Evaluation for impact on PM2.5 pollution and healthy benefits of rural scattered coal replacement-a case study of Henan Province
YU Miao1,2, MA Qiu-hong3, ZHU Ming-yue1,2, ZHANG Jing-wang1,2, WANG Ke2,4, XU Qi-xiang2,4, ZHANG Rui-qin2,4
1. College of Chemistry, Zhengzhou University, Zhengzhou 450001, China; 2. Research Institute of Environmental Science, Zhengzhou University, Zhengzhou 450001, China; 3. Xiangcheng Branch of Zhoukou Ecological Environment Bureau, Zhoukou 466000, China; 4. School of Ecology and Environment, Zhengzhou University, Zhengzhou 450001, China
Abstract:The emission reduction by scattered coal replacement in the January of 2025 was predicted with a noble county-level optimization model, which was based on the air pollutant emissions inventory of rural coal combustion of Henan in 2016. Two scenarios were set to evaluate the emission reduction potentials of rural scattered coal replacement, including Business As Usual (BAU) and Scattered Coal Treatment (SCT) scenarios. The resulting air quality improvement and healthy benefits to public caused by rural scattered coal replacement were quantified by air quality model (WRF-CMAQ) and the Poisson regression model. Combination of the envelope structure renovation and heating equipment was the most suitable heating technology for rural households in Henan Province. In comparison to the BAU scenario, the emission intensity of SO2, NOx, CO, PM10, PM2.5, VOCs and NH3 in January 2025 from rural residential combustion in Henan Province were decreased by 98.3%, 82.6%, 99.8%, 99.2%, and 99.2% in the SCT scenario. Compared with BAU scenario, monthly average PM2.5 concentration in January 2025 of the SCT scenario could be reduced for 4.1μg/m3, which could prevent totally 220 premature deaths and economic loss of 2.35 billion RMB.
Cheng M, Zhi G, Tang W, et al. Air pollutant emission from the underestimated households' coal consumption source in China[J]. Science of The Total Environment, 2017,580:641-650.
[2]
支国瑞,杨俊超,张涛,等.我国北方农村生活燃煤情况调查、排放估算及政策启示[J]. 环境科学研究, 2015,28(8):1179-1185. Zhi G R, Yang J C, Zhang T, et al. Rural household coal use survey, emission estimation and policy implications[J]. Environmental Science Research, 2015,28(8):1179-1185.
[3]
赵文慧,姜磊,张立坤,等.北京平原区平房冬季燃煤量及污染物排放估算[J]. 中国环境科学, 2017,37(3):859-867. Zhao W H, Jiang L, Zhang L K, et al. Estimation of coal consumption and related contamination emission in the plain area around Beijing during winter season[J]. Chinese Environmental Science, 2017,37(3):859-867.
[4]
Liu J, Mauzerall D L, Chen Q, et al. Air pollutant emissions from Chinese households:a major and underappreciated ambient pollution source[J]. Proceedings of the National Academy of Sciences of the United States of America, 2016,113(28):7756-7761.
[5]
徐银鸿.北方典型地区农村清洁采暖污染物排放及综合效益评估[D]. 北京:北京化工大学, 2020. Xu Y H. Pollutant emission and comprehensive benefit evaluation of clean heating in typical northern rural areas in China[D]. Beijing:Beijing University of Chemical Technology, 2020.
[6]
闫祯,金玲,陈潇君,等.京津冀地区居民采暖"煤改电"的大气污染物减排潜力与健康效益评估[J]. 环境科学研究, 2019,32(1):95-103. Yan Z, Jin L, Chen X J, et al. Assessment of air pollutants emission reduction potential and health benefits for ‘residential heating coal changing to electricity’ in the Beijing-Tianjin-Hebei region[J]. Environmental Science Research, 2019,32(1):95-103.
[7]
李朋,吴华成,周卫青,等.京津冀"以电代煤"替代大气污染物排放清单[J]. 中国环境科学, 2021,41(4):1489-1497. Li P, Wu H C, Zhou W Q, et al. Emission inventory of atmospheric pollutants replaced by "coal-to-electricity" policy in Beijing-Tianjin-Hebei region[J]. Chinese Environmental Science, 2021,41(4):1489-1497.
[8]
吴文景,常兴,邢佳,等.京津冀地区主要排放源减排对PM2.5污染改善贡献评估[J]. 环境科学, 2017,38(3):867-875. Wu W J, Chang X, Xing J, et al. Assessment of PM2.5 pollution mitigation due to emission reduction from main emission sources in the Beijing-Tianjin-Hebei region[J]. Environmental Science, 2017, 38(3):867-875.
