Heavy metal regional characteristics and potential ecological risk assessment of lakes and reservoirs in North China
LI Jie1,2,3, SONG Peng2, LI Hui1,2, CHENG Yun-xuan1, JIAO Li-xin1,3, LI Guo-dong1
1. National Engineering Laboratory for Lake Pollution Control and Ecological Restoration, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;
2. College of Agriculture, Henan University of Science and Technology, Luoyang 471000, China;
3. State Environmental Protection Key Laboratory for Lake Pollution Control, State Environmental Protection Key Laboratory of Drinking Water Source Protection, Chinese Research Academy of Environmental Sciences, Beijing 100012, China
The sediments of Baiyangdian Lake, Hengshui Lake, Yuqiao Reservoir, Songhua Lake, Dahuofang Reservoir and Xiaoxingkai Lake were selected as research objects. The contents of heavy metal elements including Cu, Zn, Pb, Cr and Ni in the sediments of the six lakes and reservoirs were determined with descriptive statistical analysis combined with multi-factor comparison of heavy metal pollution in other waters at home and abroad. The significant differences between the major sources of heavy metal pollution in the six lakes and reservoirs, the accumulation of heavy metals in the sediments and the similarities and differences with other waters at home and abroad were discussed. Heavy metal pollution in the sediments of Baiyangdian Lake, Hengshui Lake, Yuqiao Reservoir, Songhua Lake, Dahuofang Reservoir and Xiaoxingkai Lake was at a moderate to low level. There were differences in the main pollution sources between the six lakes. The heavy metal content of the sediment did not show a clear upward trend. Sediment heavy metal (Zn, Pb) are enriched in the six lakes, But the Pb content decreased compared with historical data, and the zinc content is generally higher than other regions. Dahuofang Reservoir sediments had the most heavy metal pollution. The average values of Cu, Zn, Pb, Cr and Ni were 56.28mg/kg, 142.3mg/kg, 17.44mg/kg, 97.9mg/kg, 44.44mg/kg respectively. Xiaoxingkai Lake has the lowest heavy metal content. The average values of Cu, Zn, Pb, Cr and Ni are 2.41mg/kg, 63.90mg/kg, 13.37mg/kg, 56.36mg/kg, 26.09mg/kg respectively. Comprehensive risk assessment of the six lakes and reservoirs, Dahuofang Reservoir> Yuqiao Reservoir> Baiyangdian Lake> Hengshui Lake> Songhua Lake> Xiaoxingkai Lake. The overall potential ecological risk index of heavy metals is low.
李捷, 宋鹏, 李慧, 程云轩, 焦立新, 李国栋. 北方湖库沉积物重金属区域特征及生态风险评价[J]. 中国环境科学, 2020, 40(11): 4927-4935.
LI Jie, SONG Peng, LI Hui, CHENG Yun-xuan, JIAO Li-xin, LI Guo-dong. Heavy metal regional characteristics and potential ecological risk assessment of lakes and reservoirs in North China. CHINA ENVIRONMENTAL SCIENCECE, 2020, 40(11): 4927-4935.
金相灿,王圣瑞,席海燕.湖泊生态安全及其评估方法框架[J]. 环境科学研究, 2012,25(4):357-362. Jin X C, Wang S R, Xi H Y. Lake ecological security and assessment methodology framework[J]. Research of Environmental Sciences, 2012,25(4):357-362.
[2]
余成,陈爽,张路.坦噶尼喀湖东北部入湖河流沉积物重金属分布特征与生态风险评价[J]. 环境科学, 2016,37(2):499-506. Yu C, Chen S, Zhang L. Distribution and potential ecological risk assessment of heavy metals in surface sediments of inflow rivers to northeastern lake Tanganyika[J]. Environmental Science, 2016,37(2):499-506.
