Research on optimizing air pollutant emission inventory based on electricity consumption data
ZHOU Wei-qing1, LI Peng1, WU Hua-cheng1, HE Xue-juan2, SUN Shi-da2, BO Yu2,3, HE Ke-bin3
1. Jibei Electric Power Research Institute, State Grid Jibei Electric Power Co., Ltd., (North China Electric Power Research Institute Company Limited), Beijing 100045, China; 2. Ministry of Education Key Laboratory for Earth System Modeling, Institute for Global Change Studies, Department of Earth System Science, Tsinghua University, Beijing 100084, China; 3. State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
Abstract:In order to improve the spatial and temporal resolution of the air pollutant emission inventory in the industrial sector, the method of optimizing the time and spatial distribution in the industrial sector based on the electricity consumption data was proposed, and taken Tangshan city, Hebei province as an example, the basic emission inventory and the optimized emission inventory were input into the WRF-CMAQ model to verify its optimization effect. The results showed that the WRF-CMAQ model well simulated the temporal variation and spatial distribution of pollutant concentrations in Tangshan in January, April, July and October 2019. Compared with the basic emission inventory, the correlation between the annual average simulation value and the monitoring value of PM2.5 in the optimized emission inventory increased by 3.3%, with the best improvement effect on NO2. The improvement effect was the most obvious in October, with the DR2 of PM2.5, PM10 and CO exceeded 1.4. The change of PM2.5 concentration in the optimized emission inventory had more obvious regional characteristics, with high value areas of difference appeared in some areas, such as Qianxi county and Zunhua city. The optimized emission inventory improved the accuracy of spatial simulation to a certain extent, and can better reflect the changes of pollutant emissions in the industrial sector.
周卫青, 李朋, 吴华成, 何学娟, 孙世达, 薄宇, 贺克斌. 基于电力数据优化大气污染物排放清单[J]. 中国环境科学, 2023, 43(7): 3350-3359.
ZHOU Wei-qing, LI Peng, WU Hua-cheng, HE Xue-juan, SUN Shi-da, BO Yu, HE Ke-bin. Research on optimizing air pollutant emission inventory based on electricity consumption data. CHINA ENVIRONMENTAL SCIENCECE, 2023, 43(7): 3350-3359.
吴文景,常 兴,邢 佳,等.京津冀地区主要排放源减排对PM2.5污染改善贡献评估 [J]. 环境科学, 2017,38(3):867-875. Wu W J, Chang X, Xing J, et al. Assessment of PM2.5 pollution mitigation due to emission reduction from main emission sources in the Bejing-Tianjin-Hebei Region [J]. Environmental Science, 2017, 38(3):867-875.
[2]
胡亚男,马晓燕,沙 桐,等.不同排放源对华东地区PM2.5影响的数值模拟 [J]. 中国环境科学, 2018,38(5):1616-1628. Hu Y N, Ma X Y, Sha T, et al. Impact of different emission sources on PM2.5 over East China based on numerical study [J]. China Environmental Science, 2018,38(5):1616-1628.
[3]
汤 铃,贾 敏,伯 鑫,等.中国钢铁行业排放清单及大气环境影响研究 [J]. 中国环境科学, 2020,40(4):1493-1506. Tang L, Jia M, Bo X, et al. High resolution emission inventory and atmospheric environmental impact research in Chinese iron and steel industry [J]. China Environmental Science, 2020,40(4):1493-1506.
[4]
王永红,薛志钢,柴发合,等.我国水泥工业大气污染物排放量估算 [J]. 环境科学研究, 2008,21(2):207-212. Wang Y H, Xue Z G, Cai F H, et al. Estimation of Air Pollutants Emissions of Cement Industry in China [J]. Research of Environmental Sciences, 2008,21(2):207-212.
[5]
汤 铃,薛晓达,伯 鑫,等.中国水泥排放清单及分布特征 [J]. 环境科学, 2020,41(11):4776-4785. Tang L, Xue X D, Bo X, ET AL. Contribution of Emissions from Cement to Air Quality in China [J]. Environmental Science, 2020, 41(11):4776-4785.
[6]
郑昊天,赵 斌,王书肖,等.钢铁与焦化行业大气污染物排放及空气质量影响分析 [J]. 环境影响评价, 2020,42(4):16-21. Zheng H T, Zhao B, Wang S X, et al. Air Pollutant Emissions From Steel and Coking Industries and Their Impacts on Ambient Air Quality in China [J]. Environmental Impact Assessment, 2020,42(4):16-21.
