Hydraulic experiments and numerical simulation of microplastics migration in aquatic environments
LI Yu-xuan1, DOU Ming1,2, LI Gui-qiu2, WANG Zhen2, ZHOU Yu-ze2, XING Ao-qi1
1. College of Ecology and Environment, Zhengzhou University, Zhengzhou 450001, China; 2. College of Water Conservancy and Transportation, Zhengzhou University, Zhengzhou 450001, China
Abstract:The migration behavior of microplastics in aquatic environments is governed by complex interactions among hydraulic, physical, and material-specific factors. This study integrates hydraulic experiments and force analysis to identify the critical hydraulic parameter thresholds influencing state transitions of different microplastic types in freshwater systems. A Lagrangian particle tracking method is then employed to develop a migration model grounded in well-defined physical principles. This model simulates microplastic trajectories, predicting their ultimate movement states and environmental fate. The model is validated using field data from the urban section of the Jialu River in Zhengzhou, China. Results indicate that 66.79% of microplastics in this section have particle sizes smaller than 0.5mm, with fragmented (31.1%) and fibrous (29.2%) shapes being predominant. Polypropylene (PP) migrates as floating debris with the highest velocity, while polystyrene (PS) and polyamide (PA) particles smaller than 0.5mm migrate as suspended load. In contrast, polyethylene terephthalate (PET) and PA particles larger than 0.5mm migrate as bedload or remain stationary on the riverbed. Under flow rates of 14m3/s and 20m3/s, retention rates of microplastics over 36hours were 43.79% and 47.85%, respectively, with PA and PET constituting the major retained microplastic types. These findings provide valuable insights into the hydrodynamic behavior and environmental fate of microplastics, offering guidance for pollution management in freshwater systems.
[1] 李卓然,季民,赵迎新.全球微塑料研究现状及热点可视化剖析[J].环境化学, 2022,41(4):1-13. Li Zhuoran, Ji Min, Zhao Yingxin. Global microplastic research status and hot spot visualization analysis[J]. Environmental Chemistry, 2022, 41(4):1-13. [2] Jiang Jianhao, He Lulu, Zheng Shiwei, et al. A review of microplastic transport in coastal zones[J]. Marine Environmental Research, 2024, 196:106397. [3] 张晨,王清,赵建民.海洋微塑料输运的数值模拟研究进展[J].地球科学进展, 2019,34(1):72-83. Zhang Chen, Wang Qing, Zhao Jianmin. Progress in numerical simulation of marine microplastic transport[J]. Progress in Earth Science, 2019,34(1):72-83. [4] 李嘉,李艳芳,张华.海洋微塑料物理迁移过程研究进展与展望[J].海洋科学, 2018,42(5):155-162. Li Jia, Li Yanfang, Zhang Hua. Research progress and prospect on the physical migration process of marine microplastics[J]. Marine Science, 2018,42(5):155-162. [5] 刘恩秀,郭鹤,李云,等.塑料微粒在淡水中的分布及其影响研究进展[J].环境科学与技术, 2017,40(S2):165-170. Liu Enxiu, Guo He, Li Yun, et al. Research progress on the distribution and effects of plastic particles in freshwater[J]. Environmental Science and Technology, 2017,40(S2):165-170. [6] Critchell K, Lambrechts J. Modelling accumulation of marine plastics in the coastal zone; what are the dominant physical processes?[J]. Estuarine, Coastal and Shelf Science, 2016,171:111-122. [7] Ballent A, Pando S, Purser A, et al. Modelled transport of benthic marine microplastic pollution in the Nazaré Canyon[J]. Biogeosciences, 2013,10(12):7957-7970. [8] Guo M, Noori R, Abolfathi S. Microplastics in freshwater systems:Dynamic behaviour and transport processes[J]. Resources, Conservation& Recycling, 2024,205:107578. [9] Kryss W, Holger S. Effects of particle properties on the settling and rise velocities of microplastics in freshwater under laboratory conditions.