[3]
王祖伟,王祎玮,侯迎迎,等.于桥水库水源地水体沉积物重金属空间分异与景观格局的关系[J]. 环境科学, 2016,37(9):3423-3429. Wang Z W, Wang Y W, Hou Y Y, et al. Relationship between landscape pattern and spatial variation of heavy metals in aquatic sediments in headwaters area of Yuqiao Reservoir[J]. Environmental Science, 2016,37(9):3423-3429.
[4]
季斌,杭小帅,梁斌,等.湖泊沉积物重金属污染研究进展[J]. 污染防治技术, 2013,26(5):33-40. Ji B, Hang X S, Liang B, et al. Advances in heavy metals contamination of lake sediment[J]. Pollution Control Technology, 2013,26(5):33-40.
[5]
李波,喻庆国,危锋,等.滇西北剑湖沉积物钒空间分布特征和生态风险[J]. 中国环境科学, 2019,39(5):2219-2229. Li B, Yu Q G, Wei F, et al. Spatial distribution characteristics and ecological risks of vanadium in sediments from Jianhu Lake, Northwest Yunnan Province, China[J]. China Environmental Science, 2019,39(5):2219-2229.
[6]
崔志丹,冯建国,焦立新,等.松花湖表层沉积物中PAHs及PAEs污染特征[J]. 环境科学研究, 2019,32(9):1531-1539. Cui Z D, Feng J G, Jiao L X, et al. Pollution characteristics of polycyclic aromatic hydrocarbons and phthalate esters in surface sediments of in Songhua Lake[J]. Research of Environmental Sciences, 2019,32(9):1531-1539.
[7]
高秋生,赵永辉,焦立新,等.白洋淀水体挥发性有机物污染特征与风险评价[J]. 环境科学, 2018,39(5):2048-2055. Gao Q S, Zhao Y H, Jiao L X, et al. Pollution characteristics and health risk assessment of volatile organic compounds in Baiyangdian Lake[J]. Environmental Science, 2018,39(5):2048-2055.
[8]
王乃姗,张曼胤,崔丽娟,等.河北衡水湖湿地汞污染现状及生态风险评价[J]. 环境科学, 2016,37(5):1754-1762. Wang N S, Zhang M Y, Cui L J, et al. Contamination and ecological risk assessment of mercury in Hengshuihu Wetland,Hebei Province[J]. Environmental Science, 2016,37(5):1754-1762.
[9]
贾雪莹.铁输入对小兴凯湖湿地植物-沉积物系统磷迁移的影响研究[D]. 长春:中国科学院大学(中国科学院东北地理与农业生态研究所), 2019. Jia X Y. Effects of Iron Input on phosphorus adsorption of wetlands-sediment system in Xiaoxingkai Lake[D]. Changchun:University of Chinese Academy of Sciences (Northeast Institute of Geography and Agroecology, Chinese Academy of Sciences), 2019.
[10]
宁增平,蓝小龙,黄正玉,等.贺江水系沉积物重金属空间分布特征、来源及潜在生态风险[J]. 中国环境科学, 2017,37(8):3036-3047. Ning Z P, Lan X L, Huang Z Y, et al. Spatial distribution characteristics, sources and potential ecological risk of heavy metals in sediments of the Hejiang River[J]. China Environmental Science, 2017,37(8):3036-3047.
[11]
王琳琳,于海业,张蕾,等.基于生态位适宜度模型和TOPSIS模型的间作模式评价[J]. 农业机械学报, 2017,48(4):291-297. Wang L L, Yu H Y, Zhang L, et al. Evaluation of intercropping pattern based on niche-fitness model and TOPSIS Model[J]. Journal of Agricultural Machinery, 2017,48(4):291-297.
[12]
张颖,周军,张宝杰,等.松花江表层沉积物有毒重金属污染评价[J]. 湖南大学学报(自然科学版), 2015,42(6):113-118. Zhang Y, Zhou J, Zhang B J, et al. Pollution evaluation of toxic heavy metals in the sediments of Songhua River[J]. Journal of Hunan University (Natural Sciences), 2015,42(6):113-118.