[7]
钟悦之,宋晓晖,王彦超,等.中国平板玻璃行业大气污染物排放特征研究 [J]. 中国环境科学, 2018,38(12):4451-4459. Zhong Y Z, Song X H, Wang Y C, et al. Emission characteristics from flat-glass industry in China [J]. China Environmental Science, 2018, 38(12):4451-4459.
[8]
刘 晓,胡京南,王红梅,等.基于多源数据融合的河南省建材行业排放清单 [J]. 环境科学, 2023,44(4):1924-1932. Liu X, Hu J N, Wang H M, et al. Emission Inventory of Building Materials Industry in Henan Province Based on Multi-source Data Integration [J]. Environmental Science, 2023,44(4):1924-1932.
[9]
Liu H, Wu B, Liu S, et al. A regional high-resolution emission inventory of primary air pollutants in 2012 for Beijing and the surrounding five provinces of north China [J]. Atmospheric Environment, 2018,181:20-33.
[10]
Ma X, Sha T, Wang J, et al. Investigating impact of emission inventories on PM2.5 simulations over north China plain by WRF-Chem [J]. Atmospheric Environment, 2018,195:125-140.
[11]
伯 鑫,何友江,商国栋,等.基于CEMS全国污染源清单数据库系统开发与应用 [J]. 环境工程, 2014,21(8):105-113. Bo X, He Y J, Shang G D, et al. Development and application of the national pollution emission inventory database system with CEMS [J]. Environmental Engineering, 2014,21(8):105-113.
[12]
伯 鑫,甄瑞卿,屈加豹,等.中国钢铁行业大气污染物排放清单管理系统研究 [J]. 环境污染与防治, 2017,39(5):578-582. Bo X, Zhen R Q, Qu J B, et al. Study on the management system of atmospheric pollutant emission inventory for steel industry of China [J]. Environmental Protection Technology, 2017,39(5):578-582.
[13]
伯 鑫,赵春丽,吴 铁,等.京津冀地区钢铁行业高时空分辨率排放清单方法研究 [J]. 中国环境科学, 2015,35(8):2554-2560. Bo X, Zhao C L, Wu T, et al. Emission inventory with high temporal and spatial resolution of steel industry in the Beijing-Tianjin-Hebei Region [J]. China Environmental Science, 2015,35(8):2554-2560.
[14]
何 敏,陈军辉,韩 丽,等.四川省2008~2014年水泥行业大气污染物排放清单及时空分布特征 [J]. 环境科学学报, 2017,37(1):34-43. He M, Chen J H, Han L, et al. Cement industrial emission inventories development and their temporal and spatial distribution for Sichuan province from 2008~2014 [J]. Acta Scientiae Circumstantiae, 2017, 37(1):34-43.
[15]
刘 扬,王 颖,刘 灏,等.基于WRF-Chem模拟验证的天水市主城区大气污染源排放清单 [J]. 中国环境科学, 2022,42(1):32-42. Liu Y, Wang Y, Liu H, et al. Air pollutants emission inventory for the main urban area of Tianshui City based on verification by WRF-Chem simulation [J]. China Environmental Science, 2022,42(1):32-42.
[16]
毛红梅,张凯山,第宝锋,等.成都市大气污染物排放清单高分辨率的时空分配 [J]. 环境科学学报, 2017,37(1):23-33. Mao H M, Zhang K S, Di B F, et al. The high-resolution temporal and spatial allocation of emission inventory for Chengdu [J]. Acta Scientiae Circumstantiae, 2017,37(1):23-33.
[17]
何 斌,梅士龙,陆琛莉,等.MEIC排放清单在空气质量模式中的应用研究 [J]. 中国环境科学, 2017,37(10):3658-3668. He B, Mei S L, Lu C L, et al. The application of MEIC emission inventory in air quality model [J]. China Environmental Science, 2017,37(10):3658-3668.
[18]
杨文夷,李 杰,朱莉莉,等.我国空气污染物人为源排放清单对比 [J]. 环境科学研究, 2013,26(7):703-711. Yang W Y, Li J, Zhu L L, et al. Comparison of Anthropogenic Emission Inventories of China [J]. Research of Environmental Sciences, 2013,26(7):703-711.