[9]
武娟妮,程亮,逯元堂,等.散煤采暖清洁化替代方式的生命周期清单分析[J]. 中国环境科学, 2018,38(4):1570-1578. Wu J N, Cheng l, Lu Y T, et al. Life cycle inventory analysis of clean alternatives to scattered coal heating[J]. Chinese Environmental Science, 2018,38(4):1570-1578.
[10]
王彦超,蒋春来,贺晋瑜,等.京津冀大气污染传输通道城市燃煤大气污染减排潜力[J]. 中国环境科学, 2018,38(7):2401-2405. Wang Y C, Jiang C L, He J Y, et al. Air pollutant emissions reduction potential from burning coal in cities of air pollution transmission channel in Beijing-Tianjin-Hebei area[J]. Chinese Environmental Science, 2018,38(7):2401-2405.
[11]
Zhang Q, Hao Y, Sun D, et al. Research on the clean energy heating systems in rural Beijing[J]. Energy Procedia, 2017,143:137-143.
[12]
戴海夏,安静宇,李莉,等.上海市实施清洁空气行动计划的健康收益分析[J]. 环境科学, 2019,40(1):24-32. Dai H X, An J Y, Li L, et al. Health benefit analyses of the clean air action plan implementing in Shanghai[J]. Environmental Science, 2019,40(1):24-32.
[13]
黄德生,张世秋.京津冀地区控制PM2.5污染的健康效益评估[J]. 中国环境科学, 2013,33(1):166-174. Huang D S, Zhang S Q. Health benefits evaluation for PM2.5 pollution control in Beijing-Tianjin-Hebei region of China.[J]. Environmental Science, 2013,33(1):166-174.
[14]
河南省统计局.河南省统计年鉴[M]. 北京:中国统计出版社, 2019. Henan provincial bureau of statistics. Henan statistical yearbook[M]. Beijing:China statistics press, 2019.
[15]
Peng L, Zhang Q, Yao Z, et al. Underreported coal in statistics:A survey-based solid fuel consumption and emission inventory for the rural residential sector in China[J]. Applied Energy, 2019,235:1169-1182.
[16]
Zhu M Y, Liu L, Yin S S, et al. County-level emission inventory for rural residential combustion and emission reduction potential by technology optimization:a case study of Henan, China[J]. Atmospheric Environment, 2020,228:117436.
[17]
河南省人民政府.河南省蓝天工程行动计划[EB/OL]. https://www.henan.gov.cn/2014/05-06/238864.html. The people's government of Henan province. Henan blue sky project action plan[EB/OL]. https://www.henan.gov.cn/2014/05-06/238864.html.
[18]
河南省发展和改革委员会.河南省天然气替代煤专项方案(2016~2020年)[EB/OL]. http://fgw.henan.gov.cn/2016/09-07/705142.html. The development and reform commission of Henan provincial. Henan Province natural gas substitutes coal special plan (2016~2020)[EB/OL]. http://fgw.henan.gov.cn/2016/09-07/705142.html.
[19]
河南省人民政府.河南省重污染天气应急应对攻坚战实施方案(2016~2017年)[EB/OL]. http://www.henan.gov.cn/2017/05-03/658861.html. The people's government of Henan province. Implementation plan for emergency response to heavy pollution weather in Henan Province (2016~2017)[EB/OL]. http://www.henan.gov.cn/2017/05-03/658861.html.
[20]
薛文博,武卫玲,付飞,等.中国2013年1月PM2.5重污染过程卫星反演研究[J]. 环境科学, 2015,36(3):794-800. Xue W B, Wu W L, Fu F, et al. Satellite retrieval of a heavy pollution process in january 2013 in China[J]. Environmental Science, 2015, 36(3):794-800.
[21]
河南省人民政府.河南省能源中长期发展规划(2012~2030年)[EB/OL]. https://www.henan.gov.cn/2013/06-19/238624.html. The people's government of Henan province. Energy medium and long-term development plan of Henan Province (2012~2030)[EB/OL]. https://www.henan.gov.cn/2013/06-19/238624.html.
[22]
戴彦德,胡秀莲.中国二氧化碳减排技术潜力和成本研究[M]. 北京:中国环境出版社, 2013. Dai Y D, Hu X L. Potential and cost study on China's carbon mitigation technologies[M]. Beijing:China Environment Press, 2013.