[13]
Håkanson L. An ecological risk index for aquatic pollution control-a sedimentological approach[J]. Water Research, 1980,14:975-1001.
[14]
GB 15618-2018土壤环境质量农用地土壤污染风险管控标准(试行)[S]. GB 15618-2018 Soil environmental quality-Risk control standard for soil contamination of agricultural land[S].
[15]
庞绪贵,代杰瑞,陈磊,等.山东省17市土壤地球化学背景值[J]. 山东国土资源, 2019,35(1):46-56. Pang X G, Dai J R, Chen L, et al. Soil geochemical background value of 17 cities in Shandong Province[J]. Shandong Land and Resources, 2019,35(1):46-56.
[16]
高秋生,田自强,焦立新,等.白洋淀重金属污染特征与生态风险评价[J]. 环境工程技术学报, 2019,9(1):66-75. Gao Q S, Tian Z Q, Jiao L X, et al. Pollution characteristics and ecological risk assessment of heavy metals in Baiyangdian Lake[J]. Journal of Environmental Engineering Technology, 2019,9(1):66-75.
[17]
罗燕,秦延文,张雷,等.大伙房水库沉积物重金属形态分析及污染特征[J]. 环境科学研究, 2011,24(12):1370-1377. Luo Y, Qin Y W, Zhang L, et al. Speciation and pollution characteristics of heavy metals in the sediment of Dahuofang Reservoir[J]. Research of Environmental Sciences, 2011,24(12):1370-1377.
[18]
张曼胤,崔丽娟,盛连喜,等.衡水湖湿地底泥重金属污染及潜在生态风险评价[J]. 湿地科学, 2007,(4):362-369. Zhang M Y, Cui L J, Sheng L X, et al. Pollution and ecological risk assessment of heavy metals in the Hengshuihu Wetland[J]. Wetland Science, 2007,(4):362-369.
[19]
刘丽娜,马春子,张靖天,等.东北典型湖泊沉积物氮磷和重金属分布特征及其污染评价研究[J]. 农业环境科学学报, 2018,37(3):520-529. Liu L N, Ma C Z, Zhang J T, et al. Distribution characteristics of pollution from nitrogen, phosphorus, and heavy metals in sediments of Shankou Lake in Northeast China[J]. Journal of Agro-Environment Science, 2018,37(3):520-529.
[20]
于淑玲,李晓宇,张继涛,等.小兴凯湖表层底泥磷吸附容量及潜在释放风险[J]. 中国环境科学, 2014,34(8):2078-2085. Yu S L, Li X Y, Zhang J T, et al. Phsophorus sorption capacity of surface sediments and risk assessment of potential phosphorus release in Lake Xiaoxingkai, China[J]. China Environmental Science, 2014,34(8):2078-2085.
[21]
刘文,吉力力·阿不都外力,马龙.博斯腾湖表层沉积物元素地球化学特征及重金属污染评价[J]. 地球环境学报, 2019,10(2):128-140. Liu W, Jilili·A, Ma L. Geochemical characteristics of major and trace elements and heavy metal pollution status in surface sediment of Bosten Lake[J]. Journal of Earth Environment, 2019,10(2):128-140.
[22]
郭泌汐,刘勇勤,张凡,等.西藏湖泊沉积物重金属元素特征及生态风险评估[J]. 环境科学, 2016,37(2):490-498. Guo B X, Liu Y Q, Zhang F, et al. Characteristics and risk assessment of heavy metals in core sediments from lakes of Tibet[J]. Environmental Science, 2016,37(2):490-498.
[23]
姜会敏,郑显鹏,李文.中国主要湖泊重金属来源及生态风险评估[J]. 中国人口·资源与环境, 2018,28(S1):108-112. Jiang H M, Zheng X P, Li W. Sources and ecological risk assessment of heavy metals in major lakes in China[J]. China Population, Resources and Environment, 2018,28(S1):108-112.
