Advances and prospective of nitrated organic compounds in the atmosphere
BAI Xu-rong1,2, LI Hong1, REN Yan-qin1, LONG Fang-yun1
1. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; 2. Shandong University, Environment Research Institute, Qingdao 266237, China
Abstract:Nitro-polycyclic aromatic hydrocarbons, nitro-phenols and organic nitrates are three forms of nitrogen-containing organic compounds which are greatly affected by human activities, highly reactive and have significant impacts on the atmosphere, climate change and human health. This paper focuses on the current state of research on the three forms of nitrogen-containing organic compounds in the atmosphere, and summarizes the latest findings on their environmental behavior, analysis methods, pollution characteristics, sources and causes, and then proposes their pollution prevention measures. The conclusions indicate that the environmental behaviors of nitrogen-containing organic compounds are closely related to their molecular weights, saturation vapor pressure, ambient temperature and humidity. The main analytical methods now employed for nitrogen-containing organic compounds in atmospheric environments are off-line detection in laboratories and online observation in the field, and the quantum chemistry calculation method is also used for their theoretical research. The pollution characteristics of nitrogen-containing organic compounds showed obvious spatiotemporal variations under the influence of emission sources and meteorological conditions. And the primary combustion emissions and secondary oxidation reactions were the main sources of nitrogen-containing organic compounds. Based on the limitations of the current research on nitrogen-containing organic compounds, this study proposes future research prospects to strengthen the investigation of toxic effects, improve the analytical methods and explore the generation mechanisms.
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BAI Xu-rong, LI Hong, REN Yan-qin, LONG Fang-yun. Advances and prospective of nitrated organic compounds in the atmosphere. CHINA ENVIRONMENTAL SCIENCECE, 2023, 43(7): 3416-3428.
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