基于OMI数据的新疆地区臭氧柱浓度研究

刘旻霞; 孙瑞弟; 宋佳颖; 张娅娅; 李博文; 于瑞新; 李亮

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中国环境科学 ›› 2021, Vol. 41 ›› Issue (4) : 1498-1510.

大气污染与控制

基于OMI数据的新疆地区臭氧柱浓度研究

刘旻霞, 孙瑞弟, 宋佳颖, 张娅娅, 李博文, 于瑞新, 李亮

作者信息 +

Research on ozone column concentration in Xinjiang based on OMI data

LIU Min-xia, SUN Rui-di, SONG Jia-ying, ZHANG Ya-ya, LI Bo-wen, YU Rui-xin, LI liang

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摘要

利用臭氧监测仪（OMI）卫星反演数据，对2005~2018年新疆地区大气臭氧柱浓度数据进行提取及分析，探讨其时空分布格局及影响因素.结果表明：在时间变化上，2005~2018年，新疆地区大气臭氧柱浓度整体呈现逐渐上升趋势.在空间分布上，臭氧柱浓度自北向南逐渐降低，高值区集中分布在阿尔泰、塔城北部以及昌吉北部等区域；低值区集中于和田、巴音郭楞蒙古自治州和喀什的南部大部分地区.在季节变化上，大体呈现出春夏季高于秋冬季，高值区在春夏季交替出现，冬季略高于秋季，但四季的臭氧柱浓度值呈现逐渐上升的趋势.稳定性分析表明：研究区域臭氧柱浓度整体呈现中部及南北部分散、东西部集聚的分布格局.自然因素中，气候因素、风场以及海拔均呈现显著正相关（P<0.01）；通过后向轨迹追踪发现，该区域西北和西部气流是臭氧外来的最主要输送路径，分别占总气流轨迹的78.59%、57.29%.人为因素中，臭氧柱浓度值与地区生产总值、煤炭消耗量、工业废气排放量及机动车保有量均表现出显著的正相关关系（P<0.05）.其中，挥发性有机物（VOC_s）主要来源于工业源，其次是交通源和居民源.总体来看，臭氧浓度的变化受到了诸多因素的综合影响，但气温、VOC_s的排放及吸收性气溶胶是大气臭氧浓度变化的主导因素.

Abstract

Using Ozone Monitor (OMI) satellite inversion data, the atmospheric ozone column concentration data in Xinjiang from 2005 to 2018 were extracted and analyzed, and its temporal and spatial distribution pattern and influencing factors were discussed. The results showed that:In terms of time changes, in the past 14years, the atmospheric ozone column concentration in Xinjiang had shown a gradual upward trend. In spatial distribution, the concentration of ozone column gradually decreases from north to south, and the high value areas were concentrated in Altai, northern Tacheng and northern Changji. The low-value areas were concentrated in Hotan, Bayinguoleng Mongolia Autonomous Prefecture and most of the southern parts of Kashgar. In seasonal variation, the ozone column concentration in spring and summer was higher than that in autumn and winter, the high value area appeared alternately in spring and summer, and the winter was slightly higher than that in autumn, but the ozone column concentration in the four seasons showed a gradual upward trend. Stability analysis showed that the concentration of ozone column in the study area showed a distribution pattern of dispersion in the middle, south and north, and concentration in the east and west. Among the natural factors, climatic factors, wind field and altitude all showed significant positive correlation (P<0.01); Through backward trajectory tracking, it was found that the northwest and west air flows in the region were the most important transportation routes for ozone, and they accounted for the total airflow trajectories 78.59%, 57.29%. In human factors, the concentration of ozone column had a significant positive correlation with regional GDP, coal consumption, industrial waste gas emission and vehicle ownership (P<0.05). Among them, volatile organic compounds (VOCs) mainly comed from industrial sources, followed by traffic sources and residential sources. Generally speaking, the change of ozone concentration was affected by many factors, but air temperature, VOCs emission and absorbing aerosol were the dominant factors.