[23]
马涛,庞莉,胡国斌.空气源热泵在北京市农村"煤改电"中的经济效益分析[J]. 农电管理, 2018,(1):33-34. Ma T, Pang L, Hu G B. Analysis on the economic benefits of air source heat pump in Beijing rural "coal to electricity"[J]. Rural Power Management, 2018,(1):33-34.
[24]
王敏,王选,黄祝连,等.寒冷地区农村住宅主被动太阳能结合采暖系统的技术经济性分析[J]. 建筑科学, 2011,27(S2):139-142. Wang M, Wang X, Huang Z L, et al. Technical and Economic Analysis of Combined Active and Passive Solar Space Heating System for Rural[J]. Building Science, 2011,27(S2):139-142.
[25]
姚新强,赵家伟,刘晨军,等.严寒地区农村住宅围护结构节能改造设计及经济性分析[J]. 砖瓦, 2019,(5):64-66. Yao X Q, Zhao J W, Liu C J, et al. Energy-saving renovation design and economic analysis of rural residential building envelopes in severe cold regions[J]. Brick-Tile, 2019,(5):64-66.
[26]
Zhang Q, David G. Streets, He K B, et al. NOx emission trends for China, 1995~2004:The view from the ground and the view from space[J]. Journal of Geophysical Research:Earth Surface, 2007,112(D22).
[27]
D. G. Streets, T. C. Bond, G. R. Carmichael, et al. An inventory of gaseous and primary aerosol emissions in Asia in the year 2000[J]. Journal of Geophysical Research:Earth Surface, 2003,108(D21).
[28]
Zhi G, Zhang Y, Sun J, et al. Village energy survey reveals missing rural raw coal in northern China:Significance in science and policy[J]. Environmental Pollution, 2017,223:705-712.
[29]
Cai S, Li Q, Wang S, et al. Pollutant emissions from residential combustion and reduction strategies estimated via a village-based emission inventory in Beijing[J]. Environmental Pollution, 2018, 238:230-237.
[30]
中华人民共和国环境保护部.清单编制技术指南(试行)[EB/OL]. http://www.mee.gov.cn/gkml/hbb/bgg/201501/t20150107_293955.htm. Ministry of environmental protection of the people's republic of China. Technical guidelines for inventory development (trial)[EB/OL]. http://www.mee.gov.cn/gkml/hbb/bgg/201501/t20150107_293955.htm.
[31]
田贺忠,郝吉明,陆永琪,等.中国氮氧化物排放清单及分布特征[J]. 中国环境科学, 2001,(6):14-18. Tian H Z, Hao J M, Lu Y Q, et al. Inventories and distribution characteristics of NOx emissions in China[J]. Chinese Environmental Science, 2001,(6):14-18.
[32]
王丽涛,张强,郝吉明,等.中国大陆CO人为源排放清单[J]. 环境科学学报, 2005,(12):8-13. Wang L T, Zhang Q, Hao J M, et al. Anthropogenic CO emission inventory of mainland China[J]. Acta Scientiae Circumstantiae, 2005,(12):8-13.
[33]
Zhang J, Smith K R, Ma Y, et al. Greenhouse gases and other airborne pollutants from household stoves in China:A database for emission factors[J]. Atmospheric Environment, 2000,34(26):4537-4549.
[34]
Zheng J, Zhang L, Che W, et al. A highly resolved temporal and spatial air pollutant emission inventory for the Pearl River Delta region, China and its uncertainty assessment[J]. Atmospheric Environment, 2009,43(32):5112-5122.
[35]
He M, Zheng J, Yin S, et al. Trends, temporal and spatial characteristics, and uncertainties in biomass burning emissions in the Pearl River Delta, China[J]. Atmospheric Environment, 2011,45(24):4051-4059.
[36]
Wei W, Wang S, Chatani S, et al. Emission and speciation of non-methane volatile organic compounds from anthropogenic sources in China[J]. Atmospheric Environment, 2008,42(20):4976-4988.
[37]
Liu S, Hua S, Wang K, et al. Spatial-temporal variation characteristics of air pollution in Henan of China:Localized emission inventory, WRF/Chem simulations and potential source contribution analysis[J]. Science of the Total Environment, 2018,624:396-406.
[38]
Zhong Z, Zheng J, Zhu M, et al. Recent developments of anthropogenic air pollutant emission inventories in Guangdong province, China[J]. Science of The Total Environment, 2018,627:1080-1092.
