill drainage media [J]. Geotechnique, 1998, 48(3): 389-401.
[9]
Rowe R K, Vangulck J F, Millward S C. Biologically induced clogging of a granular medium permeated with synthetic leachate [J]. Journal of Environmental Engineering and Science, 2002, 1(2): 135-156.
[10]
刘诗尧, 杨坪. 现代卫生填埋场渗滤液收集系统导排层阻塞作用研究[J]. 环境工程, 2015, 33(11): 125-128. Liu S Y, Yang P. Research status of mechanism of clogging in the granular drainage blanket in drainage systems of sanitary landfill [J]. Environmental Engineering, 2015, 33(11): 125-128.
[11]
Meng F, Zhang S, Oh Y, et al. Fouling in membrane bioreactors: An updated review [J]. Water Research, 2017, 114: 151-180.
[12]
Meireles A, Gonalves A L, Gomes I B, et al. Methods to study microbial adhesion on abiotic surfaces[J]. AIMS Bioengineering, 2015, 2(4): 297-309.
[13]
Berne C, Ellison C K, Ducret A, et al. Bacterial adhesion at the single-cell level [J]. Nature Reviews Microbiology, 2018, 16(10): 616-627.
[14]
Cavaliere R, Ball J L, Turnbull L, et al. The biofilm matrix destabilizers, EDTA and DNaseI, enhance the susceptibility of nontypeable Hemophilus influenzae biofilms to treatment with ampicillin and ciprofloxacin [J]. Microbiology Open, 2014, 3(4): 557-567.
[15]
Das T K, Ahlawat I P S, Yaduraju N T. Littleseed canarygrass (Phalaris minor) resistance to clodinafop-propargyl in wheat fields in north-western India: Appraisal and management [J]. Weed Biology and Management, 2014, 14(1): 11-20.
[16]
Mangwani N, Shukla S K, Rao T S, et al. Calcium-mediated modulation of Pseudomonas mendocina NR802 biofilm influences the phenanthrene degradation [J]. Colloids and Surfaces B: Biointerfaces, 2014, 114: 301-309.
[17]
Kjeldsen P, Barlaz M A, Rooker A P, et al. Present and long-term composition of MSW landfill leachate: A review [J]. Critical Reviews in Environmental Science and Technology, 2002, 32(4): 297-336.
[18]
Jewett D G, Hilbert T A, Logan B E, et al. Bacterial transport in laboratory columns and filters: Influence of ionic strength and pH on collision efficiency [J]. Water Research, 1995, 29(7): 1673-1680.
[19]
Burks G A, Velegol S B, Paramonova E, et al. Macroscopic and nanoscale measurements of the adhesion of bacteria with varying outer layer surface composition [J]. Langmuir, 2003, 19(6): 2366-2371.
[20]
Long G, Zhu P, Shen Y, et al. Influence of extracellular polymeric substances (EPS) on deposition kinetics of bacteria [J]. Environmental Science & Technology, 2009, 43(7): 2308-2314.
[21]
Wang Q, Ko J H, Wu H N, et al. Impact of bottom ash co-disposed with municipal solid waste on geotextile clogging in landfills [J]. Science of the Total Environment, 2021, 774: 145744.
[22]
刘丰, 王前, 吴华南, 等. 氧化石墨烯抑制填埋场土工布初期生物结垢[J]. 中国环境科学, 2020, 40(2): 695-700. Liu F, Wang Q, Wu H N, et al. Inhibition of initial bio-clogging of graphene oxide coated geotextiles in landfills [J]. China Environmental Science, 2020, 40(2): 695-700.
[23]
de Kerchove A J, Elimelech M. Calcium and magnesium cations enhance the adhesion of motile and nonmotile Pseudomonas aeruginosa on alginate films [J]. Langmuir, 2008, 24(7): 3392-3399.
[24]
Doliska A, Ribitsch V, Stana Kleinschek K, et al. Viscoelastic properties of fibrinogen adsorbed onto poly (ethylene terephthalate) surfaces by QCM-D [J]. Carbohydrate Polymers, 2013, 93(1): 246-255.
[25]
Reviakine I, Johannsmann D, Richter R P. Hearing what you cannot see and visualizing what you hear: interpreting quartz crystal microbalance data from solvated interfaces [J]. Analytical Chemistry, 2011, 83(23): 8838-8848.
[26]
Sauerbrey G. The use of quartz crystals for weighing thinlayers and for microweighing [J]. Journal of Physics, 1959, 155: 206-222.
[27]
Kou J, Tao D, Xu G. A study of adsorption of dodecylamine on quartz surface using quartz crystal microbalance with dissipation [J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2010, 368(1-3): 75-83.
