Abstract:In order to explore the boundary layer characteristics, the multi-source observation data such as automatic meteorological station data, environmental hourly concentration data, microwave radiation data, wind profile radar, aerosol lidar and WRF-Chem source tagged method were used to analyze a typical fog-haze episode in Tianjin from December 7 to 10, 2019. The results showed that: The fog-haze process can be clearly divided into four stages of fog formation, fog and haze alternation, haze, and haze dissipation. Fog-haze weather was closely related to atmospheric temperature stratification, with the generation of temperature inversion, the maximum growth rate of relative humidity and liquid water content reached 13.44%/h and 0.013g/(m3·h), respectively, showing an explosive growth up to 92% of the relative humidity, and the microwave radiation data can better predict the formation of fog. In the stage of fog and haze alternation, fog weather changed the structure of the boundary layer. The atmosphere in the fog layer was in a neutral state, being relatively conducive to the pollutant diffusion in the fog area. The high value of PM2.5 concentration mainly occurred below 400m, and the continuous inversion at the fog top inhibited the diffusion of pollutants to the upper atmosphere, resulting in the aggravation of pollutant concentration in the fog area and an increase in surface PM2.5 up to 135~223μg/m3 near to ground, maintaining moderate-severe pollution. There was a good relationship between fog-haze weather and vertical wind field. In fog and haze alternation stage, there were two situations, low wind speed and high wind speed (the southwesterly wind brought abundant water vapor), which are beneficial to the maintenance of fog. The wind speed was 6~12m/s above the fog top inversion and 1~2m/s in the fog layer. The existence of fog was not conducive to the improvement of air quality near the ground. During the fog-haze process, the local emissions contributed 36.1% to surface PM2.5 concentration in Tianjin, and the contribution of regional transport was 63.9%, demonstrating obvious regional transport characteristics of the whole pollutant process.
孟丽红, 刘海玲, 王炜, 蔡子颖, 刘丽丽, 曲平, 郝囝. 基于多源资料天津一次雾-霾过程的边界层特征[J]. 中国环境科学, 2022, 42(9): 4018-4025.
MENG Li-hong, LIU Hai-ling, WANG Wei, CAI Zi-ying, LIU Li-li, QU Ping, HAO Jian. Boundary layer characteristics of fog - haze in Tianjin based on multi - source data. CHINA ENVIRONMENTAL SCIENCECE, 2022, 42(9): 4018-4025.
Zhang Y, Zhu B, GAO J H, et al. The source apportionment of primary PM2.5 in an aerosol pollution event over Beijing-Tianjin-Hebei Region using WRF-Chem, China [J]. Aerosol & Air Quality Research, 2017,17(12):2966-2980.
[2]
Duan F K, He K B, Ma Y L, et al. Concentration and chemical characteristics of PM2.5 in Beijing, China: 2001~2002 [J]. Science of the Total Environment, 2006,355(1/2/3):264-275.
[3]
Li L, Wang W, Feng J L, et al. Composition, source, mass closure of PM2.5 aerosols for four forests in eastern China [J]. Journal of Environment Science, 2010,31(3):405-412.
[4]
Zhao X J, Zhao P S, Xu J,et al. Analysis of a winter regional haze event and its formation mechanism in the North China Plain [J]. Atmospheric Chemistry and Physics Discussions, 2013,13(1):903- 933.
[5]
孟丽红,李英华,韩素芹,等.海陆风对天津市PM2.5和O3质量浓度的影响 [J]. 环境科学研究, 2019,32(3):390-398. Meng L H, Li Y H, Han S Q, et a1. Influence of sea-land breeze on the concentrations of PM2.5 and O3 in Tianjin City [J]. Research of Environmental Science, 2019,32(3):390-398.
[6]
韩笑颜,周 颖,吕 喆,等.京津冀典型城市一次重污染过程特征及边界层结构变化对其影响 [J]. 环境科学研究, 2020,33(10):2236- 2245. Han X Y, Zhou Y, Lu Z, et a1. Characteristics of heavy air pollution process and influnce of structure variation of planetary boundary layer in typical cities of Beijing-Tianjin-Hebei Region [J]. Research of Environmental Science, 2020,33(10):2236-2245.
