Impact of the coal-to-electricity policy on PM2.5 concentration in Beijing-Tianjin-Hebei region
ZHANG Ru-ting1, CHEN Chuan-min1, WU Hua-cheng2, ZHOU Wei-qing2, LI Peng2
1. College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, China; 2. Jibei Electric Power Research Institute, State Grid Jibei Electric Power Co., Ltd., North China Electric Power Research Institute Company Limited, Beijing 100045, China
Abstract:Based on the Weather Research and Forecasting Model with Chemistry(WRF-Chem) model and combined with the meteorological parameters, the variation of PM2.5 emission before and after the implementation of the coal-to-electricity policy during the heating period(November 2018 to March 2019) over the BTH region was simulated and analyzed from the aspects of the PM2.5 concentration reduction and its spatial-temporal variation characteristic. The WRF-Chem model well stimulated the variation of PM2.5 concentration over the BTH region, and the correlation coefficient between simulated values and observed values in Beijing,Tianjin and Shijiazhuang were 0.66, 0.66 and 0.52, respectively, showing a good correlation. The implementation of the coal-to-electricity policy had an obvious effect on the reduction of PM2.5 concentration in key areas over the BTH region. The average daily mean reduction of PM2.5 was 0.2~6.1μg/m3, and the average reduction ratio was 1.2%~7.8%. The variation of the PM2.5 hourly mean concentration showed that the average reduction of PM2.5 in December 2018 was 0.4~8.3μg/m3, and the average reduction ratio was 2.3%~7.7%. Particularly, the emission reduction in Daxing District of Beijing reached 8.3μg/m3, while the reduction ratio in Tianjin area reached 7.7%. Under special meteorological conditions, the scope of the coal-to-electricity policy over the BTH region could spread to Shandong, Jiangsu, Henan and the western of Shanxi, and the maximum hourly mean reduction of PM2.5 was more than 50μg/m3.
GB3095-2012环境保护部.环境空气质量标准[S].GB3095-2012 ambient air quality standards[S].
[2]
生态环境部.2018年中国国家环境监测中心实时数据库[EB/OL]http://106.37.208.233:20035/.Ministry of Ecology and Environment. 2018 China national environmental monitoring center real-time database[EB/OL] http://106.37.208.233:20035/.
[3]
国家统计局.中国统计年鉴[M].北京:中国统计出版社, 2018.National Bureau of Statistics in China. China statistical yearbook[M].Beijing:China Statistics Press, 2018.
[4]
Shen G F, Ru M Y, Du W, et al. Impacts of air pollutants from rural Chinese households under the rapid residential energy transition[J].Nature Communications, 2019,10(1):3405.
[5]
Zhang X, Jin Y N, Dai H C, et al. Health and economic benefits of cleaner residential heating in the Beijing-Tianjin-Hebei region in China[J]. Energy Policy, 2019,127(Apr.):165-178.
[6]
Liu J, Mauzerall D L, Qi C, et al. Air pollutant emissions from Chinese households:A major and underappreciated ambient pollution source[J]. Proc. Natl. Acad. Sci. U S A, 2016,113(28):7756-7761.
[7]
Streets D G, Gupta S, Waldhoff S T, et al. Black carbon emissions in China[J]. Atmospheric Environment, 2001,35(25):4281-4296.
[8]
Zhang J F, Smith K R. Household air pollution from coal and biomass fuels in China:Measurements, health impacts, and interventions[J].Environmental Health Perspectives, 2007,115(6):848-855.
[9]
Chen Y L, Shen H Z, Smith K R, et al. Estimating household air pollution exposures and health impacts from space heating in rural China[J]. Environment International, 2018,119:117-124.
[10]
Yun X, Shen G F, Shen H Z, et al. Residential solid fuel emissions contribute significantly to air pollution and associated health impacts in China[J]. Science Advances, 2020,6(44).
[11]
中国国家发展和改革委员会.中国北方冬季清洁采暖工作计划(2017-2021年)[Z].National Development and Reform Commission of China. Work plan for clean heating in winter in northern China (2017-2021)[Z].
[12]
Chen Z X, Zhang D L, Jiang H R, et al. Environmental benefits evaluation of coal-to-electricity project in Beijing, China[J].Environmental Science and Pollution Research, 2020,24(5).
[13]
Dennis R L, Byun D W, Novak J H, et al. The next generation of integrated air quality modeling:EPA's Models-3[J]. Atmospheric Environment, 1996,30(12):1925-1938.
[14]
Environ. User's guide to the comprehensive air quality modeling system with extensions (CAMx)[Z]. Version 4.4. 2002:10-44.
[15]
Wu Q Z, Shi A, Li Y, et al. Air quality forecast of PM10 in Beijing with Community Multi-scale Air Quality Modeling (CMAQ) system:emission and improvement[J]. Geoscientific Model Development,2014,7:2243-2259.