导出引用

刘旻霞, 孙瑞弟, 宋佳颖, 张娅娅, 李博文, 于瑞新, 李亮. 基于OMI数据的新疆地区臭氧柱浓度研究[J]. 中国环境科学. 2021, 41(4): 1498-1510

LIU Min-xia, SUN Rui-di, SONG Jia-ying, ZHANG Ya-ya, LI Bo-wen, YU Rui-xin, LI liang. Research on ozone column concentration in Xinjiang based on OMI data[J]. China Environmental Science. 2021, 41(4): 1498-1510

中图分类号： X515

参考文献

[1] 唐孝炎,李金龙,栗欣,等.大气环境化学[M]. 北京:高等教育出版社, 1990:232-233. Tang X Y, Li J L, Li X, et al. Atmospheric environmental chemistry[M]. Beijing:Higher Education Press, 1990:232-233.
[2] 盛裴轩,毛节泰,李建国,等.大气物理学[M]. 北京:北京大学出版社, 2003:82-98. Sheng P X, Mao J T, Li J G, et al. Atmospheric physics[M]. Beijing:Peking University Press, 2003:82-98.
[3] Nuvolone D, Balzi D, Pepe P, et al. Ozone short-term exposure and acute coronary events:A multicity study in Tuscany (Italy)[J]. Environmental Research, 2013,126(oct.):17-23.
[4] 列淦文,叶龙华,薛立.臭氧胁迫对植物主要生理功能的影响[J]. 生态学报, 2014,34(2):294-306. Lie G W, Ye L H, Xue L. Effects of ozone stress on major plant physiological functions[J]. Journal of Ecology, 2014,34(2):294-306.
[5] 耿春梅,王宗爽,任丽红,等.大气臭氧浓度升高对农作物产量的影响[J]. 环境科学研究, 2014,27(3):239-245. Geng C M, Wang Z S, Ren L H, et al. Study on the impact of elevated atmospheric ozone on crop yield[J]. Environmental Science Research, 2014,27(3):239-245.
[6] Liu J, Tarasick D W, Fioletov V E, et al. A global ozone climatology from ozone soundings via trajectory mapping:a stratospheric perspective[J]. Atmospheric Chemistry and Physics, 2013,13(22):11441-11464.
[7] Huang C, Lou D M, Hu Z Y, et al. A PEMS study of the emissions of gaseous pollutants and ultrafine particles from gasoline and diesel-fueled vehicles[J]. Atmospheric Environment, 2013,77(3):703-710.
[8] Zhang F W, Zhao J P, Chen J, et al. Pollution characteristics of organic and elemental carbon in PM_2.5 in Xiamen, China[J]. Journal of Environmental Sciences, 2011,23(8):1342-1349.
[9] Geiger H, Kleffmann J, Wiesen P. Smog chamber studies once influence of diesel exhaust on photo smog formation[J]. Atmospheric Environment, 2002,36(11):1737-1747.
[10] Fu T M, Daniel J, Jacob, et al. Space-based formaldehyde measurements as constraints on volatile organic compound emissions in east and south Asia and implications for ozone[J]. Journal of Geophysical Research, 2007,112(D6):382-388.
[11] Fishman J, Watson C E, Larsen J C, et al. Distribution of tropospheric ozone determined from satellite data[J]. Journal of Geophysical Research Atmospheres, 1990,95(D4):3599-3617.
[12] Fishman J, Balok A E. Calculation of daily tropospheric ozone residuals using TOMS and empirically improved SBUV measurements:application to an ozone pollution episode over the eastern United States[J]. Journal of Geophysical Research Atmospheres, 1999, 104(D23):30319-30340.
[13] 李阳,巨天珍,马成,等.长江三角洲近10年甲醛柱浓度变化及影响因素[J]. 中国环境科学, 2019,39(3):897-907. Li Y, Ju T Z, Ma C, et al. The temporal, spatial variation and influencing factor of formaldehyde column concentration in the Yangtze River Delta in the past 10years[J]. China Environmental Science, 2019,39(3):897-907.
[14] 李莹,赵春生,方圆圆,等.利用卫星资料分析对流层臭氧柱总量分布特征及其可能的原因[C]. 中国气象学会2005年年会论文集, 2005. Li Ying, Zhao Chunsheng, Fang Yuanyuan, et al. Using satellite data to analyze the distribution characteristics and possible causes of total tropospheric ozone column[C]. Proceedings of the 2005Annual Meeting of the Chinese Meteorological Society, 2005.