[J]. Environmental Science& Technology, 2019,53(4):1958-1966. [10] Mel C, Claire A, Lisa W, et al. Trapped microplastics within vertical redeposited sediment:Experimental study simulating lake and channeled river systems during resuspension events[J]. Environmental Pollution, 2023,322:121212. [11] Cai Caiyuan, Zhu Liangsheng, Hong Bo. A review of methods for modeling microplastic transport in the marine environments[J]. Marine Pollution Bulletin, 2023,193:115136. [12] Xing Liming, Bolster Diogo, Liu Haifei, et al. Markovian models for microplastic transport in open-channel flows[J]. Water Resources Research, 2022,58(8):1-14. [13] He Beibei, Mitchell S, Prasanna E, et al. Dispersal and transport of microplastics in river sediments[J]. Environmental Pollution, 2021,279:116884. [14] Mia B, Ekaterina S, Ailinh N, et al. Hydrodynamic modelling of traffic-related microplastics discharged with stormwater into the Göta River in Sweden[J]. Environmental Science and Pollution Research, 2020,27(19):24218-24230. [15] Geng Xiaolong, Boufadel M C, Lopez E P. Modeling impacts of river hydrodynamics on fate and transport of microplastics in riverine environments[J]. Marine Pollution Bulletin, 2023,196:115602. [16] Zhou Tianhong, Song Shangjian, Min Rui, et al. Advances in chemical removal and degradation technologies for microplastics in the aquatic environment:A review[J]. Marine Pollution Bulletin, 2024,201:116202. [17] Verma A, Sharma G, Kumar A, et al. Microplastic pollutants in water:A comprehensive review on their remediation by adsorption using various adsorbents[J]. Chemosphere, 2024,352:141365. [18] 黄德法,王韦,余挺,等.河道模型中泥沙起动粒径公式的比较和验证[J].水利与建筑工程学报, 2008,(1):15-16,22. Huang Defa, Wang Wei, Yu Ting, et al. Comparison and verification of sediment incipient particle size formula in river channel model[J]. Journal of Water Conservancy and Construction Engineering, 2008,(1):15-16,22. [19] 吴宁,张琪,曲占庆.固体颗粒在液体中沉降速度的计算方法评述[J].石油钻采工艺, 2000,(2):51-53,56-83. Wu Ning, Zhang Qi, Qu Zhanqing. A review of computational methods for settling velocity of solid particles in liquids[J]. Oil Drilling Process, 2000,(2):51-53,56-83. [20] 段自豪,陈杰,蒋昌波,等.非恒定流作用下的推移质泥沙输移实验研究[J].中国科学:技术科学, 2019,49(11):1372-1382. Duan P, Chen J, Jiang C, et al. Experimental study on bedload sediment transport under unsteady flow[J]. China Science:Technical Science, 2019,49(11):1372-1382. [21] 阮师,李光炽.水文水力学耦合模型及其应用[J].中国农村水利水电, 2013,(6):9-11,15. Ruan S, Li G. Hydrological and hydraulic coupling model and its application[J]. China Rural Water Conservancy and Hydropower, 2013,(6):9-11,15. [22] Komar P D, Baba J. Settling velocities of circular cylinders at low Reynolds numbers[J]. Journal of Sedimentary Research, 1980,Geol.88(3):327-336. [23] Wang Zhen, Dou Ming, Ren Pengju, et al. Settling velocity of irregularly shaped microplastics under steady and dynamic flow conditions[J]. Environmental Science and Pollution Research, 2021, 28(44):62116-62132. [24] 王振,窦明,任鹏举,等.基于沉降实验的微塑料静水沉降公式拟合[J].武汉大学学报(工学版), 2021,54(8):687-693. Wang Zhen, Dou Ming, Ren Pengju, et al. Fitting formula of microplastic hydrostatic settlement based on settlement experiment[J]. Journal of Wuhan University (Engineering Edition), 2021,54(8):687-693. [25] 刘修英,黄功学,郑志宏,等.贾鲁河郑州段水质评价和污染源解析[J].水资源保护, 2020,36(4):40-46. Liu Xiuying, Huang Gongxue, Zheng Zhihong, et al. Water quality evaluation and pollution source analysis of the Zhengzhou section of the Jialu River[J]. Water Resources Protection, 2020,36(4):40-46. [26] 谢志伟,雒天峰,李翔.梯形渠道流速分布规律及测流技术研究[J].人民黄河, 2008,(1):63-64. Xie Zhiwei, Luo Tianfeng, Li Xiang. Study on velocity distribution and flow measurement technology of trapezoidal channel[J]. People's Yellow River, 2008,(1):63-64. [27] Wang Chun, Jiang Lijuan, Liu Ruiqing, et al. Comprehensive assessment of factors influencing Nile red staining:Eliciting solutions for efficient microplastics analysis[J]. Marine Pollution Bulletin, 2021, 171:112698.