[7]
孟丽红,蔡子颖,李英华,等.天津市PM2.5浓度时空分布特征及重污染过程来源模拟 [J]. 环境科学研究, 2020,33(1):9-17. Meng L H, Cai Z Y, Li Y H, et a1. Spatial and temporal distributions and source similation during heavy pollution of PM2.5 in Tianjin City [J]. Research of Environmental Science, 2020,33(1):9-17.
[8]
Wang M R, Kai K J, Sgimoto N B, et a1. Meterological factoers affecting winter particular air pollution in Ulaanbaatar from 2008 to 2016 [J]. Asian Journal of Atmospheric Environment, 2018,12(3): 244-254.
[9]
Leng C, Duan J, Xu C, et al, Insights into a historic severe haze event in Shanghai: synoptic situation, boundary layer and pollutants [J]. Atmospheric Chemistry and Physics, 2016,16(14):9221-9234.
[10]
廖晓农,张小玲,王迎春,等.北京地区冬夏季持续性雾霾发生的环境气象条件对比分析 [J]. 环境科学, 2014,35(6):2031-2044. Liao X N, Zhang X L, Wang Y C,et al. Comparative analysis on meteorological condition for persistent haze cases in summer and winter in Beijing [J]. Environmental Science, 2014,35(6):2031-2044.
[11]
周述学,邓学良,王传辉,等.华东2018年冬季一次典型雾霾过程气象成因分析 [J]. 高原气象, 2020,390(5):1110-1121. Zhou S X, Deng X L, Wang C H, et al. Analysis of meteorological conditions for a typical fog and haze event over eastern China in winter of 2018 [J]. Plateau Meteorology, 2020,39(5):1110-1121.
[12]
WANG X Q, WEI W, CHENG S Y, et al. Characteristics and classification of PM2.5, pollution episodes in Beijing from 2013 to 2015 [J]. Science of the Total Environment, 2018,612:170-179.
[13]
Li L, Wang W, Feng J L, et al. Composition, source, mass closure of PM2.5 aerosols for four forests in eastern China [J]. Journal of Environment Science, 2010,31(3):405-412.
[14]
Zhao X J, Zhao P S, Xu J,et al. Analysis of a winter regional haze event and its formation mechanism in the North China Plain [J]. Atmospheric Chemistry and Physics Discussions, 2013,13(1):903-933.
[15]
李 梦,唐贵谦,黄 俊,等.京津冀冬季大气混合层高度与大气污染的关系 [J]. 环境科学, 2015,36(6):1935-1943. Li M, Tang G Q, Huan J, et a1. Characteristics of winter atmospheric mixing layer height in Beijing-Tianjin-Hebei region and their relationship with the atmospheric pollution [J]. Environmental Science, 2015,36(6):1935-1943.
[16]
杨 军,王 蕾,刘端阳,等.一次浓雾过程的边界层特征及生消物理机制 [J]. 气象学报, 2010,68(6):998-1006. Yang J, Wang L, Liu D Y, et al. The boundary layer structure and the evolution mechanisms of a deep dense fog event [J]. Acta Meteorologica Sinica, 2010,68(6):998-1006.
[17]
潘 亮,闫凤霞,吴峻石,等.2013~2019年上海早晨接地逆温指标与PM2.5定量关系研究 [J]. 中国环境科学, 2021,41(2):517-526. Pan L, Yan F X, Wu J S, et al. Parameters of surface based inversion in the morning during 2013 to 2019 and its quantitative relationship with PM2.5 in Shanghai [J]. China Environmental Science, 2021,41(2):517- 526.
[18]
Han S Q, Zhang Y F, Wu J, et al. Evaluation of regional background particulate matter concentration based on vertical distribution characteristics [J]. Atmospheric Chemistry and Physics, 2015,15: 11165-11177.