[24]
刘嘉妮.中国五大淡水湖沉积物中重金属的污染特征及评价[D]. 长沙:中南林业科技大学, 2011. Liu J N. Character and assessment of heavy metals in the sediments from' five biggest freshwater lakes[D]. changsha:Central South University of Forestry and Technology, 2011.
[25]
王伟,樊祥科,黄春贵,等.江苏省五大湖泊水体重金属的监测与比较分析[J]. 湖泊科学, 2016,28(3):494-501. Wang W, Fan X K, Huang C G, et al. Monitoring and comparison analysis of heavy metals in the five great lakes in Jiangsu Province[J]. Lake Science, 2016,28(3):494-501.
[26]
张林英,徐颂军,付笛峰.珠江河口湿地土壤重金属污染评价及空间特征分析[J]. 热带地貌, 2018,(1):20-25. Zhang L Y, Xu S J, Fu D F. Characteristics of heavy metal pollution in the Pearl River estuary wetland soil[J]. Tropical Geomorphology, 2018,(1):20-25.
[27]
张远,石陶然,于涛,等.滇池典型湖区沉积物粒径与重金属分布特征[J]. 环境科学研究, 2013,26(4). Zhang Y, Shi T R, Yu T, et al. Sediment particle size and the distribution of heavy metals in the typical districts of Dianchi Lake[J]. Research of Environmental Sciences, 2013,26(4).
[28]
陈敬安,万国江,黄荣贵.洱海沉积物重金属地球化学相及其污染历史研究[J]. 地质地球化学, 1998:1-8. Chen J A, Wan G J, Huang R G. Geochemical facies of heavy metals in erhai sediments and their pollution history[J]. Geology Geochemistry, 1998:1-8.
[29]
田林锋,胡继伟,罗桂林,等.贵州百花湖沉积物重金属稳定性及潜在生态风险性研究[J]. 环境科学学报, 2012,32(4):885-894. Tian L F, Hu J W, Luo G L, et al. Ecological risk and stability of heavy metals in sediments from Lake Baihua in Guizhou Province[J]. Acta Scientiae Circumstantiae, 2012,32(4):885-894.
[30]
古正刚,吴敏,卫蓉,等.泸沽湖表层沉积物中重金属污染特征[J]. 环境科学与技术, 2014,37(11):111-115,136. Gu Z G, Wu M, Wei R, et al. Charactexistics of heavy metal pollution in top-layer sediment Lugu Lake[J]. Environmental Science & Technology, 2014,37(11):111-115.
[31]
Geoffrey Gokaka. Nyamwamba河重金属迁移与George Ramsar湖泊湿地污染评估[D]. 北京:清华大学, 2015. Geoffrey Gokaka. Assessment of heavy metal migration through river Nyamwamba and pollution of Lake George Ramsar site[D]. Beijing:Qinghua University, 2015.
[32]
Bintal A, Ahmad I, Chee K Y. Heavy metal concentrations in sediment and intertidal gastropod nerita lineata from two opposing sites in the Straits of Malacca[J]. Wetland Science, 2008,6(3):411-421.
[33]
Villalobos-Casta Eda B, Cortés-Martínez R, Segovia N, et al. Distribution and enrichment of trace metals and arsenic at the upper layer of sediments from Lerma River in La Piedad, Mexico:case history[J]. Environmental Earth Sciences, 2016,75(23):1490.
[34]
侯迎迎,王祖伟,苗钰婷,等.于桥水库水源地水体重金属潜在生态风险评价[J]. 天津师范大学学报(自然科学版), 2018,38(5):52-57. Hou Y Y, Wang Z W, Miao Y T, et al. Ecological risks evaiiiation of heavy metals in source water of Yuqiao Reservoir[J]. Journal of Tianjin Normal University (Natural Science Edition), 2018,38(5):52-57.