[28]
Voinova M V, Rodahl M, Jonson M, et al. Viscoelastic acoustic response of layered polymer films at fluid-solid interfaces: continuum mechanics approach [J]. Physica Scripta, 1999, 59: 391-396.
[29]
Gutman J, Walker S L, Freger V, et al. Bacterial attachment and viscoelasticity: physicochemical and motility effects analyzed using quartz crystal microbalance with dissipation (QCM-D) [J]. Environmental Science & Technology, 2013, 47(1): 398-404.
[30]
Sobeck D C, Higgins M J. Examination of three theories for mechanisms of cation-induced bioflocculation [J]. Water Research, 2002, 36(3): 527-538.
[31]
Chen G X, Walker S L. Role of solution chemistry and ion valence on the adhesion kinetics of groundwater and marine bacteria [J]. Langmuir, 2007, 23: 7162-7169.
[32]
Olsson A L J, van der Mei H C, Busscher H J, et al. Novel analysis of bacterium-substratum bond maturation measured using a quartz crystal microbalance [J]. Langmuir, 2010, 26(13): 11113-11117.
[33]
Chen K L, Elimelech M. Aggregation and deposition kinetics of fullerene (C60) nanoparticles [J]. Langmuir, 2006, 22: 10994-11001.
[34]
Nguyen T H, Elimelech M. Plasmid DNA adsorption on silica: kinetics and conformational changes in monovalent and divalent salts [J]. Biomacromolecules, 2007, 8(1): 24-32.
[35]
Alexander T E, Lozeau L D, Camesano T A. QCM-D characterization of time-dependence of bacterial adhesion [J]. The Cell Surface, 2019, 5: 100024.
[36]
Berglin M, Pinori E, Sellborn A, et al. Fibrinogen adsorption and conformational change on model polymers: Novel aspects of mutual molecular rearrangement [J]. Langmuir, 2009, 25(10): 5602-5608.
[37]
王磊, 朱苗, 苗瑞, 等. 典型一价阳离子对蛋白质膜污染的影响特性[J]. 中国环境科学, 2017, 37(5): 1792-1797. Wang L, Zhu M, Miao R, et al. Effect of monovalent cations on ultrafiltration membrane fouling of protein [J]. China Environmental Science, 2017, 37(5): 1792-1797.
[38]
Sweity A, Ying W, Ali-Shtayeh M S, et al. Relation between EPS adherence, viscoelastic properties, and MBR operation: biofouling study with QCM-D[J]. Water Research, 2011, 45(19): 6430-6440.
[39]
李脆脆, 王磊, 李陈, 等. SGO/PVDF-g-PSSA复合质子交换膜的制备及抗污染性研究[J]. 中国环境科学, 2019, 39(1): 149-156. Li C C, Wang L, Li C, et al. Preparation and characterization of SGO/PVDF-g-PSSA composite proton exchange membrane and its anti-fouling properties [J]. China Environmental Science, 2019, 39(1): 149-156.
[40]
Chang X, Bouchard D C. Multiwalled carbon nanotube deposition on model environmental surfaces [J]. Environmental Science & Technology, 2013, 47(18): 10372-10380.
[41]
Hk F, Kasemo B, Nylander T, et al. Variations in coupled water, viscoelastic properties, and film thickness of a Mefp-1protein film during adsorption and cross-linking: a quartz crystal microbalance with dissipation monitoring, ellipsometry, and surface plasmon resonance study[J]. Journal of Analytical Chemistry, 2001, 73: 5796-5804.
[42]
Caiazza N C, O'Toole G A. SadB is required for the transition from reversible to irreversible attachment during biofilm formation by Pseudomonas aeruginosa PA14 [J]. Journal of Bacteriology, 2004, 186(14): 4476-4485.
[43]
Sohna Sohna J E, Cooper M A. Does the Sauerbrey equation hold true for binding of peptides and globular proteins to a QCM? [J]. Sensing and Bio-Sensing Research, 2016, 11: 71-77.
[44]
Vo H N P, Ngo H H, Guo W, et al. Selective carbon sources and salinities enhance enzymes and extracellular polymeric substances extrusion of Chlorella sp. for potential co-metabolism [J]. Bioresource Technology, 2020, 303: 122877.
[45]
Fatima T, Arora N K. Pseudomonas entomophila PE3 and its exopolysaccharides as biostimulants for enhancing growth, yield and tolerance responses of sunflower under saline conditions [J]. Microbiological Research, 2021, 244: 126671.
[46]
Reid E, Liu X, Judd S J. Effect of high salinity on activated sludge characteristics and membrane permeability in an immersed membrane bioreactor[J]. Journal of Membrane Science, 2006, 283(1/2): 164-171.