[15] 杜君平,朱玉霞,刘锐,等.基于OMI数据的中国臭氧总量时空分布特征[J]. 中国环境监测, 2014,30(2):191-196. Du J P, Zhu Y X, Liu R, et al. Temporal and spatial distribution characteristics of total ozone in China based on OMI data[J]. China Environmental Monitoring, 2014,30(2):191-196.
[16] 蒲茜,李振亮,张悦,等.重庆市O₃污染日的大气环流分型与传输特征[J]. 中国环境科学, 2021,41(1):18-27. Pu Q, Li Z L, Zhang Y, et al. Characterization of atmospheric circulation and transmission in Chongqing City during ozone polluted days[J]. China Environmental Science, 2021,41(1):18-27.
[17] 杨芳园,卞建春,王颢樾,等.基于OMI数据分析青藏高原周边对流层低层臭氧的分布特征[J]. 云南大学学报:自然科学版, 2013,35(2):183-192. Yang F Y, Bian J C, Wang H Y, et al. Seasonal variation of atmospheric ozone in the lower troposphere surrounding the Tibetan Plateau based on OMI satellite date[J]. Journal of Yunnan University:Natural Science Edition, 2013,35(2):183-192.
[18] 宋佳颖,刘旻霞,孙瑞弟,等.基于OMI数据的东南沿海大气臭氧浓度时空分布特征研究[J]. 环境科学学报, 2020,40(2):438-449. Song J Y, Liu M X, Sun R D, et al. Temporal and spatial characteristics of atmospheric ozone concentration in Southeast Coast based on OMI data[J]. Acta Scientiae Circumstantiae, 2020,40(2):438-449.
[19] Vasilkov A, Joiner J, Seftor C. First results from a rotational Ra man scattering cloud algorithm applied to the Suomi National Pol ar-orbiting Partnership (NPP) Ozone Mapping and Profiler Suite (OMPS) Nadir Mapper[J]. Atmospheric Measurement Techniques, 2014,7(9):2897-2906
[20] Akinyemi M L. Comparative analysis of total ozone data from satellite EPTOMS and ground-based Dobson instrument at Lagos-Nigeria[J]. Journal of Innovative Research in Engineering and Science, 2011,2:162-172.
[21] Borderer G E, Scott J C, Kreher K, et al. Global ozone trends in potential vorticity coordinates using TOMS and GOME intercom pared against the Dobson network:1978~1998[J]. Journal of Geophysical Research, 2001,106:23029-23042.
[22] Rahman M M, Rahman M S, Hai-bing W U. Time series analysis of causal relationship among gdp, agricultural, industrial and service sector growth in Bangladesh[J]. China-USA Business Review, 2011, 10(1):P9-15.
[23] 张亮林,潘竟虎,张大弘.基于MODIS数据的中国气溶胶光学厚度时空分布特征[J]. 环境科学学报, 2018,38(11):4431-4439. Zhang L L, Pan J H, Zhang D H. Spatio-temporal distribution characteristics of aerosol optical depths in China based on MODIS data[J]. Acta Scientiae Circumstantiae, 2018,38(11):4431-4439.
[24] 穆少杰,李建龙,陈奕兆,等.2001~2010年内蒙古植被覆盖度时空变化特征[J]. 地理学报, 2012,67(9):1255-1268. Mu S J, Li J L, Chen Y Z, et al. Spatial differences of variations of vegetation coverage in Inner Mongolia during 2001~2010[J]. Acta Geographica Sinica, 2012,67(9):1255-1268.
[25] 黄秋霞.新疆典型区域近地面臭氧浓度特征分析[D]. 乌鲁木齐,新疆大学, 2014. Huang Q X. Analysis of characteristics of near-ground ozone concentration in typical areas of Xinjiang[D]. Xinjiang University, 2014.
[26] 张倩倩,张兴嘉.基于卫星和地面观测的2013年以来我国臭氧时空分布及变化特征[J]. 环境科学, 2019,40(3):1133-1141. Zhang Q Q, Zhang X J. Ozone spatial-temporal distribution and trend over China since 2013:Insight from satellite and surface observation[J]. Environmental Science, 2019,40(3):1133-1141.
[27] 梅世玉,麻金继,张鑫.APEC期间京津冀地区NO₂浓度的时空变化特征研究[J]. 大气与环境光学学报, 2016,11(4):281-287. Mei S Y, Ma J J, Zhang X. Research on the spatio-temporal changes of NO₂ concentration in the Beijing-Tianjin-Hebei region during APEC[J]. Journal of Atmospheric and Environmental Optics, 2016, 11(4):281-287.
