云南省优势矿产尾矿砂捕集及矿化封存CO<sub>2</sub>潜力分析

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摘要为了解云南省尾矿库“两个清单”中保留库的碳减排潜力,使用改进的Steinour方程计算了云南省各州市不同类型尾矿砂的CO₂固定量,根据《IPCC国家温室气体列表指南》中提供的方法计算了云南省2011~2020年碳排放量.结果表明,红河州、玉溪市、昆明市尾矿砂的捕集及矿化封存CO₂的潜力较大,占云南省保留库尾矿砂CO₂矿化封存量的65.79%;铅锌矿、赤泥、锡矿的理论固碳量较高,分别为0.201, 0.173, 0.158t/t,以上3种尾矿砂的固碳量占云南省尾矿砂固碳量的79.45%;若将云南省保留库堆存的尾矿砂全部用于CO₂的矿化封存,可减少2011~2020年间云南省累积碳排放量的2.81%,工业碳累积排放量的3.16%,采矿业碳排放量的12.36%,具有较好的工业应用前景.

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	张云
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	胡学伟

关键词 ：矿化封存, 改进的Steinour方程, 尾矿砂, 碳排放, 云南省

Abstract：The modified Steinour equation was used to calculate the CO₂ mineralization of different types of tailings in various cities of Yunnan Province to understand the potential for mitigating carbon emissions from the reserve ponds on the "two lists" of tailings ponds in Yunnan Province. The carbon emissions in Yunnan Province from 2011 to 2020 were estimated using the method provided in IPCC Guidelines for National Greenhouse Gas Inventory. The tailings in Honghe Prefecture, Yuxi City, and Kunming City revealed a high potential for CO₂ sequestration, accounting for 65.79% of the total CO₂ mineralization sequestration of tailings in Yunnan Province. The theoretical carbon sequestration rate of lead-zinc ore, red mud, and tin ore is relatively high, being 0.201, 0.173, and 0.158t/t, respectively. The carbon sequestration of above three tailings accounts for 79.45% of the total carbon sequestration of tailings in Yunnan Province. By using all the reserved tailings for CO₂ mineralization and sequestration in Yunnan Province, the accumulated carbon emissions from 2011 to 2020 will be reduced by 2.81%, 3.16% from the industrial sector, and 12.36% from the mining sector. In summary, CO₂ capture and mineralization sequestration of tailings could serve as green technologies under dual carbon targets in China.

Key words： mineral sequestration modified Steinour equation tailings carbon emission Yunnan Province

收稿日期: 2022-02-25

PACS:

X22

基金资助:国家重点研发计划(2018YFC1802603);云南省生态环境厅环保技术研究项目(YNJH2019224);矿物加工科学与技术国家重点实验室开放基金(BGRIMM-KJSKL-2022-08)

通讯作者: 胡学伟,教授,huxuewei@kust.edu.cn E-mail: huxuewei@kust.edu.cn

作者简介: 张云(1988-),女,四川会理人,昆明理工大学博士研究生,主要从事二氧化碳捕集与封存方向的研究.发表论文10余篇.

引用本文:

张云, 胡寒, 周宏辉, 田森林, 黄建洪, 胡学伟. 云南省优势矿产尾矿砂捕集及矿化封存CO₂潜力分析[J]. 中国环境科学, 2022, 42(9): 4351-4361. ZHANG Yun, HU Han, ZHOU Hong-hui, TIAN Sen-lin, HUANG Jian-hong, HU Xue-wei. Potential of CO₂ capture and mineralization of dominant mineral tailings in Yunnan Province. CHINA ENVIRONMENTAL SCIENCECE, 2022, 42(9): 4351-4361.

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http://www.zghjkx.com.cn/CN/ 或 http://www.zghjkx.com.cn/CN/Y2022/V42/I9/4351

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