[19]
陈建华,李 政,刘翰青,等.基于企业用电数据的大气污染防治工作研究进展 [J]. 环境工程技术学报, 2023,13(2):510-516. Chen J H, Li Z, Liu H Q, et al. Research progress of air pollution prevention and control based on enterprise electricity consumption data [J]. Journal of Environmental Engineering Technology, 2023, 13(2):510-516.
[20]
奚增辉,王卫斌,洪祎祺,等.基于电力大数据的大气污染物实时排放总量测算研究 [J]. 环境科学与管理, 2022,47(5):77-81. Xi Z H, Wang W B, Hong Y Q, et al. Estimation of real-time emissions of air pollutants based on electric power big data [J]. Environmental Science and Management, 2022,47(5):77-81.
[21]
李 睿.电力大数据在大气污染精准防控领域的应用及建议 [J]. 环境保护, 2022,50(10):28-31. Li R. Application and suggestion of power big data in the field of air pollution precise prevention and control [J]. Environmental Protection, 2022,50(10):28-31.
[22]
吴佳静,贾 璐.电力大数据在生态保护中的应用探索 [J]. 中国电力企业管理, 2022,20:60-61. Wu J J, Jia L. Exploration on the application of power big data in ecological protection [J]. China Power Enterprise Management, 2022, 20:60-61.
[23]
张 沛,杨华飞,许元斌.电力大数据及其在电网公司的应用 [J]. 中国电机工程学报, 2014,34(20):85-92. Zhang P, Yang H F, Xu Y B, et al. Power big data and its application scenarios in power grid [J]. Proceedings of the CSEE, 2014,34(20): 85-92.
[24]
张山山,吴巧玲,王仁雷,等.基于“互联网+”的火电厂环保智能监管系统研究与应用 [J]. 华电技术, 2020,42(1):20-24. Zhang S S, Wu Q L, Wang R L, et al. Research and application of environmental intelligent supervision system for thermal power plants based on“Internet +” [J]. Huadian Technology, 2020,42(1):20-24.
[25]
雒 军,唐 坚,赵 喆,等.基于大数据的电力环保数据平台建设 [J]. 电力大数据, 2020,23(1):58-63. Luo J, Tang J, Zhao Z, et al. Construction of Power Environmental Protection Data Platform Based on Big Data [J]. Power Systems and Big Data, 2020,23(1):58-63.
[26]
张英杰,孔少飞,汤莉莉,等.基于在线监测的江苏省大型固定燃煤源排放清单及其时空分布特征 [J]. 环境科学, 2015,36(8):9:2775-2783. Zhang Y J, Kong S F, Tang L L, et al. Analysis on Emission Inventory and Temporal-Spatial Characteristics of Pollutants from Key Coal-Fired Stationary Sources in Jiangsu Province by OnLine Monitoring Data [J]. Environmental Science, 2015,36(8):9:2775-2783.
[27]
胡 雪,王 鑫,刘启贞,等.典型大气污染源动态排放清单编制方法及应用研究 [J]. 中国环境监测, 2020,36(5):54-62. Hu X, Wang X, Liu Q Z, et al. Research on the technique and application of compiling dynamic emission inventory of Typical Air Pollution Sources [J]. Environmental Monitoring in China, 2020, 36(5):54-62.
清华大学.城市大气污染源排放清单编制技术手册 [EB/OL]. https://max.book118.com/html/2018/1116/8107025055001133.shtm. Tsinghua University. Technical Manual for Urban Air Pollution Source Emission Inventory [EB/OL]. https://max.book118.com/html/2018/1116/8107025055001133.shtm.
[30]
Chou M D, Suarez M J, Ho C H, et al: Parameterizations for cloud overlapping and shortwave single-scattering properties for use in general circulation and cloud ensemble models [J]. Climate, 1998,11: 202-214.
[31]
Mlawer E J, Taubman S J, Brown P D, et al. Radiative transfer for inhomogeneous atmospheres: RRTM, a validated correlated-k model for the longwave [J]. Journal of Geophysical Research: Atmospheres, 1997,102(D14):16663-16682.
[32]
Kain J S. The Kain-Fritsch convective parameterization: an update [J]. Journal of Applied Meteorology and Climatology, 2004,43(1):170-181.
[33]
Pleim J E. A combined local and nonlocal closure model for the atmospheric boundary layer. Part II: Application and Evaluation in a mesoscale meteorological model [J]. Journal of Applied Meteorology and Climatology, 2007.46(9):1396-1409.