[19]
刘 超,花 丛,张恒德,等.L波段探空雷达秒数据在污染天气边界层分析中的应用 [J]. 气象, 2017,43(5):591-597. Liu C, Hua C, Zhang H D, et al. Application of L-band radar sounding data in analyzing polluted weather boundary layer [J]. Meteorological Monthly, 2017,43(5):591-597.
[20]
Liu C, Hua C, Zhang H D, et al. A severe fog-haze episode in Beijing-Tianjin-Hebei region: characteristics sources and impacts of boundary layer structure [J]. Atmospheric Pollution Research, 2019, 10:1190-1202.
[21]
孟丽红,张 敏,韩素芹.天津市郊区冬季大气边界层风、温场结构与特征 [J]. 中国环境科学, 2012,32(10):1758-1763. Meng L H, Zhang M, Han S Q.Structures and characteristics of the atmospheric boundary layer in winter of the Tianjin suburb [J]. China Environmental Science, 2012,32(10):1758-1763.
[22]
张 敏,蔡子颖,韩素芹,等.天津污染天气边界层温度层结变化特征及预报阈值确定 [J]. 环境科学学报, 2018,38(6):2270-2278. Zhang M, Cai Z Y, Han S Q, et al. The research on threshold and regularity of temparature stratification in heavy polltion weather in Tianjin [J]. Acta Scientiae Circumstantiae, 2018,38(6):2270-2278.
[23]
姚 青,刘敬乐,蔡子颖,等.天津一次雾-霾天气过程的近地层温湿结构和湍流特征分析 [J]. 环境科学学报, 2018,38(10):3856-3867. Yao Q, Liu J L, Cai Z Y, et al. Analysis of temperature and moisture structure and turbulence characteristics of a smog and haze weather process in Tianjin [J]. Acta Scientiae Circumstantiae, 2018,38(10): 3856-3867.
[24]
蔡子颖,韩素芹,吴彬贵,等.天津一次雾过程的边界层特征研究 [J]. 气象, 2012,38(9):1103-1109. Cai Z Y, Han S Q, Wu B G, et al. Analysis an characteristics of atmospheric boundary layer during a fog process in Tianjin [J]. Meteorological Monthly, 2012,38(9):1103-1109.
[25]
Guo L J, Guo X L, Fang C G,et al. Observation analysis on characteristics of formation, evolution and transition of a long-lasting severe fog and haze episode in North China [J]. Science China Earth Sciences, 2015,58(3):329-344.
[26]
Liu, H, Liu, C, Xie, Z, et al. A paradox for air pollution controlling in China revealed by “APEC Blue”and “Parade Blue” [J]. Scientific Reports, 2016,6:1-13.
Ju T T, Wu B G, Zhang H S, et al. Parameterization of radiation fog-top height and methods evaluation in Tianjin [J]. Atmospheric, 2020,11(5480):1-18.
[29]
余文韬,吴振玲,何群英,等.天津天气预报手册 [M]. 北京:气象出版社, 2015:83-92. Yu W T, Wu Z L, He Q Y, et al. The weather forecast manual of Tianjin [M]. Beijing: China Meteorological Press, 2015:83-92.
[30]
Wang S, Liao T T, Wang L L, et al. Process analysis of characteristics of the boundary layer during a heavy haze pollution episode in an inland megacity, China [J]. Journal of Environmental Science, 2016,40:138-144.
[31]
Wu W N, Zha Y, Zhang J H, et al. A temperature inversion-induced air pollution process as analyzed from Mie LiDAR data [J]. Science of the Total Environment, 2014,479/480:102-108.
[32]
Yuan Z X, Qin J, Zheng X, et al. The relationship between atmospheric circulation, boundary layer and near-surface turbulence in severe fog-haze pollution periods [J]. Journal of Atmospheric and Solar–Terrestrial Physics, 2020,200:105216.
[33]
杨 旭,蔡子颖,韩素芹,等.基于无人机探空和数值模拟天津一次重污染过程分析 [J]. 环境科学, 2021,42(1):9-18. Yang X,Cai Z Y,Han S Q,et al. Heavy polltion episode in Tianjin based on UAV meteorological sounding and numerical model [J]. Environmental Science, 2021,42(1):9-18.