Estimation of biogenic VOCs emissions and its spatial-temporal distribution in Urumqi
ZHANG Lei1,2, JI Ya-qin1,2, ZHAO Jie1,2, WANG Xin-hua3, ZHANG Wei1,2, GUO Yu-hong4, WANG Shi-bao1,2
1. College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China;
2. State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, Tianjin 300350, China;
3. Chinese Research Academy of Environmental Sciences, Beijing 100012, China;
4. Xinjiang Environmental Monitoring Station, Urumqi 830011, China
Based on the data of land use, meteorological data, leaf area index and Palmer drought index of 2015, the GLOBEIS model was utilized to calculate the emissions of biogenic, and the emissions inventory of biogenic VOCs in Urumqi was established. The results showed that the total emissions of biogenic VOCs in 2015 was approximately 13750.72t, of which isoprene, monoterpene and other VOCs were 77.00t, 5057.51t and 8616.20t, accounting for 0.56%, 36.78% and 62.66%, respectively. The emissions intensity of the total emissions of the biogenic VOCs was 1.82t/(km2.a). The temporal distribution of VOCs emissions ranked summer > spring > autumn > winter; the spatial distribution of biogenic VOCs were mainly focused on the middle of Urumqi County, Dabancheng district and the south of Midong district.
张蕾, 姬亚芹, 赵杰, 王歆华, 张伟, 郭宇宏, 王士宝. 乌鲁木齐市天然源VOCs排放量估算与时空分布特征[J]. 中国环境科学, 2017, 37(10): 3692-3698.
ZHANG Lei, JI Ya-qin, ZHAO Jie, WANG Xin-hua, ZHANG Wei, GUO Yu-hong, WANG Shi-bao. Estimation of biogenic VOCs emissions and its spatial-temporal distribution in Urumqi. CHINA ENVIRONMENTAL SCIENCECE, 2017, 37(10): 3692-3698.
Hallquist M, Wenger J C, Baltensperger U, et al. The formation, properties and impact of secondary organic aerosol:current and emergingissues[J]. Atmospheric Chemistry & Physics, 2009,9(1):5155-5236.
Chameides W L, Lindsay R W, Richardson J, et al. The role of biogenic hydrocarbons in urban photochemical smog:Atlanta as a case study.[J]. Science, 1988,241(4872):1473-1475.
[5]
Guenther A B, Zimmerman P R, Harley P C, et al. Isoprene and monoterpene emission rate variability:Model evaluations and sensitivity analyses[J]. Journal of Geophysical Research Atmospheres, 1993,98(D7):12609-12617.
Skaltsas T, Avgouropoulos G, Tasis D. A global model of natural volatile organic compound emissions[J]. Journal of Geophysical Research, 1995,100(D5):8873-8892.
[10]
The global emission and interactions system (GLOBEIS)[EB/OL]. http://www.giobeis.com/about.html. 2015-03-12.
[11]
Guenther. Estimates of global terrestrial isoprene emissions using MEGAN (model of emissions of gases and aerosols from nature)[J]. Atmospheric Chemistry and Physics Discussions, 2006,6:3181-3210.
[12]
Guenther A, Geron C, Pierce T, et al. Natural emissions of non-methane volatile organic compounds, carbon monoxide, and oxides of nitrogen from North America[J]. Atmospheric Environment, 2000,34(12):2205-2230.
Zheng J, Zheng Z, Yu Y, et al. Temporal, spatial characteristics and uncertainty of biogenic VOC emissions in the Pearl River Delta region, China[J]. Atmospheric Environment, 2010,44(44):1960-1969.
[15]
Feldman M S, Howard T, Mcdonald-Buller E, et al. Applications of satellite remote sensing data for estimating biogenic emissions in southeastern Texas[J]. Atmospheric Environment, 2010,44(7):917-929.
[16]
Xiao Z, Liang S, Wang J, et al. Real-time retrieval of Leaf Area Index from MODIS time series data[J]. Remote Sensing of Environment, 2011,115(1):97-106.