[34]
Xiu A J, Pleim J E. Development of a land surface model. part I: application in a mesoscale meteorological model [J]. Journal of Applied Meteorology and Climatology, 2001,40(2):192-209.
[35]
Hong S Y, Lim J O J. The WRF single-moment 6-class mcrophysics scheme (WSM6) [J]. Asia-pacific Journal of Atmospheric Sciences, 2006,42:129-151.
[36]
Jena C, Ghude S D, Beig G, et al. Inter comparison of different NOx emission inventories and associated variation in simulated surface ozone in Indian region [J]. Atmospheric Environment, 2015,117:61-73.
[37]
曹天慧,王 哲,张 晶,陈学舜,等.“9·3”阅兵期间协同减排措施对北京市大气PM2.5质量浓度及其来源影响的数值模拟 [J]. 北京师范大学学报(自然科学版), 2017,53(2):201-207. Cao T H, Wang Z, Zhang J, et al. Coordinated emission reduction measures for atmospheric PM2.5 in Beijing during the parade on September 3 [J]. Journal of Beijing Normal University (Nature Science), 2017,53(2):201-207.
[38]
伯 鑫,阚 慧,陈金胜,等.中国电力行业大气污染物排放时间特征谱研究 [C]//2017中国环境科学学会科学与技术年会论文集(第一卷), 2017:798-803. Bo X, Kan H, Chen J S, et al. Study on time temporal profile of air pollutant emission from power industry in China [C]//2017 Annual Conference of Science and Technology, Chinese Society of Environmental Sciences (Vol.1), 2017:798-803.
[39]
Zhang M D, Chen W W, Shen X J, et al. Comprehensive and high-resolution emission inventory of atmospheric pollutants for the northernmost cities agglomeration of Harbin-Changchun, China: Implications for local atmospheric environment management [J]. Journal of Environmental Sciences, 2021,104:150-168.
[40]
冉海潮,雷团团,伯 鑫,等.基于管理数据的工业源排放清单校核研究-以沧州为例 [J]. 环境影响评价, 2019,41(4):46-54. Ran H C, Lei T T, Bo X, et al. Research on the verification of industrial source emission inventory considering environmental management data: taking Cangzhou as an example [J]. Environmental impact assessment, 2019,41(4):46-54.
[41]
Tang L, Xue X D, Jia M, et al. Iron and steel industry emissions and contribution to the air quality in China [J]. Atmospheric Environment, 2020,237:117668.
[42]
段文娇,郎建垒,程水源,等.京津冀地区钢铁行业污染物排放清单及对PM2.5影响 [J]. 环境科学, 2018,38(4):1445-1454. Duan W J, Lang J L, Cheng S Y, et al. Air Pollutant Emission Inventory from Iron and Steel Industry in the Beijing-Tianjin-Hebei Region and Its Impact on PM2.5 [J]. Environmental Science, 2018,38(4):1445-1454.
[43]
Bo X, Li Z L, Qu J B, et al. The spatial-temporal pattern of sintered flue gas emissions in iron and steel enterprises of China [J]. Journal of Cleaner Production, 2020,266:121667.
[44]
唐山市统计局.2019年唐山市统计月报[EB/OL]. http://www.tangshan.gov.cn/zhuzhan/sjfb/ Tangshan Bureau of Statistics. Tangshan statistical monthly report 2019 [EB/OL]. http://www.tangshan.gov.cn/zhuzhan/sjfb/
[45]
US EPA (Environmental Protection Agency), 2007. Guidance on the Use of Models and Other Analyses for Demonstrating Attainment of Air Quality Goals for Ozone, PM2.5, and Regional Haze [EB/OL]. https://www.epa.gov/sites/default/files/2020-10/documents/final-03-pm-rh-guidance.pdf
[46]
Boylan J W, Russell A G. PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models [J]. Atmospheric Environment, 2005,40(26):4946-4959.
[47]
Emery C, Liu Z, Russell A G, et al. Recommendations on statistics and benchmarks to assess photochemical model performance [J]. Air Waste Management Association, 2017,67(5):582-598.
[48]
Zhang S X, Zhang Z Z, Li Y, et al. Formation processes and source contributions of ground-level ozone in urban and suburban Beijing using the WRF-CMAQ modelling system [J]. Journal of Environmental Science, 2023,127:753-766.
[49]
Abushammala M F M, Basir N E A, Basir H, et al. Regional landfills methane emission inventory in Malaysia [J]. Water Management & Research, 2011,29(8):863-873.