[28] 张远航,李金龙.中国城市光化学烟雾污染研究[J]. 北京大学学报(自然科学版), 1998,34(2):392-400. Zhang Y H, Li J L. 1998. Study on photochemical smog pollution in Chinese cities[J]. Journal of Peking University (Natural Science Edition), 1998,34(2):392-400.
[29] 贺克斌.打赢蓝天保卫战需要加快钢铁行业超低排放改造[N]. 中国环境报, 2019-05-06(3). He K B. Winning the blue sky defense battle requires accelerating the ultra-low emission transformation of the steel industry[N]. China Environment News, 2019-05-06(3).
[30] 生态环境部大气环境司.全国大气污染防治工作进展及建议[J]. 环境保护, 2018,46(19):11-15. Ministry of Ecology and Environment. Progress and suggestions on air pollution control in China[J]. Environmental Protection, 2018,46(19):11-15.
[31] 周春艳,王桥,厉青,等.近10年长江三角洲对流层NO₂柱浓度时空变化及影响因素[J]. 中国环境科学, 2016,36(7):1921-1930. Zhou C Y, Wang Q, Li Q, et al. Spatio-temporal change and influencing factors of tropospheric NO₂ column density of Yangtze River Delta in the decade[J]. Chinese Environmental Science, 2016, 36(7):1921-1930.
[32] 黄鑫,李亚丽,王靖中,等.1980~2016年陕西省冬季霾日数时空变化及增多成因初探[J]. 中国环境科学, 2019,39(9):3671-3681. Huang X, Li Y L, Wang J Z, et al. The spatial-temporal variations of haze in Shaanxi Province from 1980 to 2016 and the initial exploration of the increase[J]. Chinese Environmental Science, 2019,39(9):3671-3681.
[33] 古珊,杨显玉,吕世华,等.基于OMI数据的四川盆地对流层甲醛时空分布特征[J]. 环境科学学报, 2019,39(9):2860-2872. Gu S, Yang X Y, Lü S H, et al. Spatiotemporal variations in OMI satellite-based tropospheric formaldehyde in Sichuan Basin[J]. Acta Scientiae Circumstantiae, 2019,39(9):2860-2872.
[34] 刘树华,缪育聪,李婧,等.京津冀地区大气边界层结构与多尺度大气环流对大气污染扩散影响研究与展望[C]. 2017中国环境科学学会科学与技术年会论文集(第1卷), 2017. Liu S H, Miao Y C, Li J, et al. Research and prospect on the influence of atmospheric boundary layer structure and multiscale atmospheric circulation on air pollution diffusion in Beijing-Tianjin-Hebei region[C]. 2017 Proceedings of the Annual Conference of Science and Technology of Chinese Society of Environmental Sciences (Volume 1), 2017.
[35] 奇奕轩.北京北郊夏季臭氧及其前体物污染特征及影响因素研究[D]. 北京:中国环境科学研究院, 2017. Qi Y X. Research on pollution characteristics and influencing factors of ozone and its precursors in the northern suburbs of Beijing in summer[D]. Beijing:Chinese Academy of Environmental Sciences, 2017.
[36] 周牡丹.气候变化情景下新疆地区干旱指数及作物需水量预测[D]. 西北农林科技大学, 2014. Zhou M D. Drought Index and Crop Water Demand Forecast in Xinjiang under Climate Change Scenario[D]. Yangling:Northwest A&F University, 2014.
[37] 王金相.西北地区典型能源工业基地排放对局地环境空气质量的影响[D]. 兰州:兰州大学, 2018. Wang J X. Impact of emissions from typical energy industrial bases in Northwest China on local ambient air quality[D]. Lanzhou:Lanzhou University, 2018.
[38] 李俊华,常化振,陈亮,等.大气臭氧前体物NO_x和VOCs排放控制关键技术[C]. 中国大气环境科学与技术大会暨中国环境科学学会大气环境分会学术年会, 2012. Li J H, Chang H Z, Chen L, et al. Key technologies for NO_x and VOCs emission control of atmospheric ozone precursors[C]. China Conference on Atmospheric Environmental Science and Technology and the Annual Conference of the Atmospheric Environment Branch of the Chinese Society of Environmental Sciences, 2012.
[39] 徐建华.中国上空臭氧柱浓度和地面紫外辐射强度的预测[D]. 北京:北京大学, 2003. Xu J H. Prediction of ozone column concentration and ground ultraviolet radiation intensity over China[D]. Beijing:Beijing University, 2003.
[40] Li M, Zhang Q, Kurokawa J I, et al. MIX:A mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP[J]. Atmospheric Chemistry And Physics, 2017,17:935-963.