[39]
河南省人民政府.河南省人口发展规划(2016~2030年)[EB/OL]. https://www.henan.gov.cn/2017/05-25/248952.html. The people's government of Henan province. Population development plan of Henan province (2016~2030)[EB/OL]. https://www.henan.gov.cn/2017/05-25/248952.html.
[40]
Bai L, Lu X, Yin S S, et al. A recent emission inventory of multiple air pollutant, PM2.5 chemical species and its spatial-temporal characteristics in central China[J]. Journal of Cleaner Production, 2020,269:122114.
王杰.中国空气质量在线监测分析平台[EB/OL]. https://www.aqistudy.cn/historydata/about.php. Wang J. Air quality online monitoring and analysis platform in China[EB/OL]. https://www.aqistudy.cn/historydata/about.php.
[43]
James W B, Armistead G R. PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models[J]. Atmospheric Environment, 2005,40(26):4946-4959.
[44]
中国环境监测总站.环境空气质量预报预警方法技术指南[M]. 北京:中国环境科学出版社, 2014. China national environmental monitoring centre. Technical guide for ambient air quality forecast and early warning methods[M]. Beijing:China Environmental Science Press, 2014.
[45]
朱媛媛,高愈霄,刘冰,等.京津冀秋冬季PM2.5污染概况和预报结果评估[J]. 环境科学, 2019,40(12):5191-5201. Zhu Y Y, Gao Y X, Liu B, et al. Concentration characteristics and assessment of model-predicted results of PM2.5 in the Beijing-Tianjin-Hebei region in autumn and winter[J]. Environmental Science, 2019,40(12):5191-5201.
[46]
郁莎燕.重大事件空气质量管控措施的健康效益评估-以南京市青奥会为例[D]. 南京:南京大学, 2019:75-76. Yu S Y. Health benefit assessment of air quality control measures for major events-taking the 2014 Nanjing Youth Olympic Games as an example[D]. Nanjing:Nanjing University, 2019:75-76.
[47]
谢元博,陈娟,李巍.雾霾重污染期间北京居民对高浓度PM2.5持续暴露的健康风险及其损害价值评估[J]. 环境科学, 2014,35(1):1-8. Xie Y B, Chen J, Li W. An assessment of PM2.5 related health risks and impaired values of Beijing residents in a consecutive high-level exposure during heavy haze days[J]. Environmental Science, 2014, 35(1):1-8.
[48]
谢鹏,刘晓云,刘兆荣,等.我国人群大气颗粒物污染暴露-反应关系的研究[J]. 中国环境科学, 2009,29(10):1034-1040. Xie P, Liu X Y, Liu Z R, et al. Exposure-response functions for health effects of ambient particulate matter pollution applicable for China[J]. Environmental Science, 2009,29(10):1034-1040.
[49]
World Health Organization. Air quality guidelines for particulate matter, ozone, nitrogen dioxide and sulfur dioxide[R]//Global Update 2005. Switzerland:World Health Organization, 2006.
[50]
Shang Y, Sun Z W, Cao J J, et al. Systematic review of Chinese studies of short-term exposure to air pollution and daily mortality[J]. Environment International, 2013,54:100-111.
[51]
国家卫生和计划生育委员会.2017中国卫生和计划生育统计年鉴[M]. 北京:中国协和医科大学出版社, 2017. National health and family planning. China health and family planning statistical yearbook in 2017[M]. Beijing:Peking Union Medical College Press, 2017.
[52]
魏国茹,史兴民.西安市PM2.5健康损害价值评估[J]. 环境科学, 2018,39(7):3014-3021. Wei G R, Shi X M. Evaluation the extent of health damage caused by PM2.5 particulate in Xi'an[J]. Environmental Science, 2018,39(7):3014-3021.
[53]
谢旭轩.健康的价值:环境效益评估方法与城市空气污染控制策略[D]. 北京:北京大学, 2011. Xie X X, The value of health:Environmental benefit assessment methods and urban air pollution control strategies[D]. Beijing:Beijing University, 2011.
[54]
Boylan J W, Russell A G. P M and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models[J]. Atmospheric Environment, 2006,40(26):4946-4959.
[55]
陈楚,王体健,李源昊,等.濮阳市秋冬季大气细颗粒物污染特征及来源解析[J]. 环境科学, 2019,40(8):3421-3430. Chen C, Wang T J, Li Y H, et al. Pollution characteristics and source apportionment of fine particulate matter in autumn and winter in Puyang, China[J]. Environmental Science, 2019,40(8):3421-3430.