[16]
王德羿,王体健,韩军彩,等."2+26"城市大气重污染下PM2.5来源解析[J].中国环境科学, 2020,40(1):92-99.Wang D Y, Wang T J, Han J C, et al. Source apportionment of PM2.5under heavy air pollution conditions in "2+26" cities[J]. China Environmental Science, 2020,40(1):92-99.
[17]
Wu D W, Fung J C H, Yao T, et al. A study of control policy in the Pearl River Delta region by using the particulate matter source apportionment method[J]. Atmospheric Environment, 2013,76(Sep.):147-161.
[18]
Wang Z F, Jie L I, Wang Z, et al. Modeling study of regional severe hazes over mid-eastern China in January 2013 and its implications on pollution prevention and control[J]. Science China Earth Sciences,2014,57(1):3-13.
[19]
Wang T J, Jiang F, Deng J J, et al. Urban air quality and regional haze weather forecast for Yangtze River Delta region[J]. Atmospheric Environment, 2012,58(Oct.):70-83.
[20]
Tie X, Madronich S, Li G, et al. Simulation of Mexico City plumes during the MIRAGE-Mex field campaign using the WRF-Chem model[J]. Atmospheric Chemistry & Physics Discussions, 2009,9(14):4621-4638.
[21]
Zhang L, Wang T, Lv M Y, et al. On the severe haze in Beijing during January 2013:Unraveling the effects of meteorological anomalies with WRF-Chem[J]. Atmospheric Environment, 2015,104(Mar.):11-21.
[22]
Sha T, Ma X Y, Jia H L, et al. Aerosol chemical component:Simulations with WRF-Chem and comparison with observations in Nanjing[J]. Atmospheric environment, 2019,218(Dec.):116982.1-116982.14.
[23]
Liu C, Huang J P, Hu X M, et al. Evaluation of WRF-Chem simulations on vertical profiles of PM2.5with UAV observations during a haze pollution event[J]. Atmospheric Environment, 2021:118332-118343.
[24]
Liu J, Mauzerall D L, Chen Q, et al. Air pollutant emissions from Chinese households:A major and underappreciated ambient pollution source[J]. Proc. Natl. Acad. Sci. U S A, 2016,113(28):7756-7761.
[25]
Bilsback K R, Baumgartner J, Cheeseman M, et al. Estimated Aerosol Health and Radiative Effects of the Residential Coal Ban in the Beijing-Tianjin-Hebei Region of China[J]. Aerosol and Air Quality Research, 2020,20(11):2332-2346.
[26]
Meng W J, Zhong Q R, Chen Y L, et al. Energy and air pollution benefits of household fuel policies in northern China[J]. Proceedings of the National Academy of Sciences, 2019,116(34):201904182.
[27]
Skamarock W C, Klemp J B, Dudhia J. Prototypes for the WRF (Weather Research and Forecasting) model[Z]. Preprints, 2001.
[28]
余钟奇,瞿元昊,周广强,等.2018年秋冬季长江三角洲区域PM2.5污染来源数值研究[J].中国环境科学, 2020,40(10):64-73.Yu Z Q, Qu Y H, Zhou G Q, et al. Numerical simulations of PM2.5pollution source in the Yangtze River Delta region in fall and winter in 2018[J]. China Environmental Science, 2020,40(10):64-73.
[29]
Zaveri R A, Peters L K. A new lumped structure photochemical mechanism for large-scale applications[J]. Journal of Geophysical Research Atmospheres, 1999,104(23):30387-30415.
[30]
Wild O, Zhu X, Prather M J, et al. Accurate simulation of in-and below-cloud photolysis in tropospheric chemical models[J]. Journal of Atmospheric Chemistry, 2000,37(3):245-282.
[31]
Barnard J C, Chapman E G, Fast J D, et al. An evaluation of the FAST-J photolysis algorithm for predicting nitrogen dioxide photolysis rates under clear and cloudy sky conditions[J].Atmospheric Environment, 2004,38(21):3393-3403.
[32]
Zaveri R A, Easter R C, Fast J D, et al. Model for simulating aerosol Interactions and chemistry (MOSAIC).[J]. Journal of Geophysical Research Atmospheres, 2008,113(D13204).
[33]
Kain J S. The kain-fritsch convective parameterization:an update[J].Journal of Applied Meteorology, 2004,43:170-181.
[34]
Lin Y L, Farley R D, Orville H D. Bulk parameterization of the snow field in a cloud model[J]. Journal of Applied Meteorology and Climatology, 1983,22(6):1065-1092.
[35]
Mlawer E J, Taubman S J, Brown P D, et al. Radiative transfer for inhomogeneous atmospheres:RRTM, a validated correlated-k model for the longwave[J]. Journal of Geophysical Research Atmospheres,1997,102(D104):16663-16682.
[36]
Dudhia J. Numerical study of convection observed during the winter monsoon experiment using a mesoscale two-dimensional model[J].Journal of Atmospheric Sciences, 1989,46:3077-3107.
[37]
Janji Z I. Nonsingular implementation of the Mellor-Yamada level 2.5scheme in the NCEP meso model[J]. NCEP Office Note, 2002, 437.
[38]
Janji Z I. The step-mountain eta coordinate model:further developments of the convection, viscous sublayer, and turbulence closure schemes[J].Monthly Weather Reviewer, 1994,122(5):927-945.
[39]
Monin A S, Obukhov A M. Basic laws of turbulent mixing in the surface layer of the atmosphere[J]. Contrib. Geophys. Inst. Acad. Sci.,1954,24(151):163-187.
[40]
Hong S Y, Pan H L. Nonlocal boundary layer vertical diffusion in a medium-range forecast model[J]. Monthly Weather Reviewer, 1996,124(10):2322-2339.
[41]
Chen F, Dudhia J. Coupling an advanced land surface-hydrology model with the penn state-NCAR MM5 modeling system. Part I:model implementation and sensitivity[J]. Monthly Weather Reviewer,2001,129(4):569-585.
[42]
李朋,吴华成,周卫青,等.京津冀"煤改电"替代大气污染物排放清单[J].中国环境科学, 2021,41(4):1489-497.Li P, Wu H C, Zhou W Q, et al. Emission inventory of atmospheric pollutants replaced by "coal-to-electricity" policy in Beijing-TianjinHebei region[J]. China Environmental Science, 2021,41(4):1489-497.
[43]
周广强,谢英,吴剑斌,余钟奇,常炉予,高伟.基于WRF-Chem模式的华东区域PM2.5预报及偏差原因[J].中国环境科学, 2016,36(8):2251-2259.Zhou G Q, Xie Y, Wu J B, et al. WRF-Chem based on PM2.5 forecast and bias analysis over the East China Region[J]. China Environmental Science, 2016,36(8):2251-2259.
[44]
Zhang B, Wang Y X, Hao J M. Simulating aerosol-radiation-cloud feedbacks on meteorology and air quality over eastern China under severe haze conditions in winter[J]. Atmospheric Chemistry and Physics, 2015,14(5):2387-2404.
[45]
张晗宇,温维,程水源,等.京津冀区域典型重污染过程与反馈效应研究[J].中国环境科学, 2018,38(4):1209-1220.Zhang H Y, Wen W, Cheng S Y, et al. Study on typical heavy pollution process and feedback effect in Beijing-Tianjin-Hebei region[J].China Environmental Science, 2018,38(4):1209-1220.
[46]
US EPA (Environmental Protection Agency). Guidance on the use of models and other analyses for demonstrating attainment of air quality goals for ozone, PM2.5, and regional haze[EB/OL]. https://nepis.epa.gov/Exe/ZyPDF.cgi/P1009OL1.PDF?Dockey=P1009OL1.PDF.
[47]
Boylan J W, Russell A G. PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models[J].Atmospheric Environment, 2005,40(26):4946-4959.
[48]
Emery C, Liu Z, Russell A G, et al. Recommendations on statistics and benchmarks to assess photochemical model performance[J]. Air Waste Management Association, 2017,67(5):582-598.
[49]
闫祯,金玲,陈潇君,等.京津冀地区居民采暖"煤改电"的大气污染物减排潜力与健康效益评估[J].环境科学研究, 2019,32(1):101-109.Yan Z, Jing L, Chen X J, et al. Assessment of air pollutants emission reduction potential and health benefits for "residential heating coal changing to electricity" in the Beijing-Tianjin-Hebei Region[J].China Environmental Science, 2019,32(1):101-109.
[50]
李珊珊,程念亮,徐峻,等.2014年京津冀地区PM2.5浓度时空分布及来源模拟[J].中国环境科学, 2015,35(10):2908-2916.Li S S, Cheng N L, Xu J, et al. Spatial and temporal distributions and source simulation of PM2.5 in Beijing-Tianjin-Hebei region in 2014[J]. China Environmental Science, 2015,35(10):2908-2916.
[51]
Liu J, Mauzerall D L, Qi C, et al. Air pollutant emissions from Chinese households:A major and underappreciated ambient pollution source[J]. Proc Natl Acad Sci U S A, 2016,113(28):7756-7761.
[52]
王彦超,蒋春来,贺晋瑜,等.京津冀大气污染传输通道城市燃煤大气污染减排潜力[J].中国环境科学, 2018,38(7):2401-2405.Wang Y C, Jiang C L, He J Y,, et al. Air pollutant emissions reduction potential from burning coal in cities of air pollution transmission channel in Beijing-Tianjin-Hebei area[J]. China Environmental Science, 2018,38(7):2401-2405.
[53]
Zheng B, Dan T, Meng L, et al. Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions[J].Atmospheric Chemistry & Physics Discussions, 2018,18(19):14095-14111.
[54]
Xie X, Ai H S, Deng Z G. Impacts of the scattered coal consumption on PM2.5 pollution in China[J]. Journal of Cleaner Production,2019,245:118922.